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arXiv:chao-dyn/9706026 · Physical Review Letters

Spontaneous Emission in Chaotic Cavities

T. Sh. Misirpashaev, Piet W. Brouwer, C. W. J. Beenakker

Published Sep 8, 1997• 10 citations
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Abstract

The spontaneous emission rate $\ensuremath{\gamma}$ of a two-level atom inside a chaotic cavity fluctuates strongly from one point to another because of fluctuations in the local density of modes. For a cavity with perfectly conducting walls and an opening containing $N$ wave channels, the distribution of $\ensuremath{\gamma}$ is given by $P(\ensuremath{\gamma})\ensuremath{\propto}{\ensuremath{\gamma}}^{N/2\ensuremath{-}1}(\ensuremath{\gamma}+{\ensuremath{\gamma}}_{0}{)}^{\ensuremath{-}N\ensuremath{-}1}$, where ${\ensuremath{\gamma}}_{0}$ is the free-space rate. For small $N$ the most probable value of $\ensuremath{\gamma}$ is much smaller than the mean value ${\ensuremath{\gamma}}_{0}$.

DOI
10.1103/physrevlett.79.1841

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The spontaneous emission rate \ensuremathγ\ensuremath{\gamma}\ensuremathγ of a two-level atom inside a chaotic cavity fluctuates strongly from one point to another because of fluctuations in the local density of modes. For a cavity with perfectly conducting walls and an opening containing NNN wave channels, the distribution of \ensuremathγ\ensuremath{\gamma}\ensuremathγ is given by P(\ensuremathγ)\ensuremath∝\ensuremathγN/2\ensuremath−1(\ensuremathγ+\ensuremathγ0)\ensuremath−N\ensuremath−1P(\ensuremath{\gamma})\ensuremath{\propto}{\ensuremath{\gamma}}^{N/2\ensuremath{-}1}(\ensuremath{\gamma}+{\ensuremath{\gamma}}_{0}{)}^{\ensuremath{-}N\ensuremath{-}1}P(\ensuremathγ)\ensuremath∝\ensuremathγN/2\ensuremath−1(\ensuremathγ+\ensuremathγ0​)\ensuremath−N\ensuremath−1, where \ensuremathγ0{\ensuremath{\gamma}}_{0}\ensuremathγ0​ is the free-space rate. For small NNN the most probable value of \ensuremathγ\ensuremath{\gamma}\ensuremathγ is much smaller than the mean value \ensuremathγ0{\ensuremath{\gamma}}_{0}\ensuremathγ0​.
We revisit the problem of spontaneous emission by a two-level system in a cavity, concentrating in particular on those aspects associated with the finite propagation time of light between the atom and the cavity boundaries. We find that spontaneous emission always occurs first at the free space rate and there is then an abrupt change in these dynamics when light reflected by the cavity mirrors returns to the atom, leading to interference effects that result either in an enhancement or a reduction of this rate or in a periodic exchange of excitation between the atom and the cavity field. From this point of view, reversible spontaneous emission in terms of single-mode ``vacuum Rabi oscillations'' can be interpreted as resulting from the interference between the multimode partial waves reflected at the cavity mirrors and the instantaneously radiated light. \textcopyright{} 1996 The American Physical Society.
We show that the spontaneous emission of a moving atom inside a cavity is modified by two different mechanisms. The first one is a Doppler-induced detuning of the cavity line that leads to observable changes in the spontaneous emission rate for atomic velocities in excess of a characteristic velocity vcav{\mathit{v}}_{\mathrm{cav}}vcav​=c/Q, Q being the quality factor of the cavity. In addition, spatial mode effects can lead to a temporal modulation of the exponential decay rate. This modulation is observable for velocities that do not exceed another characteristic velocity vmod{\mathit{v}}_{\mathrm{mod}}vmod​ which is typically several orders of magnitude smaller than vcav{\mathit{v}}_{\mathrm{cav}}vcav​.
A brief review is given of theoretical and experimental investigations of the spontaneous emission from an atom in a resonator cavity. A theory of spontaneous emission from a two-level atom in free space and in a cavity is presented in a methodical unified manner. In a single-mode resonator the structure of the spectrum of the emitted photons is a singlet or a doublet, depending on the ratio of the cavity damping to the constant of the interaction of an atom with a field. The emission spectrum of an atom in a cavity with two modes with similar frequencies may have a triplet structure.
Introduction Ever since 1916/17 when Einstein argued [45] [46] that spontaneous emission must occur if matter and radiation are to achieve thermal equilibrium, physicists have believed that spontaneous emission is an inherent quantum mechanical property of atoms and that excited atoms inevitably radiate. This view, however, overlooks the fact that spontaneous emission is a consequence of the coupling of quantized energy states of atoms with the quantized radiation field, and is a manifestation of quantum noise or of emission ‘stimulated’ by ‘vacuum fluctuations’. An infinity of vacuum states is available to the photon radiated by an excited atom placed in free space, leading to the effective irreversibility of such emissions. If these vacuum states are modified, as for example by placing an excited atom between closely spaced mirrors or in a small cavity (essentially the Casimir effect), spontaneous emission can be greatly inhibited or enhanced or even made reversible. Recent advances in atomic and optical techniques have made it possible to control and manipulate spontaneous emission. A whole new branch of quantum optics called ‘cavity QED’ has developed since 1987 utilizing these dramatic changes in spontaneous emission rates in cavities to construct new kinds of microscopic masers or micromasers that operate with a single atom and a few photons or with photons emitted in pairs in a two-photon transition.