Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

arXiv:cond-mat/0002095

Influence of center-of-mass correlations on spontaneous emission and Lamb shift in dense atomic gases

Michael Fleischhauer

Published Feb 7, 2000• 0 citations
arXivHTMLPDF

Abstract

Local field effects on the rate of spontaneous emission and Lamb shift in a dense gas of atoms are discussed taking into account correlations of atomic center-of-mass coordinates. For this the exact retarded propagator in the medium is calculated in independent scattering approximation and employing a virtual-cavity model. The resulting changes of the atomic polarizability lead to modifications of the medium response which can be of the same order of magnitude but of opposite sign than those due to local field corrections of the dielectric function derived by Morice, Castin, and Dalibard [Phys.Rev.A 51, 3896 (1995)].

DOI
10.48550/arxiv.cond-mat/0002095

Related papers

Spontaneous emission and level shifts in absorbing disordered dielectrics and dense atomic gases: A Green’s-function approach

Michael Fleischhauer

Spontaneous emission and Lamb shift of atoms in absorbing dielectrics and dense atomic gases are discussed using a microscopic Green's-function approach. Uncorrelated and random atomic positions are assumed, and the associated unphysical interactions between different atoms at the same location are eliminated (local field correction). For the case of an atom in a purely dispersive medium, the spontaneous-emission rate is altered by the well-known Lorentz local-field factor. When the mean distance between atoms becomes less than the resonance wavelength, results different from previously suggested expressions are found. In particular, it is shown that nearest-neighbor interactions become important. The results suggest that, for large densities, absorbing disordered dielectrics cannot accurately be described by a macroscopic approach that neglects correlations between atomic positions.

arXiv:quant-ph/9902076•Physical Review A•Sep 1, 1999•44 citations

Local-field approach to the interaction of an ultracold dense Bose gas with a light field

Konstantin V. Krutitsky, Frank Burgbacher, Jürgen Audretsch

The propagation of the electromagnetic field of a laser through a dense Bose gas is examined and nonlinear operator equations for the motion of the center of mass of the atoms are derived. The goal is to present a self-consistent set of coupled Maxwell-Bloch equations for atomic and electromagnetic fields generalized to include the atomic center-of-mass motion. Two effects are considered. The ultracold gas forms a medium for the Maxwell field which modifies its propagation properties. Combined herewith is the influence of the dipole-dipole interaction between atoms which leads to a density-dependent shift of the atomic transition frequency. It is expressed in a position-dependent detuning and is the reason for the nonlinearity. This results in a direct and physically transparent way from the quantum field-theoretical version of the local-field approach to electrodynamics in quantum media. The equations for the matter fields are general. Previously published nonlinear equations are obtained as limiting cases. As an atom-optical application the scattering of a dense beam of a Bose gas is studied in the Raman-Nath regime. The main conclusion is that for increasing density of the gas the dipole-dipole interaction suppresses or enhances the scattering depending on the sign of the detuning.

arXiv:quant-ph/9811049•Physical Review A•Feb 1, 1999•27 citations

Radiative atom-atom interactions in optically dense media: Quantum corrections to the Lorentz-Lorenz formula

Michael Fleischhauer, Susanne F. Yelin

Generalized single-atom Maxwell-Bloch equations for optically dense media are derived taking into account noncooperative radiative atom-atom interactions. Applying a Gaussian approximation and formally eliminating the degrees of freedom of the quantized radiation field and of all but a probe atom leads to an effective time-evolution operator for the probe atom. The mean coherent amplitude of the local field seen by the atom is shown to be given by the classical Lorentz-Lorenz relation. The second-order correlations of the field lead to terms that describe relaxation or pump processes and level shifts due to multiple scattering or reabsorption of spontaneously emitted photons. In the Markov limit a nonlinear and nonlocal single-atom density matrix equation is derived. To illustrate the effects of the quantum corrections, we discuss amplified spontaneous emission and radiation trapping in a dense ensemble of initially inverted two-level atoms and the effects of radiative interactions on intrinsic optical bistability in coherently driven systems.

arXiv:quant-ph/9809087•Physical Review A•Mar 1, 1999•73 citations

Electro-optical effects in dense and cold atomic gases

Igor M. Sokolov

On the basis of the general theoretical approach developed previously by Fofanov et al. [Ya. A. Fofanov et al., Phys. Rev. A 84, 053811 (2011)], we analyze the atomic polarization created by weak monochromatic light in an optically thick, dense, and cold atomic ensemble placed in an electrostatic field. On this basis, we determine complex refractive indexes and the permittivity tensor of the medium. We analyze the dispersion of the permittivity and its dependence on the strength of the field and on the density of the medium. We show that electro-optic effects in dilute and cold gases differ essentially from those in dense ones. In the latter case, electric field modifies the shape, amplitude, and typical linewidth of the atomic resonance. The electric field also modifies the collective Lamb shift. Observed peculiarities are explained as a result of the indirect influence of the field on optical properties of dense gases through modification of polyatomic collective effects caused by interatomic dipole-dipole interactions.

Physical Review A•Jul 17, 2018•8 citations

Quantum local-field corrections and spontaneous decay

Stefan Scheel, L. Knöll, Dirk‐Gunnar Welsch +1 more

A recently developed scheme [S. Scheel, L. Kn\"oll, and D.-G. Welsch, Phys. Rev. A 58, 700 (1998)] for quantizing the macroscopic electromagnetic field in linear dispersive and absorbing dielectrics satisfying the Kramers-Kronig relations is used to derive the quantum local-field correction for the standard virtual-sphere-cavity model. The electric and magnetic local-field operators are shown to become approximately consistent with QED only if the polarization noise is fully taken into account. It is shown that the polarization fluctuations in the local field can dramatically change the spontaneous decay rate, compared with the familiar result obtained from the classical local-field correction. In particular, the spontaneous emission rate strongly depends on the radius of the local-field virtual cavity.

arXiv:quant-ph/9811067•Physical Review A•Aug 1, 1999•85 citations

Spontaneous emission in dielectrics

Peter W. Milonni

The theory of spontaneous emission in dielectric media is extended to take proper account of dispersion and local field corrections. For the case of spontaneous emission in a plasma or radiative electron-hole recombination in a semiconductor, there are effectively no local field corrections. A shift of emission lines due to a dispersive host medium is predicted and interpreted. The corrections to spontaneous and stimulated emission due to dielectric interfaces in microcavity lasers are discussed.

Bulletin of the American Physical Society•May 1, 1993•0 citations
Local field effects on the rate of spontaneous emission and Lamb shift in a dense gas of atoms are discussed taking into account correlations of atomic center-of-mass coordinates. For this the exact retarded propagator in the medium is calculated in independent scattering approximation and employing a virtual-cavity model. The resulting changes of the atomic polarizability lead to modifications of the medium response which can be of the same order of magnitude but of opposite sign than those due to local field corrections of the dielectric function derived by Morice, Castin, and Dalibard [Phys.Rev.A 51, 3896 (1995)].
Spontaneous emission and Lamb shift of atoms in absorbing dielectrics and dense atomic gases are discussed using a microscopic Green's-function approach. Uncorrelated and random atomic positions are assumed, and the associated unphysical interactions between different atoms at the same location are eliminated (local field correction). For the case of an atom in a purely dispersive medium, the spontaneous-emission rate is altered by the well-known Lorentz local-field factor. When the mean distance between atoms becomes less than the resonance wavelength, results different from previously suggested expressions are found. In particular, it is shown that nearest-neighbor interactions become important. The results suggest that, for large densities, absorbing disordered dielectrics cannot accurately be described by a macroscopic approach that neglects correlations between atomic positions.
The propagation of the electromagnetic field of a laser through a dense Bose gas is examined and nonlinear operator equations for the motion of the center of mass of the atoms are derived. The goal is to present a self-consistent set of coupled Maxwell-Bloch equations for atomic and electromagnetic fields generalized to include the atomic center-of-mass motion. Two effects are considered. The ultracold gas forms a medium for the Maxwell field which modifies its propagation properties. Combined herewith is the influence of the dipole-dipole interaction between atoms which leads to a density-dependent shift of the atomic transition frequency. It is expressed in a position-dependent detuning and is the reason for the nonlinearity. This results in a direct and physically transparent way from the quantum field-theoretical version of the local-field approach to electrodynamics in quantum media. The equations for the matter fields are general. Previously published nonlinear equations are obtained as limiting cases. As an atom-optical application the scattering of a dense beam of a Bose gas is studied in the Raman-Nath regime. The main conclusion is that for increasing density of the gas the dipole-dipole interaction suppresses or enhances the scattering depending on the sign of the detuning.
Generalized single-atom Maxwell-Bloch equations for optically dense media are derived taking into account noncooperative radiative atom-atom interactions. Applying a Gaussian approximation and formally eliminating the degrees of freedom of the quantized radiation field and of all but a probe atom leads to an effective time-evolution operator for the probe atom. The mean coherent amplitude of the local field seen by the atom is shown to be given by the classical Lorentz-Lorenz relation. The second-order correlations of the field lead to terms that describe relaxation or pump processes and level shifts due to multiple scattering or reabsorption of spontaneously emitted photons. In the Markov limit a nonlinear and nonlocal single-atom density matrix equation is derived. To illustrate the effects of the quantum corrections, we discuss amplified spontaneous emission and radiation trapping in a dense ensemble of initially inverted two-level atoms and the effects of radiative interactions on intrinsic optical bistability in coherently driven systems.
On the basis of the general theoretical approach developed previously by Fofanov et al. [Ya. A. Fofanov et al., Phys. Rev. A 84, 053811 (2011)], we analyze the atomic polarization created by weak monochromatic light in an optically thick, dense, and cold atomic ensemble placed in an electrostatic field. On this basis, we determine complex refractive indexes and the permittivity tensor of the medium. We analyze the dispersion of the permittivity and its dependence on the strength of the field and on the density of the medium. We show that electro-optic effects in dilute and cold gases differ essentially from those in dense ones. In the latter case, electric field modifies the shape, amplitude, and typical linewidth of the atomic resonance. The electric field also modifies the collective Lamb shift. Observed peculiarities are explained as a result of the indirect influence of the field on optical properties of dense gases through modification of polyatomic collective effects caused by interatomic dipole-dipole interactions.
A recently developed scheme [S. Scheel, L. Kn\"oll, and D.-G. Welsch, Phys. Rev. A 58, 700 (1998)] for quantizing the macroscopic electromagnetic field in linear dispersive and absorbing dielectrics satisfying the Kramers-Kronig relations is used to derive the quantum local-field correction for the standard virtual-sphere-cavity model. The electric and magnetic local-field operators are shown to become approximately consistent with QED only if the polarization noise is fully taken into account. It is shown that the polarization fluctuations in the local field can dramatically change the spontaneous decay rate, compared with the familiar result obtained from the classical local-field correction. In particular, the spontaneous emission rate strongly depends on the radius of the local-field virtual cavity.
The theory of spontaneous emission in dielectric media is extended to take proper account of dispersion and local field corrections. For the case of spontaneous emission in a plasma or radiative electron-hole recombination in a semiconductor, there are effectively no local field corrections. A shift of emission lines due to a dispersive host medium is predicted and interpreted. The corrections to spontaneous and stimulated emission due to dielectric interfaces in microcavity lasers are discussed.