The coherent storage and phase modulation of x-ray single-photon wave packets in the resonant scattering of light off nuclei is theoretically investigated. We show that by switching off and on again the magnetic field in the nuclear sample, phase-sensitive storage of photons in the keV regime can be achieved. Corresponding π phase modulation of the stored photon can be accomplished if the retrieving magnetic field is rotated by 180°. The development of such x-ray single-photon control techniques is a first step towards forwarding quantum optics and quantum information to shorter wavelengths and more compact photonic devices.The coherent storage and phase modulation of x-ray single-photon wave packets in the resonant scattering of light off nuclei is theoretically investigated. We show that by switching off and on again the magnetic field in the nuclear sample, phase-sensitive storage of photons in the keV regime can be achieved. Corresponding π phase modulation of the stored photon can be accomplished if the retrieving magnetic field is rotated by 180°. The development of such x-ray single-photon control techniques is a first step towards forwarding quantum optics and quantum information to shorter wavelengths and more compact photonic devices.

arXiv:1205.5503Physical Review LettersNov 9, 201258 citations

Quantum and Nonlinear Optics with Hard X-Rays

Ralf Röhlsberger, Jörg Evers, S. Shwartz

Springer eBooksJan 1, 20161 citation

Quantum and Nonlinear Optics with Hard X-Rays

Ralf Röhlsberger, Jörg Evers, S. Shwartz

Springer eBooksJan 1, 20154 citations

Generation of Short Hard-X-Ray Pulses of Tailored Duration Using a Mössbauer Source

Wang, G., Liao, W.

We theoretically investigate a scheme for the generation of single hard-x-ray pulses of controllable duration in the range of 1–100 ns from a radioactive Mössbauer source. The scheme uses a magnetically perturbed 57FeBO3 crystal illuminated with recoilless 14.4-keV photons from a 57Co radioisotope nuclide. Such a compact x-ray source is useful for the extension of quantum optics to the 10-keV energy scale, which has been in the spotlight in recent years. So far, experimental achievements have mostly been attained in synchrotron radiation facilities. However, the use of tabletop and portable hard-x-ray sources for time-resolved measurements and for implementing coherent control over nuclear quantum-optics systems has still been limited. The availability of compact hard-x-ray sources may become the engine for the application of quantum-information schemes down to the subatomic scale. We demonstrate that the present method is versatile and provides an economic solution, utilizing a Mössbauer source, to perform time-resolved nuclear scattering, to produce suitable pulses for photon storage, and to flexibly generate x-ray single-photon entanglement.We theoretically investigate a scheme for the generation of single hard-x-ray pulses of controllable duration in the range of 1–100 ns from a radioactive Mössbauer source. The scheme uses a magnetically perturbed 57FeBO3 crystal illuminated with recoilless 14.4-keV photons from a 57Co radioisotope nuclide. Such a compact x-ray source is useful for the extension of quantum optics to the 10-keV energy scale, which has been in the spotlight in recent years. So far, experimental achievements have mostly been attained in synchrotron radiation facilities. However, the use of tabletop and portable hard-x-ray sources for time-resolved measurements and for implementing coherent control over nuclear quantum-optics systems has still been limited. The availability of compact hard-x-ray sources may become the engine for the application of quantum-information schemes down to the subatomic scale. We demonstrate that the present method is versatile and provides an economic solution, utilizing a Mössbauer source, to perform time-resolved nuclear scattering, to produce suitable pulses for photon storage, and to flexibly generate x-ray single-photon entanglement.

Jul 6, 201810 citations

Quantum and Nonlinear Optics with Hard X-Rays

Ralf Röhlsberger, Jörg Evers, S. Shwartz

Springer eBooksJan 1, 202011 citations

Transient coherent phase modulation of nuclear states via a high-repetition-rate laser

Nan Xue, Haohan Shi, Kailin Zhang +1 more

Advancements in x-ray sources extend the scope of light-matter interactions into the x-ray-nuclear regime. Precise temporal control of quantum phases provides fundamental insights into quantum systems and serves as a cornerstone for numerous quantum technologies. Nevertheless, achieving phase control of quantum systems with high temporal and spatial resolution remains a substantial challenge in the realm of hard x-ray quantum optics due to the ultrashort oscillation periods of photons. In this study, we propose to manipulate the magnetic properties of a thin $^{57}\text{Fe}$ film using near-infrared (NIR) pulses characterized by a high repetition rate. By calculating the evolution of quantum beats, we can theoretically extract the phase information of the nuclear response. Coherence within the nuclear ensemble is preserved throughout the entire process. This control scheme achieves quantum shifts with zeptosecond precision and modulates the spectral line shape within the frequency domain. Our proposal introduces a high-resolution method for rapidly manipulating nuclear states using optical laser pulses.Advancements in x-ray sources extend the scope of light-matter interactions into the x-ray-nuclear regime. Precise temporal control of quantum phases provides fundamental insights into quantum systems and serves as a cornerstone for numerous quantum technologies. Nevertheless, achieving phase control of quantum systems with high temporal and spatial resolution remains a substantial challenge in the realm of hard x-ray quantum optics due to the ultrashort oscillation periods of photons. In this study, we propose to manipulate the magnetic properties of a thin $^{57}\text{Fe}$ film using near-infrared (NIR) pulses characterized by a high repetition rate. By calculating the evolution of quantum beats, we can theoretically extract the phase information of the nuclear response. Coherence within the nuclear ensemble is preserved throughout the entire process. This control scheme achieves quantum shifts with zeptosecond precision and modulates the spectral line shape within the frequency domain. Our proposal introduces a high-resolution method for rapidly manipulating nuclear states using optical laser pulses.

Physical Review AFeb 13, 20253 citations

^{57}\text{Fe}

film using near-infrared (NIR) pulses characterized by a high repetition rate. By calculating the evolution of quantum beats, we can theoretically extract the phase information of the nuclear response. Coherence within the nuclear ensemble is preserved throughout the entire process. This control scheme achieves quantum shifts with zeptosecond precision and modulates the spectral line shape within the frequency domain. Our proposal introduces a high-resolution method for rapidly manipulating nuclear states using optical laser pulses.