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arXiv:cond-mat/0301489

Comment on ``Ramsey Fringes in a Bose-Einstein Condensate between Atoms and Molecules''

Eric Braaten, H.‐W. Hammer, Masaoki Kusunoki

Published Jan 24, 2003• 1 citation
arXivHTMLPDF

Abstract

In Phys. Rev. Lett. 89, 180401 (2002) [cond-mat/0204504], Kokkelmans and Holland interpret the results of a recent experiment at JILA that demonstrated atom-molecule coherence in a Bose-Einstein condensate. Using a mean-field approximation to a resonance field theory involving an atom condensate and a molecular condensate, they find that the molecular condensate is tiny compared to the atom condensate. We show that if the probability for the molecular field to create a diatomic molecule is correctly included, the numbers of atoms in the atom condensate and in the condensate of diatomic molecules are comparable.

DOI
10.48550/arxiv.cond-mat/0301489

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An evaluation of magnetic field and density dependence of the Josephson frequency in atom-Molecule Coherence in Bose gases and study of emergence of molecular Bose-Einstein condensate from a Fermi gas

Using the theoretical formalism of R A Duine and H T C Stoof (arXiv: cond-mat/0303230v) 22 March 2003), we have theoretically evaluated magnetic field and density dependence of the Josephson frequency in coherence atom-molecule oscillation in Bose-Einstein condensed gas.Our theoretically obtained results show that Josephson frequency increases with both magnetic field for constant condensate density and also with condensate density for fixed magnetic field.Our theoretically evaluated results are in good agreement with the experimental data and also with other theoretical workers.Using the theoretical formalism of Markes Greiner etal (Nature, 26 Nov (2005)) , we have studied the emergence of molecular Bose-Einstein condensate from a Fermi gas of 6 Li atoms.The study has been performed with the help of Feshbach resonance.We have evaluated molecular condensate fraction N0/N as a function of (T/TC) and as a function of (T/TF).We have also evaluated scattering length 'a' in unit of a0, of mixture of two lowest hyperfine states of 6 Li atom, temperature (µK) all as a function of magnetic field (mT) near the crossing of the An evaluation …

Journal of Chemical Biological and Physical Sciences•Jan 30, 2018•1 citation
In Phys. Rev. Lett. 89, 180401 (2002) [cond-mat/0204504], Kokkelmans and Holland interpret the results of a recent experiment at JILA that demonstrated atom-molecule coherence in a Bose-Einstein condensate. Using a mean-field approximation to a resonance field theory involving an atom condensate and a molecular condensate, they find that the molecular condensate is tiny compared to the atom condensate. We show that if the probability for the molecular field to create a diatomic molecule is correctly included, the numbers of atoms in the atom condensate and in the condensate of diatomic molecules are comparable.
We discuss the frequency and visibility of atom-molecule Ramsey fringes observed in recent experiments by Claussen et al. [Phys. Rev. A 67, 060701 (2003)]. In these experiments a 85Rb^{85}\mathrm{Rb}85Rb Bose-Einstein condensate was exposed to a sequence of magnetic field pulses on the high-field side of the 155G155\phantom{\rule{0.3em}{0ex}}\mathrm{G}155G Feshbach resonance. The observed oscillation frequencies largely agree with the theoretically predicted magnetic field dependence of the binding energy of the highest excited diatomic vibrational state, except for a small region very close to the singularity of the scattering length. Our analytic treatment of the experiment, as well as our dynamical simulations, follow the magnitude of the measured oscillation frequencies as well as the visibilities of the Ramsey fringes. We show that significant deviations from a purely binary dynamics, with an associated binding frequency, occur when the spatial extent of the molecular wave function becomes comparable with the mean distance between the atoms in the dilute gas. The experiments thus clearly identify the conditions under which diatomic molecules may be identified as a separate entity of the gas or, conversely, when the concept of binary physics in a many-body environment is bound to break down.
In this comment, we argue that the recent experiment of Ketterle and co-workers does not necessarily need to be interpreted as indicating that the true scattering amplitude between two molecules becomes small (8 nm measured vs. 120 nm predicted). Rather it can be interpreted as indicating that the energy of the achieved state is much lower than both the (variational) energy for a BCS state and the energy of a molecular condensate. In this sense, we suggest that the experiment may point to a novel many-body state, that is neither the BCS nor the molecular BEC state, and that still has to be identified.
Atom–molecule coherence in a Bose-Einstein condensate (BEC) has been demonstrated. Sudden changes were made to the magnetic field near a Feshbach resonance such that oscillations between atomic and molecular states were excited. The frequency of these oscillations was measured over a large range of magnetic fields and was found to be in excellent quantitative agreement with the predicted energy difference between two colliding atoms and the bound molecular state. This agreement indicates that we have created a quantum superposition of atoms and diatomic molecules, which are chemically different species. 1
We extend classical-field methods [Blakie et al., Adv. Phys. 57, 363 (2008)] to provide a description of atom-molecule systems. We use a model of Bose-Einstein condensation of atoms close to a Feshbach resonance, in which the tunable scattering length of the atoms is described using a system of coupled atom and molecule fields [Holland et al., Phys. Rev. Lett. 86, 1915 (2001)]. We formulate the basic theoretical methods for a coupled atom-molecule system, including the determination of the phenomenological parameters in our system, the Thomas-Fermi description of Bose-Einstein condensate, the Bogoliubov--de Gennes equations, and the Bogoliubov excitation spectrum for a homogenous condensed system. We apply this formalism to the special case of Bragg scattering from a uniform condensate and find that for moderate and large scattering lengths, there is a dramatic difference in the shift of the peak of the Bragg spectra, compared to that based on a structureless atom model. The result is compatible with the experimental results of Papp et al. [Phys. Rev. Lett 101, 135301 (2008)] for Bragg scattering from a nonuniform condensate.
Using the theoretical formalism of R A Duine and H T C Stoof (arXiv: cond-mat/0303230v) 22 March 2003), we have theoretically evaluated magnetic field and density dependence of the Josephson frequency in coherence atom-molecule oscillation in Bose-Einstein condensed gas.Our theoretically obtained results show that Josephson frequency increases with both magnetic field for constant condensate density and also with condensate density for fixed magnetic field.Our theoretically evaluated results are in good agreement with the experimental data and also with other theoretical workers.Using the theoretical formalism of Markes Greiner etal (Nature, 26 Nov (2005)) , we have studied the emergence of molecular Bose-Einstein condensate from a Fermi gas of 6 Li atoms.The study has been performed with the help of Feshbach resonance.We have evaluated molecular condensate fraction N0/N as a function of (T/TC) and as a function of (T/TF).We have also evaluated scattering length 'a' in unit of a0, of mixture of two lowest hyperfine states of 6 Li atom, temperature (µK) all as a function of magnetic field (mT) near the crossing of the An evaluation …