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arXiv:cond-mat/0210015

Quantum Phase Transitions in Models of Magnetic Impurities

R. Bulla, M. Vojta

Published Oct 1, 2002• 1 citation
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Abstract

Zero temperature phase transitions not only occur in the bulk of quantum systems, but also at boundaries or impurities. We review recent work on quantum phase transitions in impurity models that are generalizations of the standard Kondo model describing the interaction of a localized magnetic moment with a metallic fermionic host. Whereas in the standard case the moment is screened for any antiferromagnetic Kondo coupling as T to 0, the common feature of all systems considered here is that Kondo screening is suppressed due to the competition with other processes. This competition can generate unstable fixed points associated with phase transitions, where the impurity properties undergo qualitative changes. In particular, we discuss the coupling to both non-trivial fermionic and bosonic baths as well as two-impurity models, and make connections to recent experiments.

DOI
10.48550/arxiv.cond-mat/0210015

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Recent work is reviewed on continuous quantum phase transitions in impurity models, both with fermionic and bosonic baths – these transitions are interesting realizations of boundary critical phenomena at zero temperature. The models with fermion bath are generalizations of the standard Kondo model, with the common feature that Kondo screening of the localized spin can be suppressed due to competing processes. The models with boson bath are related to the spin–boson model of dissipative two-level systems, where the interplay between tunneling and friction results in multiple phases. The competition inherent to all models can generate unstable fixed points associated with quantum phase transitions, where the impurity properties undergo qualitative changes. Interestingly, certain impurity transitions feature both lower-critical and upper-critical “dimensions” and allow for epsilon-type expansions. Results are presented for a number of observables, obtained by both analytical and numerical renormalization group techniques, and connections made to experiments.
We investigate quantum impurity problems, where a local magnetic moment is coupled to the spin density of a bosonic environment, leading to bosonic versions of the standard Kondo and Anderson impurity models. In a physical situation, these bosonic environments can correspond either to deconfined spinons in certain classes of Z2{Z}_{2}Z2​ frustrated antiferromagnets, or to particles in a multicomponent Bose gase (in which case the spin degree of freedom is attributed to hyperfine levels). Using renormalization group techniques, we establish that our impurity models, which feature an exchange interaction analogous to Kondo impurities in Fermi liquids, allow flow toward a stable strong-coupling state. Since the low-energy bosons exist around a single point in momentum space, and there is no Fermi surface, an impurity quantum phase transition occurs at intermediate coupling, separating screened and unscreened phases. This behavior is qualitatively different from previously studied spin-isotropic variants of the spin-boson model, which display stable intermediate-coupling fixed points and no screening.
We revisit the physics of a Kondo impurity coupled to a fermionic host with a diverging power-law density of states near the Fermi level, $\ensuremath{\rho}(\ensuremath{\omega})\ensuremath{\sim}{|\ensuremath{\omega}|}^{r}$, with exponent $\ensuremath{-}1<r<0$. Using the analytical understanding of several fixed points, based partially on powerful mappings between models with bath exponents rrr and $(\ensuremath{-}r)$, combined with accurate numerical renormalization group calculations, we determine thermodynamic quantities within the stable phases and also near the various quantum phase transitions. Antiferromagnetic Kondo coupling leads to strong screening with a negative zero-temperature impurity entropy, while ferromagnetic Kondo coupling can induce a stable fractional spin moment. We formulate the quantum field theories for all critical fixed points of the problem, which are fermionic in nature and allow for a perturbative renormalization-group treatment.
We discuss the dynamics of magnetic moments in d-wave superconductors. In particular, we focus on moments induced by doping nonmagnetic impurities into cuprates. The interaction of such moments with the Bogoliubov quasiparticles of the superconductors can be described by variants of the pseudogap Kondo model, characterized by a power-law density of states at the Fermi level. The numerical renormalization-group technique is employed to investigate this Kondo problem for realistic band structures and particle-hole asymmetries, both at zero and finite temperatures. In particular, we study the boundary quantum phase transition between the local-moment and asymmetric strong-coupling phases, and argue that this transition has been observed in recent nuclear magnetic resonance experiments. We determine the spectral properties of both phases and the location of the critical point as a function of Kondo coupling and doping, and discuss quantum-critical crossovers near this phase transition. In addition, changes in the local density of states around the impurity are calculated as functions of temperature, being relevant to scanning tunneling microscopy experiments.
In a metal, a magnetic impurity is fully screened by the conduction electrons at low temperature. In contrast, impurity moments coupled to spin-1 bulk bosons, such as triplet excitations in paramagnets, are only partially screened, even at the bulk quantum critical point. We argue that this difference is not due to the quantum statistics of the host particles but instead related to the structure of the impurity-host coupling, by demonstrating that frustrated magnets with bosonic spinon excitations can display a bosonic version of the Kondo effect. However, the Bose statistics of the bulk implies distinct behavior, such as a weak-coupling impurity quantum phase transition, and perfect screening for a range of impurity spin values. We discuss implications of our results for the compound Cs2CuCl4, as well as possible extensions to multicomponent bosonic gases.
We discuss models of interacting magnetic impurities coupled to a metallic host, which show one or more boundary quantum phase transitions where the ground-state spin changes as a function of the interimpurity couplings. The simplest example is realized by two spin-12\frac{1}{2}21​ Kondo impurities coupled to a single orbital of the host. We investigate the phase diagram and crossover behavior of this model and present numerical renormalization-group results together with general arguments showing that the singlet-doublet quantum phase transition is either of first order or of the Kosterlitz-Thouless type, depending on the symmetry of the Kondo couplings. Thus we find an exponentially small energy scale within the Kondo regime, and a two-stage Kondo effect, in a single-channel situation. Connections to other models and possible applications are discussed.