arXiv:cond-mat/0105096 · Physical review. B, Condensed matter
Magnetism of a tetrahedral cluster spin chain
Wolfram Brenig, K. W. Becker
Abstract
We discuss the magnetic properties of a dimerized and completely frustrated tetrahedral spin-1/2 chain. Using a combination of exact diagonalization and bond-operator theory the quantum phase diagram is shown to incorporate a singlet product, a dimer, and a Haldane phase. In addition we consider one- and two-triplet excitations in the dimer phase and evaluate the magnetic Raman cross section which is found to be strongly renormalized by the presence of a two-triplet bound state. The link to a novel tellurate materials is clarified.