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arXiv:cond-mat/0203171 · Physical review. B, Condensed matter

Ring exchange, the exciton Bose liquid, and bosonization in two dimensions

Arun Paramekanti, Leon Balents, Matthew P. A. Fisher

Published Aug 20, 2002• 193 citations
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Abstract

Motivated by the high-${T}_{c}$ cuprates, we consider a model of bosonic Cooper pairs moving on a square lattice via ring exchange. We show that this model offers a natural middle ground between a conventional antiferromagnetic Mott insulator and the fully deconfined fractionalized phase that underlies the spin-charge separation scenario for high-${T}_{c}$ superconductivity. We show that such ring models sustain a stable critical phase in two dimensions, the exciton Bose liquid (EBL). The EBL is a compressible state, with gapless but uncondensed boson and ``vortex'' excitations, power-law superconducting and charge-ordering correlations, and broad spectral functions. We characterize the EBL with the aid of an exact plaquette duality transformation, which motivates a universal low-energy description of the EBL. This description is in terms of a pair of dual bosonic phase fields, and is a direct analog of the well known one-dimensional bosonization approach. We verify the validity of the low-energy description by numerical simulations of the ring model in its exact dual form. The relevance to the high-${T}_{c}$ superconductors and a variety of extensions to other systems are discussed, including the bosonization of a two-dimensional fermionic ring model.

DOI
10.1103/physrevb.66.054526

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Motivated by the high-Tc{T}_{c}Tc​ cuprates, we consider a model of bosonic Cooper pairs moving on a square lattice via ring exchange. We show that this model offers a natural middle ground between a conventional antiferromagnetic Mott insulator and the fully deconfined fractionalized phase that underlies the spin-charge separation scenario for high-Tc{T}_{c}Tc​ superconductivity. We show that such ring models sustain a stable critical phase in two dimensions, the exciton Bose liquid (EBL). The EBL is a compressible state, with gapless but uncondensed boson and ``vortex'' excitations, power-law superconducting and charge-ordering correlations, and broad spectral functions. We characterize the EBL with the aid of an exact plaquette duality transformation, which motivates a universal low-energy description of the EBL. This description is in terms of a pair of dual bosonic phase fields, and is a direct analog of the well known one-dimensional bosonization approach. We verify the validity of the low-energy description by numerical simulations of the ring model in its exact dual form. The relevance to the high-Tc{T}_{c}Tc​ superconductors and a variety of extensions to other systems are discussed, including the bosonization of a two-dimensional fermionic ring model.
We investigate a hard-core boson model with ring-only exchanges on a square lattice, where a K1{K}_{1}K1​ term acts on 1$\ifmmode\times\else\texttimes\fi{}$1 plaquettes and a K2{K}_{2}K2​ term acts on 1$\ifmmode\times\else\texttimes\fi{}2and22 and 22and2\ifmmode\times\else\texttimes\fi{}$1 plaquettes, with a goal of realizing a novel exciton Bose liquid (EBL) phase first proposed by Paramekanti et al. [Phys. Rev. B 66, 054526 (2002)]. We construct Jastrow-type variational wave functions for the EBL, study their formal properties, and then use them as seeds for a projective quantum Monte Carlo study. Using the Green's function Monte Carlo approach, we obtain an unbiased phase diagram that at half-filling reveals a charge density wave for small K2{K}_{2}K2​, a valence bond solid for intermediate K2{K}_{2}K2​, and possibly for large K2{K}_{2}K2​ the EBL phase. Away from half-filling, the EBL phase is present for intermediate K2{K}_{2}K2​ and remains stable for a range of densities below 1/2 before phase separation occurs at lower densities.
We present a quantum Monte Carlo study of a hard-core boson model with ring-only exchanges on a square lattice, where a K1 term acts on 1×1 plaquettes and a K2 term acts on 1×2 and 2×1 plaquettes. At half-filling, the phase diagram reveals charge density wave for small K2, valence bond solid for intermediate K2, and possibly for large K2 the novel exciton Bose liquid (EBL) phase first proposed by Paramekanti et al [Phys. Rev. B 66, 054526 (2002)10.1103/PhysRevB.66.054526]. Away from half-filling, the EBL phase is present already for intermediate K2 and remains stable for a range of densities below 1/2 before phase separation sets in at lower densities.
We establish compelling evidence for the existence of new quasi-one-dimensional descendants of the ddd-wave Bose liquid (DBL), an exotic two-dimensional quantum phase of uncondensed itinerant bosons characterized by surfaces of gapless excitations in momentum space [O. I. Motrunich and M. P. A. Fisher, Phys. Rev. B 75, 235116 (2007)]. In particular, motivated by a strong-coupling analysis of the gauge theory for the DBL, we study a model of hard-core bosons moving on the NNN-leg square ladder with frustrating four-site ring exchange. Here, we focus on four- and three-leg systems where we have identified two novel phases: a compressible gapless Bose metal on the four-leg ladder and an incompressible gapless Mott insulator on the three-leg ladder. The former is conducting along the ladder and has five gapless modes, one more than the number of legs. This represents a significant step forward in establishing the potential stability of the DBL in two dimensions. The latter, on the other hand, is a fundamentally quasi-one-dimensional phase that is insulating along the ladder but has two gapless modes and incommensurate power-law transverse density-density correlations. While we have already presented results on this latter phase elsewhere [M. S. Block et al., Phys. Rev. Lett. 106, 046402 (2011)], we will expand upon those results in this work. In both cases, we can understand the nature of the phase using slave-particle-inspired variational wave functions consisting of a product of two distinct Slater determinants, the properties of which compare impressively well to a density matrix renormalization group solution of the model Hamiltonian. Stability arguments are made in favor of both quantum phases by accessing the universal low-energy physics with a bosonization analysis of the appropriate quasi-1D gauge theory. We will briefly discuss the potential relevance of these findings to high-temperature superconductors, cold atomic gases, and frustrated quantum magnets.
The guiding conception of vortex-condensation-driven Mott insulating behavior is central to the theory of the nodal liquid. We amplify our earlier description of this idea and show how vortex condensation in two-dimensional (2D) electronic systems is a natural extension of 1D Mott insulating and 2D bosonic Mott insulating behavior. For vortices in an underlying superconducting pair field, there is an important distinction between the condensation of flux hc/2ehc/2ehc/2e and flux hc/ehc/ehc/e vortices. The former case leads to spin-charge confinement, exemplified by the band insulator and the charge-density wave. In the latter case, spin and charge are liberated, leading directly to a 2D Mott insulator exhibiting spin-charge separation. Possible upshots include not only the nodal liquid, but also an undoped antiferromagnetic insulating phase with gapped excitations exhibiting spin-charge separation.
The exciton Bose liquid (EBL) is a hypothesized phase of bosons in 2+1D2+1\text{D}2+1D which possesses a dispersion that is gapless along the coordinate axes in momentum space. The low energy theory of the EBL involves modes on all length scales, extending all the way down to the lattice spacing. In this paper, we discuss a renormalization group scheme that can be used to address the stability of this and related phases of matter. We find that, in the absence of an extensively large symmetry group, realizing the simplest formulation of the EBL always requires fine-tuning. However, we also argue that the addition of certain marginal interactions can be used to realize a stable phase, without the need for fine-tuning. A simple generalization to 3+1D3+1\text{D}3+1D is also discussed.
Fermions in two dimensions, when subject to anisotropic spin-dependent hopping, can potentially give rise to unusual paired states in unpolarized mixtures that can behave as non-Fermi liquids. One possibility is a fully paired state with a gap for fermion excitations in which the Cooper pairs remain uncondensed. Such a ``Cooper-pair Bose-metal'' phase would be expected to have a singular Bose surface in momentum space. As demonstrated in the context of two-dimensional bosons hopping with a frustrating ring-exchange interaction, an analogous Bose-metal phase has a set of quasi-one-dimensional descendant states when put on a ladder geometry. Here we present a density matrix renormalization group study of the attractive Hubbard model with spin-dependent hopping on a two-leg ladder geometry. In our setup, one spin species moves preferentially along the leg direction, while the other does so along the rung direction. We find compelling evidence for the existence of a novel Cooper-pair Bose-metal phase in a region of the phase diagram at intermediate coupling. We further explore the phase diagram of this model as a function of hopping anisotropy, density, and interaction strength, finding a conventional superfluid phase as well as a phase of paired Cooper pairs with ddd-wave symmetry, similar to the one found in models of hard-core bosons with ring exchange. We argue that simulating this model with cold Fermi gases on spin-dependent optical lattices is a promising direction for realizing exotic quantum states.