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arXiv:cond-mat/0211206 · Physical review. B, Condensed matter

Dynamics of short-time-scale energy relaxation of optical excitations due to electron-electron scattering in the presence of arbitrary disorder

Imre Varga, P. Thomas, T. Meier, S. W. Koch

Published Sep 23, 2003• 4 citations
arXivHTMLPDF

Abstract

A nonequilibrium occupation distribution relaxes towards the Fermi-Dirac distribution due to electron-electron scattering even in finite Fermi systems. The dynamic evolution of this thermalization process assumed to result from an optical excitation is investigated numerically by solving a Boltzmann equation for the carrier populations using a one-dimensional disordered system. We focus on the short-time-scale behavior. The logarithmically long time scale associated with the glassy behavior of interacting electrons in disordered systems is not treated in our investigation. For weak disorder and short range interaction we recover the expected result that the relaxation rate is enhanced by disorder. For sufficiently strong disorder, however, we find an opposite trend due to the reduction of scattering probabilities originating from the strong localization of the single-particle states. Long-range interaction in this regime produces a similar effect. The relaxation rate is found to scale with the interaction strength, however, the interplay between the implicit and the explicit character of the interaction produces an anomalous exponent.

DOI
10.1103/physrevb.68.113104

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A nonequilibrium occupation distribution relaxes towards the Fermi-Dirac distribution due to electron-electron scattering even in finite Fermi systems. The dynamic evolution of this thermalization process assumed to result from an optical excitation is investigated numerically by solving a Boltzmann equation for the carrier populations using a one-dimensional disordered system. We focus on the short-time-scale behavior. The logarithmically long time scale associated with the glassy behavior of interacting electrons in disordered systems is not treated in our investigation. For weak disorder and short range interaction we recover the expected result that the relaxation rate is enhanced by disorder. For sufficiently strong disorder, however, we find an opposite trend due to the reduction of scattering probabilities originating from the strong localization of the single-particle states. Long-range interaction in this regime produces a similar effect. The relaxation rate is found to scale with the interaction strength, however, the interplay between the implicit and the explicit character of the interaction produces an anomalous exponent.
Ultracold fermionic atoms in a disordered optical lattice can realize the disordered Fermi-Hubbard model, allowing investigations of the nature of strongly-correlated fermions in a minimal setting. This thesis describes two such studies. In the first, we observe the momentum relaxation of strongly-correlated fermions in the absence of disorder. We find a violation of the weak-scattering prediction for the scaling with temperature, which is analogous to the linear-in-temperature scaling of resistivity in substances called ``bad metals.'' In the second, we probe a disordered and strongly-correlated system using quenches of the interaction strength that take it far from equilibrium. We find that the relaxation of double occupancies following the quenches has distinct dynamical regimes controlled by the interplay of interactions and disorder. We present a minimal picture of the relaxation process that illustrates the origin of these regimes, which are related to the Mott--metal--Anderson transitions of the ground state at half-filling.
Abstract We study the relaxation of a non‐equilibrium carrier distribution under the influence of the electron‐electron interaction in the presence of disorder. Based on the Anderson model, our Hamiltonian is composed from a single particle part including the disorder and a two‐particle part accounting for the Coulomb interaction. We apply the equation‐of‐motion approach for the density matrix, which provides a fully microscopic description of the relaxation. Our results show that the nonequilibrium distribution in this closed and internally interacting system relaxes exponentially fast during the initial dynamics. This fast relaxation can be described by a phenomenological damping rate. The total single particle energy decreases in the redistribution process, keeping the total energy of the system fixed. It turns out that the relaxation rate decreases with increasing disorder. (© 2008 WILEY‐VCH Verlag GmbH & Co. KGaA, Weinheim)
Quench dynamics in a two-dimensional system of interacting fermions is analyzed within the semiclassical truncated Wigner approximation (TWA). The models with short-range and long-range interactions are considered. We show that in the latter case, the TWA is very accurate, becoming asymptotically exact in the infinite-range limit, provided that the semiclassical Hamiltonian is correctly identified. Within the TWA, different dynamical timescales of charges and spins can be clearly distinguished. Interestingly, for a weak and moderate disorder strength, we observe subdiffusive behavior of charges, while spins exhibit diffusive dynamics. At strong disorder, the quantum Fisher information shows logarithmic growth in time with a slower increase for charges than for spins. It is shown that in contrast to the short-range model, strong inhomogeneities such as domain walls in the initial state can significantly slow down thermalization dynamics, especially at weak disorder. This behavior can put additional challenges in designing cold-atom experimental protocols aimed to analyze possible many-body localization in such systems. While within this approach we cannot make any definite statements about the existence of a many-body localized phase, we see a very fast crossover as a function of disorder strength from rapidly thermalizing to a slow glassylike regime both for the short-range and long-range models.
The Luttinger liquid model, which describes interacting electrons in a single-channel quantum wire, is completely integrable in the absence of disorder and as such does not exhibit any relaxation to equilibrium. We consider relaxation processes induced by inelastic electron-electron interactions in a disordered Luttinger liquid, focusing on the equilibration rate and its essential differences from the electron-electron scattering rate as well as the rate of phase relaxation. In the first part of the paper, we review the basic concepts in a disordered Luttinger liquid at equilibrium. These include the elastic renormalization, dephasing, and interference-induced localization. In the second part, we formulate a conceptually important framework for systematically studying the nonequilibrium properties of a strongly correlated (non-Fermi) Luttinger liquid. We derive a coupled set of kinetic equations for the fermionic and bosonic distribution functions that describe the evolution of a nonequilibrium Luttinger liquid. Remarkably, the energy equilibration rate in the conducting disordered quantum wire (at sufficiently high temperature, when the localization effects are suppressed by dephasing) is shown to be on the order of the rate of elastic scattering off disorder, independent of the interaction constant and temperature.
We study the real-time dynamics of local occupation numbers in a one-dimensional model of spinless fermions with a random on-site potential for a certain class of initial states. The latter are thermal (mixed or pure) states of the model in the presence of an additional static force but become nonequilibrium states after a sudden removal of this static force. For this class and high temperatures, we show that the induced dynamics is given by a single correlation function at equilibrium, independent of the initial expectation values being prepared close to equilibrium (by a weak static force) or far away from equilibrium (by a strong static force). Remarkably, this type of universality holds true in both the ergodic phase and the many-body localized regime. Moreover, it does not depend on the specific choice of a unit cell for the local density. We particularly discuss two important consequences. First, the long-time expectation value of the local density is uniquely determined by the fluctuations of its diagonal matrix elements in the energy eigenbasis. Thus, the validity of the eigenstate thermalization hypothesis is not only a sufficient but also a necessary condition for thermalization. Second, the real-time broadening of density profiles is always given by the current autocorrelation function at equilibrium via a generalized Einstein relation. In the context of transport, we discuss the influence of disorder for large particle-particle interactions, where normal diffusion is known to occur in the disorder-free case. Our results suggest that normal diffusion is stable against weak disorder, while they are consistent with anomalous diffusion for stronger disorder below the localization transition. Particularly, for weak disorder, Gaussian density profiles can be observed for single disorder realizations, which we demonstrate for finite lattices up to 31 sites.
We examine electron-electron mediated relaxation following ultrafast electric field pump excitation of the fermionic degrees of freedom in the Falicov-Kimball model for correlated electrons. The results reveal a dichotomy in the temporal evolution of the system as one tunes through the Mott metal-to-insulator transition: in the metallic regime relaxation can be characterized by evolution toward a steady state well described by Fermi-Dirac statistics with an increased effective temperature; however, in the insulating regime this quasithermal paradigm breaks down with relaxation toward a nonthermal state with a complicated electronic distribution as a function of momentum. We characterize the behavior by studying changes in the energy, photoemission response, and electronic distribution as functions of time. This relaxation may be observable qualitatively on short enough time scales that the electrons behave like an isolated system not in contact with additional degrees of freedom which would act as a thermal bath, especially when using strong driving fields and studying materials whose physics may manifest the effects of correlations.