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arXiv:cond-mat/0003040

Breakdown of the Onsager reaction field theory in two dimensions

Avinash Kumar Singh

Published Mar 3, 2000• 1 citation
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Abstract

It is shown that for the spin 1/2 anisotropic Heisenberg model the result for the transition temperature is completely insensitive to the anisotropy within the Onsager reaction field theory, which yields a vanishing T_c in two dimensions, in total conflict with the expected finite T_c, increasing with anisotropy. This establishes that the breakdown of the Onsager reaction field theory in two dimensions is not limited to the Ising model, but actually extends over the whole range of anisotropy. Therefore, for the isotropic case, the results of vanishing T_c and exponential dependence of spin correlation length should be seen as mere coincidence.

DOI
10.48550/arxiv.cond-mat/0003040

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It is shown that for the spin 1/2 anisotropic Heisenberg model the result for the transition temperature is completely insensitive to the anisotropy within the Onsager reaction field theory, which yields a vanishing T_c in two dimensions, in total conflict with the expected finite T_c, increasing with anisotropy. This establishes that the breakdown of the Onsager reaction field theory in two dimensions is not limited to the Ising model, but actually extends over the whole range of anisotropy. Therefore, for the isotropic case, the results of vanishing T_c and exponential dependence of spin correlation length should be seen as mere coincidence.
The anisotropic Heisenberg model has been investigated by interpolating anisotropy between the Ising and isotropic Heisenberg limits via general spin high temperature series (HTS) for the zero-field susceptibility of the ferromagnets for the square lattice. This is done by locating the critical temperature ( T c (2) ) and the susceptibility exponent (γ) from the analysis of the series by Pade approximant and ratio methods. The critical temperature is found to be spin dependent. It decreases as anisotropy changes from the Ising limit towards the isotropic limit and remains finite (lower than that of Stanley and Kaplan) for all the spins except for S =1/2 at the isotropic limit. Exponent γ is almost Ising like for the anisotropic system and anomalous jump in it occurs for the isotropic case. In addition, expressions for the magnetization are derived by using spin-wave theory. The limit of complete isotropy has been found not to be a special case for the susceptibility, in contrast to magnetization.
A real-space effective-field renormalization-group method (ERFG) recently derived for computing critical properties of Ising spins is extended to treat the quantum spin-1/2 anisotropic Heisenberg model. The formalism is based on a generalized but approximate Callen–Suzuki spin relation and utilizes a convenient differential operator expansion technique. The method is illustrated in several lattice structures by employing its simplest approximation version in which clusters with one (N′=1) and two (N=2) spins are used. The results are compared with those obtained from the standard mean-field (MFRG) and Migdal–Kadanoff (MKRG) renormalization-group treatments and it is shown that this technique leads to rather accurate results. It is shown that, in contrast with the MFRG and MKRG predictions, the EFRG, besides correctly distinguishing the geometries of different lattice structures, also provides a vanishing critical temperature for all two-dimensional lattices in the isotropic Heisenberg limit. For the simple cubic lattice, the dependence of the transition temperature Tc with the exchange anisotropy parameter Δ [i.e., Tc(Δ)], and the resulting value for the critical thermal crossover exponent φ [i.e., Tc≂Tc(0)+AΔ1/φ ] are in quite good agreement with results available in the literature in which more sophisticated treatments are used.
The anisotropic two-dimensional Ising model in the presence of a magnetic field is studied within two different approaches: the effective-field theory (EFT) with correlation and the Bethe-Peierls (BP) approximation. The model consists of ferromagnetic interaction (Jx)({J}_{x})(Jx​) in the xxx direction and antiferromagnetic interaction (Jy)({J}_{y})(Jy​) in the yyy direction. The phase diagram in the $T\text{\ensuremath{-}}H$ plane is obtained for the particular case Jx=Jy{J}_{x}={J}_{y}Jx​=Jy​. Special focus is given in the low-temperature region of the phase diagram, where a first-order phase transition is observed using the mean-field approximation, which is in disagreement with the linear chain approximation (LCA). Our results indicate a second-order phase transition for all values of H∕J∊[0,2]H∕J∊[0,2]H∕J∊[0,2], with the presence of a reentrant behavior only observed in the BP approximation in accordance with the results of the LCA and exact solution. The null field critical temperature is an increasing function of r=Jy∕Jxr={J}_{y}∕{J}_{x}r=Jy​∕Jx​, and in the $r\ensuremath{\rightarrow}0$ limit we have found, using BP and EFT, the approximate form ${k}_{B}{T}_{N}∕{J}_{x}\ensuremath{\simeq}A∕\mathrm{ln}(1∕r)$ in accordance with the exact result of Onsager.
Within a real-space renormalization-group framework, the spin-\textonehalf{} Heisenberg ferromagnet in the presence of an Ising-like anisotropy on a self-dual hierarchical lattice is discussed. The results are exact for this lattice but can also be considered as a quite satisfactory approximation for the simple square one. The controversial point on how Tc{T}_{c}Tc​ vanishes in the isotropic Heisenberg limit is analyzed: Quite strong evidence is presented favoring a continuous function of anisotropy. The crossover from the isotropic Heisenberg model to the pure Ising one is exhibited.
Onsager reaction field theory is used to investigate the one-dimensional ferromagnetic long-range interacting spin chain with the antiferromagnetic nearest-neighbor interaction (NNI) [Formula: see text]. The ferromagnetic long-range interactions considered in this paper decay as [Formula: see text] with the distance [Formula: see text] between lattice sites. It is found that both the zero temperature and finite-temperature phase diagrams of the system are strongly affected by the interplay between ferromagnetic long-range and antiferromagnetic NNIs. The critical temperature and the uniform susceptibility are obtained as a function of [Formula: see text] and [Formula: see text]. At finite temperatures and in the region [Formula: see text] in which [Formula: see text] is dependent of [Formula: see text], the ferromagnetic-paramagnetic phase transition survives for [Formula: see text] and no phase transition exists for [Formula: see text]. At [Formula: see text], the ferromagnetic-antiferromagnetic phase transition happens at zero temperature for [Formula: see text]. The ground state of the system keeps ferromagnetic when [Formula: see text]. But for [Formula: see text], the system becomes antiferromagnetic at all temperatures.