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arXiv:cond-mat/0212259 · Physical Review Letters

Full Aging in Spin Glasses

G. F. Rodriguez, G. G. Kenning, R. Orbach

Published Jul 15, 2003• 88 citations
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Abstract

The discovery of dynamic memory effects in the magnetization decays of spin glasses in 1983 marked a turning point in the study of the highly disordered spin glass state. Detailed studies of the memory effects have led to much progress in understanding the qualitative features of the phase space. Even so, the exact nature of the magnetization decay functions has remained elusive, causing confusion. In this Letter, we report strong evidence that the thermoremanent magnetization decays scale with the waiting time t(w). By employing a series of cooling protocols, we demonstrate that the rate at which the sample is cooled to the measuring temperature plays a major role in the determination of scaling. As the effective cooling time t(eff)(c) decreases, t/t(w) scaling improves and for t(eff)(c)<20 s we find almost perfect t/t(w) scaling, i.e., full aging.

DOI
10.1103/physrevlett.91.037203

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The discovery of dynamic memory effects in the magnetization decays of spin glasses in 1983 marked a turning point in the study of the highly disordered spin glass state. Detailed studies of the memory effects have led to much progress in understanding the qualitative features of the phase space. Even so, the exact nature of the magnetization decay functions has remained elusive, causing confusion. In this Letter, we report strong evidence that the thermoremanent magnetization decays scale with the waiting time t(w). By employing a series of cooling protocols, we demonstrate that the rate at which the sample is cooled to the measuring temperature plays a major role in the determination of scaling. As the effective cooling time t(eff)(c) decreases, t/t(w) scaling improves and for t(eff)(c)<20 s we find almost perfect t/t(w) scaling, i.e., full aging.
The deviations from full or pure aging behavior, i.e. perfect t/twt/t_wt/tw​ scaling of the correlation and response functions of aging glassy systems, are not well understood theoretically. Recent experiments of Rodriguez et al. (Phys. Rev. Lett. 91, 037203 (2003)) have shown that full aging applies to the thermoremanent magnetization in the limit of infinite cooling rate during the initial quench. In numerical models, instantaneous thermal quenches can be--and usually are--applied. This has motivated the present numerical investigations of the aging behavior of Edwards-Anderson Ising spin glass models with both short- and long-range Gaussian interactions, respectively. We sample the distribution of residence time ttt in suitably defined metastable valleys entered at age twt_wtw​, finding that the deviations from t/twt/t_wt/tw​ scaling are small and decrease systematically as the system size grows and/or the temperature decreases. Finally, the connection between this behavior and the scaling of the correlation function itself is discussed.
Aging phenomena have been studied in very different materials like polymers, supercooled liquids or disordered orientational crystals. We recall here the main features of aging in spin glasses, and use this example of magnetic systems as a guideline for the description of the others. A particular attention is put on the sensitivity of aging to the cooling rate and to temperature variations. This allows us to point out differences between temperature specific processes, yielding ``rejuvenation and memory effects'' as known in spin glasses, and domain growth processes, giving cumulative contributions at different temperatures. The relevance of wall depinning processes to rejuvenation and memory effects is discussed at the light of recent results on disordered ferromagnets.
We investigate the role of a magnetic field on the aging properties of spin glasses, focusing both on ac susceptibility measurements with an additional field variation and on thermoremanent magnetization (TRM) relaxation (to which the field variation is inherent). We propose a scaling of the TRM decay curves for various amplitudes of the magnetic field. Regarding aging as a random walk in a set of traps, we analyze the transient modification of the dynamics after a field change as twofold: an average reduction of relaxation times, well described by a Zeeman reduction of the energy barriers (hard traps), together with an ``emptying out'' of some other relaxation modes (fragile traps) corresponding to a partial quench effect. The fragile traps are associated with the longest time scales, that is to processes involving a large number of spins. A quantitative analysis of the results allows us to estimate a typical number of spins involved in both types of traps, as well as to discuss the growth of the energy barriers as a function of the number of spins.
Aging of two-dimensional (2D) Ising spin glasses with short-range interactions Rb2{\mathrm{Rb}}_{2}Rb2​${\mathrm{Cu}}_{1\mathrm{\ensuremath{-}}\mathit{x}}$Cox{\mathrm{Co}}_{\mathit{x}}Cox​F4{\mathrm{F}}_{4}F4​ (Tc{\mathit{T}}_{\mathit{c}}Tc​=0) is studied in the critical regime via the low-frequency ac susceptibility and via the dc magnetization for x=0.22 and 0.33. After quenching to low temperatures, slow logarithmic relaxation is observed for both the in-phase and out-of-phase ac susceptibilities. Using the droplet scaling model, the spin-glass correlation length R is concluded to increase after a temperature quench as R\ensuremath{\propto}(lnt${)}^{1/\mathrm{\ensuremath{\psi}}}$, with t in units of some microscopic time. The exponent \ensuremath{\psi}=1.0\ifmmode\pm\else\textpm\fi{}0.1 compares with recent theoretical results and numerical simulations for 2D short-range Ising spin glasses. The waiting-time dependence found for the field-cooled and zero-field-cooled dc magnetizations points to a markedly slower crossover from the quasiequilibrium to the nonequilibrium regime than in 3D. From experiments with different cooling histories, finally, the equilibrium spin-glass state is inferred to be strongly dependent on the temperature.
We consider the nonequilibrium behavior of the spin-glass ordered phase within the droplet scaling theory introduced previously. The fundamental long-time nonequilibrium process is assumed to be the thermally activated growth of spin-glass ordered domains. The remanent magnetization, m(t), in zero field is found to decay at long times as m(t)\ensuremath{\sim}${R}_{t}^{\mathrm{\ensuremath{-}}\ensuremath{\lambda}}$, where Rt{R}_{t}Rt​\ensuremath{\sim}(lnt${)}^{1/\ensuremath{\psi}}$ is the linear domain size, \ensuremath{\psi} is the previously introduced barrier exponent describing the growth of activation-barrier heights with length scale, and \ensuremath{\lambda} is a new nonequilibrium dynamic exponent, satisfying the relation \ensuremath{\lambda}\ensuremath{\ge}d/2 for d-dimensional systems. The effects of waiting for partial equilibration before making a measurement are studied in various regimes. The effects of quenching first to one temperature and then to another are also examined. Such experiments can, in principle, be used to obtain information about the relative rate of dynamic evolution as well as the overlap between the equilibrium states at different temperatures. In particular, the length scale ${L}_{\ensuremath{\Delta}T}$, below which equilibrium correlations at temperatures T and T+\ensuremath{\Delta}T are similar, plays an important role. The decay of m(t) and the growth of spin-glass order after a quench are examined in Monte Carlo simulations of the Sherrington-Kirkpatrick model.
Memory and rejuvenation effects in the magnetic response of off-equilibrium spin glasses have been widely regarded as the doorway into the experimental exploration of ultrametricity and temperature chaos (maybe the most exotic features in glassy free-energy landscapes). Unfortunately, despite more than twenty years of theoretical efforts following the experimental discovery of memory and rejuvenation, these effects have thus far been impossible to simulate reliably. Yet, three recent developments convinced us to accept this challenge: first, the custom-built Janus II supercomputer makes it possible to carry out "numerical experiments" in which the very same quantities that can be measured in single crystals of CuMn are computed from the simulation, allowing for parallel analysis of the simulation/experiment data. Second, Janus II simulations have taught us how numerical and experimental length scales should be compared. Third, we have recently understood how temperature chaos materializes in aging dynamics. All three aspects have proved crucial for reliably reproducing rejuvenation and memory effects on the computer. Our analysis shows that (at least) three different length scales play a key role in aging dynamics, while essentially all theoretical analyses of the aging dynamics emphasize the presence and the crucial role of a single glassy correlation length.