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arXiv:cond-mat/0106037 · Physical review. B, Condensed matter

Haldane-gapped spin chains as Luttinger liquids: Correlation functions at finite field

Robert Konik, Paul Fendley

Published Oct 29, 2002• 53 citations
arXivHTMLPDF

Abstract

We study the behavior of Heisenberg, antiferromagnetic, integer-spin chains in the presence of a magnetic field exceeding the attendant spin gap. For temperatures much smaller than the gap, the spin chains exhibit Luttinger liquid behavior. We compute exactly both the corresponding Luttinger parameter and the Fermi velocity as a function of magnetic field. This enables the computation of a number of correlators from which we derive the spin conductance, the expected form of the dynamic structure factor relevant to inelastic neutron-scattering experiments, and NMR relaxation rates. We also comment upon the robustness of the magnetically induced gapless phase both to finite temperature and finite couplings between neighboring chains.

DOI
10.1103/physrevb.66.144416

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We study the finite temperature, low energy, long wave-length spectrum of the dynamic structure factor of the spin-1/21/21/2 antiferromagnetic Heisenberg chain in the presence of exchange anisotropy and external magnetic fields. Using imaginary-time quantum Monte-Carlo we extract parameters, relevant to characterize a {\it renormalized} Luttinger liquid. For small momentum our results are consistent with a change from propagating spinon density waves to spin diffusion, described by a finite-frequency spin-current relaxation rate. Results for this relaxation rate as well as other Luttinger liquid parameters are presented versus temperature, momentum, magnetic field, and anisotropy, including finite-size analysis, and checks for anomalous diffusion. Our results are consistent with exact diagonalization and Bethe Ansatz, where available, and with corroborate findings of other previous studies using bosonization, transfer matrix renormalization group, and quantum Monte-Carlo.
We study the ground-state spin correlations in the gapless incommensurate regime of a S=1/2S=1/2S=1/2 XXZ\mathrm{XXZ}XXZ chain and a two-leg antiferromagnetic ladder under a magnetic field, in which the gapless excitations form a Tomonaga-Luttinger (TL) liquid. We calculate numerically the two-spin correlation functions and the local magnetization in the two models using the density-matrix renormalization-group method. By fitting the numerical results for an open XXZ\mathrm{XXZ}XXZ chain of 100 spins to correlation functions of a Gaussian model, we determine the TL-liquid parameter K and the amplitudes of the correlation functions. The value of K estimated from the fits is in excellent agreement with the exact value obtained from the Bethe ansatz. We apply the same method to the open ladder consisting of 200 spins and determine the dependence of K on the magnetization M. The $K\ensuremath{-}M$ relation changes drastically depending on the ratio of the coupling constants in the leg and rung directions. We also discuss implications of these results to experiments on the nuclear spin relaxation rate 1/T1{1/T}_{1}1/T1​ and dynamical spin structure factors.
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We have studied the zero- and low-temperature behaviors of anisotropic alternating antiferromagnetic-ferromagnetic Heisenberg spin-12\frac{1}{2}21​ chains in a transverse magnetic field. Using the analytical spinless fermion approach, the thermodynamic behavior of the model has been studied. We have introduced a different order parameter to distinguish the gapless Luttinger liquid phase from the other gapped phases. The exact diagonalization Lanczos results are also used to compare with the spinless fermion ones. We have found a double peak structure in the specific-heat curves for the region between the two quantum critical points. Using the numerical full diagonalization results, the existence of the double peak structure is confirmed.
Inelastic neutron scattering is employed to study transverse spin correlations of a Heisenberg S=1/2S=1/2S=1/2 chain compound in a magnetic field of 7.5 T. The target compound is the antiferromagnetic Heisenberg S=1/2S=1/2S=1/2 chain material 2(1,4-dioxane)$\ifmmode\cdot\else\textperiodcentered\fi{}2({\mathrm{H}}_{2}\mathrm{O})\ifmmode\cdot\else\textperiodcentered\fi{}{\mathrm{CuCl}}_{2}$, or CuDCl for short. The validity and the limitations of the scaling relation for the transverse dynamic structure factor are tested, discussed, and compared to the Tomonaga-Luttinger spin liquid theory and to Bethe-ansatz results for the Heisenberg model.