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arXiv:cond-mat/0202227 · Journal of the Physical Society of Japan

Effects of Charge Ordering on Spin-Wave of Quarter-Filled Spin-Density-Wave States

Yuh Tomio, Yasunari Kurihara, Yoshikazu Suzumura

Published Apr 1, 2002• 4 citations
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Abstract

Spin-wave excitations of quarter-filled spin-density-wave state, which coexists with charge ordering, have been studied for one-dimensional extended Hubbard model with the nearest-neighbor repulsive interaction (V) and next-nearest-neighbor one (V_2). We calculate dispersion relations for the acoustic and optical spin-wave within the random phase approximation. Our numerical calculation shows that energy spectrum of the acoustic branch is well described by a simple sine function form. In the states coexisting with charge-density-wave, the spin-wave velocity decreases with increasing V or V_2. Our numerical result, that velocity reduces to zero in the limit of large V or V_2, is analyzed in terms of a spin 1/2 Heisenberg model with effective antiferromagnetic exchange interaction.

DOI
10.1143/jpsj.71.1174

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Spin-wave excitations of quarter-filled spin-density-wave state, which coexists with charge ordering, have been studied for one-dimensional extended Hubbard model with the nearest-neighbor repulsive interaction (V) and next-nearest-neighbor one (V_2). We calculate dispersion relations for the acoustic and optical spin-wave within the random phase approximation. Our numerical calculation shows that energy spectrum of the acoustic branch is well described by a simple sine function form. In the states coexisting with charge-density-wave, the spin-wave velocity decreases with increasing V or V_2. Our numerical result, that velocity reduces to zero in the limit of large V or V_2, is analyzed in terms of a spin 1/2 Heisenberg model with effective antiferromagnetic exchange interaction.
We study spin fluctuations in quarter-filled one-dimensional spin-density-wave systems in presence of short-range Coulomb interactions. By applying a path integral method, the spin-wave velocity is calculated as a function of on-site (U),(U),(U), nearest (V) and next-nearest (V2){(V}_{2})(V2​) neighbor-site interactions. With increasing V or V2,{V}_{2},V2​, the pure spin-density-wave state evolves into a state with coexisting spin- and charge-density waves. The spin-wave velocity is reduced when several density waves coexist in the ground state, and may even vanish at large V. The effect of dimerization along the chain is also considered.
The collective modes representing density fluctuation in a spin density wave (SDW) have been examined for a one-dimensional electron system of a quarter-filled extended Hubbard model with the next-nearest-neighbor interaction ( V 2 ). Within the random phase approximation (RPA), we obtain a new collective mode, which appears with increasing V 2 . The mode describes the relative motion between density wave with up spin and that with down spin. The gap in the excitation spectrum vanishes at a critical value of V 2 corresponding to the onset of the coexistence of 2 k F -SDW, 2 k F -charge density wave and 4 k F -SDW in the ground state ( k F being the Fermi wave vector).
Several kinds of spin density wave (SDW) states with both quarter-filled band and dimerization are reexamined for a one-dimensional system with on-site, nearest-neighbor and next-nearest-neighbor repulsive interactions, which has been investigated by Kobayashi et al. (J. Phys. Soc. Jpn. 67 (1998) 1098). Within the mean-field theory, the ground state and the response to the density variation are calculated in terms of phase variables, θθθ and ϕϕϕ, where θθθ expresses the charge fluctuation of SDW and ϕϕϕ describes the relative motion between density wave with up spin and that with down spin respectively. It is shown that the exotic state of coexistence of 2k_F-SDW and 2k_F-charge density wave (CDW) is followed by 4k_F-SDW but not by 4k_F-CDW where k_F denotes a Fermi wave vector. The harmonic potential with respect to the variation of θθθ and/or ϕϕϕ disappears for the interactions, which lead to the boundary between the pure 2k_F-SDW state and the corresponding coexistent state.
We study stripe orders of charge and spin density waves in the extended Hubbard model with the nearest-neighbor Coulomb repulsion V within the mean field approximation. We obtain V vs. T(temperature) phase diagram for the on-site Coulomb interaction U/t=8.0 and the filling n=0.8, here t is a nearest-neighbor transfer energy. Our result shows that the diagonal stripe spin density wave state (SDW) is stable for small V, but for large V the most stable state changes to a charge density wave-antiferromagnetic (CDW-AF) state. Especially we find at low temperature and for a certain range of value of V, a vertical stripe CDW-AF state becomes stable.
We examine effects of the next-nearest-neighbor repulsion on electronic states of a one-dimensional interacting electron system which consists of quarter-filled band and interactions of on-site and nearest-neighbor repulsion. We derive the effective Hamiltonian for the electrons around wave number $\pm \kf$ ($\kf$: Fermi wave number) and apply the renormalization group method to the bosonized Hamiltonian. It is shown that the next-nearest-neighbor repulsion makes $4\kf$-charge ordering unstable and suppresses the spin fluctuation. Further the excitation gaps and spin susceptibility are also evaluated.
We study the one-dimensional extended Hubbard model with alternating size of the hopping integrals using the density-matrix renormalization group method. We calculate the spin gap, the Tomonaga-Luttinger parameter, and the charge-density-wave order parameter for various dimerizations, interaction strengths, and band fillings. At half band-filling the spin and charge excitations are gapped but these gaps disappear for infinitesimal hole doping. At quarter filling, the umklapp scattering in the half-filled lower Peierls band generates a gap for the charge excitations but the gapless spin excitations can be described in terms of an effective antiferromagnetic Heisenberg model. Beyond a critical strength for the nearest-neighbor interaction, the dimerized extended Hubbard model at quarter filling develops a charge-density-wave ground state. The dimerization and the nearest-neighbor Coulomb interaction strongly reduce the Tomonaga-Luttinger parameter from its value for the bare Hubbard model. We discuss the relevance of our findings for the Bechgaard salts.