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arXiv:cond-mat/0302135 · Physical review. B, Condensed matter

Magnetization plateaux in Bethe ansatz solvable spin- S ladders

M. Maslen, Murray T. Batchelor, Jan de Gier

Published Jul 29, 2003• 8 citations
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Abstract

We examine the properties of the Bethe ansatz solvable two- and three-leg spin-$S$ ladders. These models include Heisenberg rung interactions of arbitrary strength and thus capture the physics of the spin-$S$ Heisenberg ladders for strong rung coupling. The discrete values derived for the magnetization plateaux are seen to fit with the general prediction based on the Lieb-Schultz-Mattis theorem. We examine the magnetic phase diagram of the spin-1 ladder in detail and find an extended magnetization plateau at the fractional value $〈M〉=\frac{1}{2}$ in agreement with the experimental observation for the organic polyradical spin-1 ladder compound BIP-TENO.

DOI
10.1103/physrevb.68.024418

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We examine the properties of the Bethe ansatz solvable two- and three-leg spin-SSS ladders. These models include Heisenberg rung interactions of arbitrary strength and thus capture the physics of the spin-SSS Heisenberg ladders for strong rung coupling. The discrete values derived for the magnetization plateaux are seen to fit with the general prediction based on the Lieb-Schultz-Mattis theorem. We examine the magnetic phase diagram of the spin-1 ladder in detail and find an extended magnetization plateau at the fractional value 〈M〉=12〈M〉=\frac{1}{2}〈M〉=21​ in agreement with the experimental observation for the organic polyradical spin-1 ladder compound BIP-TENO.
We present a solvable ladder model which displays magnetization plateaus at fractional values of the total magnetization. Plateau signatures are also shown to exist along special lines. The model has isotropic Heisenberg interactions with additional many-body terms. The phase diagram can be calculated exactly for all values of the rung coupling and the magnetic field. We also derive the anomalous behavior of the susceptibility near the plateau boundaries. There is good agreement with the phase diagram obtained recently for the pure Heisenberg ladders by numerical and perturbative techniques.
This article considers recent advances in the investigation of the thermal and magnetic properties of integrable spin ladder models and their applicability to the physics of strong coupling ladder compounds. For this class of compounds the rung coupling J ⊥ is much stronger than the coupling J ∥ along the ladder legs. The ground state properties of the integrable two-leg spin- and the mixed spin-() ladder models at zero temperature are analysed by means of the Thermodynamic Bethe Ansatz (TBA). Solving the TBA equations yields exact results for the critical fields and critical behaviour. The thermal and magnetic properties of the models are discussed in terms of the recently introduced High Temperature Expansion (HTE) method, which is reviewed in detail. In the strong coupling region the integrable spin- ladder model exhibits three quantum phases: (i) a gapped phase in the regime , (ii) a fully polarized phase for , and (iii) a Luttinger liquid magnetic phase in the regime H c1<H<H c2. The critical behaviour in the vicinity of the critical points H c1 and H c2 is of Pokrovsky-Talapov type. The temperature-dependent thermal and magnetic properties are directly evaluated from the exact free energy expression and compared to known experimental results for the strong coupling ladder compounds (5IAP)2CuBr4· 2H2O, Cu2(C5H12N2)2Cl4, (C5H12N)2CuBr4, BIP-BNO and [Cu2(C2\O 2)(C10H8N2)2)](NO3)2. Similar analysis of the mixed spin-() ladder model reveals a rich phase diagram, with a and a full saturation magnetization plateau within the strong antiferromagnetic rung coupling regime. For weak rung coupling, the fractional magnetization plateau is diminished and a new quantum phase transition occurs. The phase diagram can be directly deduced from the magnetization curve obtained from the exact result derived from the TBA and HTE. The results are applied to the mixed ferrimagnetic ladder compound PNNBNO. The thermodynamics of the spin-orbital model with different single-ion anisotropies is also discussed. For this model single-ion anisotropy can trigger different quantum phase transitions within the spin and orbital degrees of freedom, with magnetization plateaux arising from different spin and orbit Landé g-factors.
In this paper we continue and extend a systematic study of plateaux in magnetization curves of antiferromagnetic Heisenberg spin-1/2 ladders. We first review a bosonic field-theoretical formulation of a single XXZ\mathrm{XXZ}XXZ chain in the presence of a magnetic field, which is then used for an Abelian bosonization analysis of NNN weakly coupled chains. Predictions for the universality classes of the phase transitions at the plateaux boundaries are obtained in addition to a quantization condition for the value of the magnetization on a plateau. These results are complemented by and checked against strong-coupling expansions. Finally, we analyze the strong-coupling effective Hamiltonian for an odd number NNN of cylindrically coupled chains numerically. For N=3N=3N=3 we explicitly observe a spin gap with a massive spinon-type fundamental excitation and obtain indications that this gap probably survives the limit $\stackrel{\ensuremath{\rightarrow}}{N}\ensuremath{\infty}$.
We analyze the phase diagram of a system of spin-1/2 Heisenberg antiferromagnetic chains interacting through a zig-zag coupling, also called zig-zag ladders. Using bosonization techniques we study how a spin-gap or more generally plateaux in magnetization curves arise in different situations. While for coupled XXZ chains, one has to deal with a recently discovered chiral perturbation, the coupling term which is present for normal ladders is restored by an external magnetic field, dimerization or the presence of charge carriers. We then proceed with a numerical investigation of the phase diagram of two coupled Heisenberg chains in the presence of a magnetic field. Unusual behaviour is found for ferromagnetic coupled antiferromagnetic chains. Finally, for three (and more) legs one can choose different inequivalent types of coupling between the chains. We find that the three-leg ladder can exhibit a spin-gap and/or non-trivial plateaux in the magnetization curve whose appearance strongly depends on the choice of coupling.
We investigate, at T =0, the magnetization process of the S =1 frustrated two-leg spin ladder having the leg interaction ( J ), the rung interaction ( J 0 ) and the diagonal interaction ( J d ), especially focusing on the appearance and the disappearance of the magnetization plateaux. We use the degenerate perturbation theory, the level spectroscopy analysis of the numerical diagonalization data and the DMRG. When J d =0, the M s /2 plateau ( M s is the saturation magnetization) appears for J 0 / J > 1.463. Then there is no M s /2 plateau for the so-called isotropic case J = J 0 . In case of J d > 0, J d helps the M s /2 plateau. And also, the M s /4 and (3/4) M s plateaux appear when J d is sufficiently large. These two plateaux are associated with the spontaneous breaking of the translation symmetry along the leg direction. We show the plateau phase diagram on the J d versus J plane, and also the magnetic phase diagram on the H versus J d plane for fixed J .
We study the T=0T=0T=0 magnetization of frustrated two-leg spin ladders with arbitrary value of the spin SSS. In the strong-rung limit, we use degenerate perturbation theory to prove that frustration leads to magnetization plateaus at fractional values of the magnetization for all spins SSS and to determine the critical ratios of parallel to diagonal inter-rung couplings for the appearance of these plateaus. These ratios depend both on the plateau and on the spin. To confirm these results and to investigate the properties of these ladders away from the strong-coupling limit, we have performed extensive density-matrix renormalization-group calculations for $S\ensuremath{\le}2$. For large enough inter-rung couplings, all plateaus simply disappear, leading to a magnetization curve typical of integer-spin chains in a magnetic field. The intermediate region turns out to be surprisingly rich however, with, upon increasing the inter-rung couplings, the development of magnetization jumps and, in some cases, the appearance of one or more phase transitions inside a given plateau.