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arXiv:cond-mat/0106355

Breakdown of Migdal-Eliashberg theory in the infinite-dimensional Holstein model

J. P. Hague, N. d’Ambrumenil

Published Jun 18, 2001• 0 citations
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Abstract

We investigate the applicability of Migdal--Eliashberg (ME) theory by revisiting Migdal's analysis within the dynamical mean-field theory framework. First, we compute spectral functions, the quasi-particle weight, the self energy, renormalised phonon frequency and resistivity curves of the half-filled Holstein model. We demonstrate how ME theory has a phase-transition-like instability at intermediate coupling, and how the Engelsberg--Schrieffer (ES) picture is complicated by low-energy excitations from higher order diagrams (demonstrating that ES theory is a very weak coupling approach). Through consideration of the lowest-order vertex correction, we analyse the applicability of ME theory close to this transition. We find a breakdown of the theory in the intermediate coupling adiabatic limit due to a divergence in the vertex function. The region of applicability is mapped out, and it is found that ME theory is only reliable in the weak coupling adiabatic limit, raising questions about the accuracy of recent analyses of cuprate superconductors which do not include vertex corrections.

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We investigate the applicability of Migdal--Eliashberg (ME) theory by revisiting Migdal's analysis within the dynamical mean-field theory framework. First, we compute spectral functions, the quasi-particle weight, the self energy, renormalised phonon frequency and resistivity curves of the half-filled Holstein model. We demonstrate how ME theory has a phase-transition-like instability at intermediate coupling, and how the Engelsberg--Schrieffer (ES) picture is complicated by low-energy excitations from higher order diagrams (demonstrating that ES theory is a very weak coupling approach). Through consideration of the lowest-order vertex correction, we analyse the applicability of ME theory close to this transition. We find a breakdown of the theory in the intermediate coupling adiabatic limit due to a divergence in the vertex function. The region of applicability is mapped out, and it is found that ME theory is only reliable in the weak coupling adiabatic limit, raising questions about the accuracy of recent analyses of cuprate superconductors which do not include vertex corrections.
The normal state of the Holstein model is studied at half-filling in infinite dimensions and in the adiabatic regime. The dynamical mean-field equations are solved using perturbation expansions around the extremal paths of the effective action for the atoms. We find that the Migdal-Eliashberg expansion breaks down in the metallic state if the electron-phonon coupling $\ensuremath{\lambda}$ exceeds a value of about 1.3 in spite of the fact that the formal expansion parameter $\ensuremath{\lambda}{\ensuremath{\omega}}_{0}{/E}_{F} ({\ensuremath{\omega}}_{0}$ is the phonon frequency, EF{E}_{F}EF​ the Fermi energy) is much smaller than 1. The breakdown is due to the appearance of more than one extremal path of the action. We present numerical results which illustrate in detail the evolution of the local Green's function, the self-energy, and the effective atomic potential as a function of $\ensuremath{\lambda}.$
It is widely believed that in the adiabatic limit the Fermi liquid state of an electron-phonon system, described by Migdal-Eliashberg theory, remains stable until the dressed phonon softens. Our variational and analytic analysis of the prototypical Holstein model shows that, in a wide range of fillings both in 3D and 2D, a polaronic/bipolaronic state emerges before phonon softening; at small filling in 3D this happens already at weak coupling. We show that a polaronic/bipolaronic state emerges, upon increasing coupling, via an intermediate pseudogap-type mixed state, in which some fermions retain Fermi liquid behavior, yet Luttinger's theorem is violated. At even larger couplings the density of states gradually approaches its form in the atomic limit.
We present a method for solving impurity models with electron-phonon coupling, which treats the phonons efficiently and without approximations. The algorithm is applied to the Holstein-Hubbard model in the dynamical mean field approximation, where it allows access to strong interactions, very low temperatures, and arbitrary fillings. We show that a renormalized Migdal-Eliashberg theory provides a reasonable description of the phonon contribution to the electronic self-energy in strongly doped systems, but fails if the quasiparticle energy becomes of order of the phonon frequency.
It is widely believed that in the adiabatic limit the Fermi liquid state of an electron-phonon system, described by Migdal-Eliashberg theory, remains stable until the dressed phonon softens. Our variational and analytic analysis of the prototypical Holstein model shows that, in a wide range of fillings both in 3D and 2D, a polaronic/bipolaronic state emerges before phonon softening; at small filling in 3D this happens already at weak coupling. We show that a polaronic/bipolaronic state emerges, upon increasing coupling, via an intermediate pseudogap-type mixed state, in which some fermions retain Fermi liquid behavior, yet Luttinger's theorem is violated. At even larger couplings the density of states gradually approaches its form in the atomic limit.
We examine the range of validity of the second-order cumulant expansion (CE) for the calculation of spectral functions, quasiparticle properties, and mobility of the Holstein polaron. We devise an efficient numerical implementation that allows us to make comparisons in a broad interval of temperature, electron-phonon coupling, and phonon frequency. For a benchmark, we use the dynamical mean-field theory which gives, as we have recently shown, rather accurate spectral functions in the whole parameter space, even in low dimensions. We find that in one dimension, the CE resolves well both the quasiparticle and the first satellite peak in a regime of intermediate coupling. At high temperatures, the charge mobility assumes a power law $\ensuremath{\mu}\ensuremath{\propto}{T}^{\ensuremath{-}2}$ in the limit of weak coupling and $\ensuremath{\mu}\ensuremath{\propto}{T}^{\ensuremath{-}3/2}$ for stronger coupling. We find that, for stronger coupling, the CE gives slightly better results than the self-consistent Migdal approximation (SCMA), while the one-shot Migdal approximation is appropriate only for a very weak electron-phonon interaction. We also analyze the atomic limit and the spectral sum rules. We derive an analytical expression for the moments in CE and find that they are exact up to the fourth order, as opposed to the SCMA where they are exact to the third order. Finally, we analyze the results in higher dimensions.