Quantum correlations arising from measurements on pairs of entangled particles are often referred to as the most non-classical feature of quantum mechanics. As such, they have found a role in many fundamental tests of quantum mechanics and most emerging applications in the field of quantum communication. The most well-known fundamental test is the Bell inequality. Its repeated violation in countless experiments has convinced physicists that local hidden variables cannot describe the correlations arising from measurements on entangled particles. On the application side, quantum correlations have been used in quantum key distribution, which aims to provably secure messages during transmission, and quantum repeaters, which are essential for future long-distance quantum communication. The main goal of this thesis was to use quantum entanglement for new fundamental studies and quantum communication applications. Towards this end, we developed a high-fidelity source of entanglement and used it in a fundamental test where we bounded the predictive power any physical theory could have about the outcomes of measurements on entangled particles. Secondly, we made use of entangling measurements to develop a new quantum cryptography system based on the promising MDI-QKD protocol, which protects users from otherwise undetectable hacking attacks. We developed a detailed model of MDI-QKD systems with which one can optimize any implementation, deployed our MDI-QKD system across the city of Calgary, and demonstrated the feasibility of this protocol and of long-distance entangling measurements. Thirdly, we have built a source of entanglement compatible with quantum memories, which is an essential ingredient of quantum repeaters. We then demonstrated several crucial steps towards a functioning quantum repeater, including the preservation of entanglement during storage and, more generally, the entire photonic wavefunction. While further work is required to bring our demonstrations to real-world applications, we are confident that they will prove useful in guiding future developments.
Quantum correlations arising from measurements on pairs of entangled particles are often referred to as the most non-classical feature of quantum mechanics. As such, they have found a role in many fundamental tests of quantum mechanics and most emerging applications in the field of quantum communication. The most well-known fundamental test is the Bell inequality. Its repeated violation in countless experiments has convinced physicists that local hidden variables cannot describe the correlations arising from measurements on entangled particles. On the application side, quantum correlations have been used in quantum key distribution, which aims to provably secure messages during transmission, and quantum repeaters, which are essential for future long-distance quantum communication. The main goal of this thesis was to use quantum entanglement for new fundamental studies and quantum communication applications. Towards this end, we developed a high-fidelity source of entanglement and used it in a fundamental test where we bounded the predictive power any physical theory could have about the outcomes of measurements on entangled particles. Secondly, we made use of entangling measurements to develop a new quantum cryptography system based on the promising MDI-QKD protocol, which protects users from otherwise undetectable hacking attacks. We developed a detailed model of MDI-QKD systems with which one can optimize any implementation, deployed our MDI-QKD system across the city of Calgary, and demonstrated the feasibility of this protocol and of long-distance entangling measurements. Thirdly, we have built a source of entanglement compatible with quantum memories, which is an essential ingredient of quantum repeaters. We then demonstrated several crucial steps towards a functioning quantum repeater, including the preservation of entanglement during storage and, more generally, the entire photonic wavefunction. While further work is required to bring our demonstrations to real-world applications, we are confident that they will prove useful in guiding future developments.
Quantum Key Distribution (QKD) has opened a new avenue for secure communication, by allowing one to distribute a random secret key between two users that are connected through a public channel without revealing information to unauthorized parties. If a message is encrypted with the one time pad (a well-known crytography algorithm) using secret keys created by QKD, then the ciphertext is information-theoretically secure and thus unbreakable for adversaries. Despite its unprecedented security, loss in the physical channel has prevented QKD from being used over distances beyond a few hundred kilometers. Fortunately, quantum repeaters have opened a path for long-distance QKD by providing a means to establish entanglement between distant users. The goal of this thesis has been to develop a source of entangled photon pairs that is suitable for quantum repeaters and then use it to test some of the fundamental building blocks of a quantum repeater : the heralded creation of entangled photons by means of entanglement swapping with properties that allow interfacing with optical quantum memories; the reversible mapping of quantum states from members of entangled photon pairs in and out of solid-state quantum memories; two-photon interference and a Bell state measurement with photons recalled from separate quantum memories. The demonstration of these key ingredients of a quantum repeater constitutes a significant step towards the establishment of entanglement over hundreds of kilometer distance, and hence long-distance QKD.
In this thesis, we investigate the uses of entanglement and its verification in quantum communication. Typically, it is the presence of entanglement which allows quantum communication protocols to outperform their classical counterparts, or to achieve tasks which are infeasible with classical physics. Therefore, the verification of entanglement can provide fundamental tests to certify that experimental implementations of such protocols operate quantum mechanically. The main object here is to develop a verification procedure which is adaptable to a wide range of applications, and whose implementation has low requirements on experimental resources. We present such a procedure in the form of the Expectation Value Matrix. The structure of this thesis is as follows: Chapters 1 and 2 give a short introduction and background information on quantum theory and the quantum states of light. In particular, we discuss the basic postulates of quantum mechanics, quantum state discrimination, the description of quantum light and the homodyne detector. Chapter 3 gives a brief introduction to quantum information and in particular to entanglement, and we discuss the basics of quantum key distribution and teleportation. The general framework of the Expectation Value Matrix is introduced. The main matter of this thesis is contained in the subsequent three chapters, which describe different quantum communication protocols and the corresponding adaptation of the entanglement verification method. The subject of Chapter 4 is quantum key distribution, where the detection of entanglement is a means of excluding intercept-resend attacks, and the presence of quantum correlations in the raw data is a necessary precondition for the generation of secret key. We investigate a continuous-variable version of the two-state protocol and develop the Expectation Value Matrix method for such qubit-mode systems. Furthermore, we analyse the role of the phase reference with respect to the security of the protocol and raise awareness of a corresponding security threat. For this, we adapt the verification method to different settings of Stokes operator measurements. In Chapter 5, we investigate quantum memory channels and propose a fundamental bench- mark for these based on the verification of entanglement. After describing some physical effects which can be used for the coherent storage of light, we focus on the storage of squeezed light. This situation requires an extension of our verification procedure to sources of mixed input states. We propose such an extension, and give a detailed analysis of its application to squeezed thermal states, displaced thermal states and mixed qubit states. This is supplemented by finding the optimal entanglement-breaking channels for each of these situations, which provides us with an indication of the strength of the extension to our entanglement criterion. The subject of Chapter 6 is also the benchmarking of quantum memory or teleportation experiments. Considering a number of recently published benchmark criteria, we investigate the question which one is most useful to actual experiments. For this, a criterion must be both strong, i.e., easy to overcome, and it must be implementable with a reasonable amount of experimental resources. We first compare the different criteria for typical settings and sort them according to their resilience to excess noise. Then, we introduce a further improvement to the Expectation Value Matrix method, which results in the desired optimal benchmark criterion. Finally, we investigate naturally occurring phase fluctuations and find them to further simplify the implementation of our criterion. Thus, we formulate the first truly useful way of validating experiments for the quantum storage or transmission of light.
One of the most fascinating recent developments in research has been how different disciplines have become more and more interconnected. So much so that fields as disparate as information theory and fundamental physics have combined to produce ideas for the next generation of computing and secure information technologies, both of which have far reaching consequences. For more than fifty years Moore's law, which describes the trend of the transistor's size shrinking by half every two years, has proven to be uncannily accurate. However, the computing industry is now approaching a fundamental barrier as the size of a transistor approaches that of an individual atom and the laws of physics and quantum mechanics take over. Rather then look at this as the end, quantum information science has emerged to ask the question of what additional power and functionality might be realized by harnessing some of these quantum effects. This thesis presents work on the sub-field of quantum cryptography which seeks to use quantum means in order to assure the security of ones communications. The beauty of quantum cryptographic methods are that they can be proven secure, now and indefinitely into the future, relying solely on the validity of the laws of physics for their proofs of security. This is something which is impossible for nearly all current classical cryptographic methods to claim. \n \nThe thesis begins by examining the first implementation of an entangled quantum key distribution system over two free-space optical links. This system represents the first test-bed of its kind in the world and while its practical importance in terrestrial applications is limited to a smaller university or corporate campus, the system mimics the setup for an entangled satellite system aiding in the study of distributing entangled photons from an orbiting satellite to two earthbound receivers. Having completed the construction of a second free-space link and the automation of the alignment system, I securely distribute keys to Alice and Bob in two distant locations separated by 1,575 m with no direct line-of-sight between them. I examine all of the assumptions necessary for my claims of security, something which is particularly important for moving these systems out of the lab and into commercial industry. I then go on to describe the free-space channel over which the photons are sent and the implementation of each of the major system components. I close with a discussion of the experiment which saw raw detected entangled photon rates of 565 s^{-1} and a quantum bit error rate (QBER) of 4.92% resulting in a final secure key rate of 85 bits/s. Over the six hour night time experiment I was able to generate 1,612,239 bits of secure key. \n \nWith a successful QKD experiment completed, this thesis then turns to the problem of improving the technology to make it more practical by increasing the key rate of the system and thus the speed at which it can securely encrypt information. It does so in three different ways, involving each of the major disciplines comprising the system: measurement hardware, source technology, and software post-processing. First, I experimentally investigate a theoretical proposal for biasing the measurement bases in the QKD system showing a 79% improvement in the secret key generated from the same raw key rates. Next, I construct a second generation entangled photon source with rates two orders of magnitude higher than the previous source using the idea of a Sagnac interferometer. More importantly, the new source has a QBER as low as 0.93% which is not only important for the security of the QKD system but will be required for the implementation of a new cryptographic primitive later. Lastly, I study the free-space link transmission statistics and the use of a signal-to-noise ratio (SNR) filter to improve the key rate by 25.2% from the same amount of raw key. The link statistics have particular relevance for a current project with the Canadian Space Agency to exchange a quantum key with an orbiting satellite - a project which I have participated in two feasibility studies for. \n \nWanting to study the usefulness of more recent ideas in quantum cryptography this thesis then looks at the first experimental implementation of a new cryptographic primitive called oblivious transfer (OT) in the noisy storage model. This primitive has obvious important applications as it can be used to implement a secure identification scheme provably secure in a quantum scenario. Such a scheme could one day be used, for example, to authenticate a user over short distances, such as at ATM machines, which have proven to be particularly vulnerable to hacking and fraud. Over a four hour experiment, Alice and Bob measure 405,642,088 entangled photon pairs with an average QBER of 0.93% allowing them to create a secure OT key of 8,939,150 bits. As a first implementer, I examine many of the pressing issues currently preventing the scheme from being more widely adopted such as the need to relax the dependance of the OT rate on the loss of the system and the need to extend the security proof to cover a wider range of quantum communication channels and memories. It is important to note that OT is fundamentally different than QKD for security as the information is never physically exchanged over the communication line but rather the joint equality function f(x) = f(y) is evaluated. Thus, security in QKD does not imply security for OT. \n \nFinally, this thesis concludes with the construction and initial alignment of a second generation free-space quantum receiver, useful for increasing the QKD key rates, but designed for a fundamental test of quantum theory namely a Svetlichny inequality violation. Svetlichny's inequality is a generalization of Bell's inequality to three particles where any two of the three particles maybe be non-locally correlated. Even so, a violation of Svetlichny's inequality shows that certain quantum mechanical states are incompatible with this restricted class of non-local yet realistic theories. Svetlichny's inequality is particularly important because while there has been an overwhelming number of Bell experiments performed testing two-body correlations, experiments on many-body systems have been few and far between. Experiments of this type are particularly valuable to explore since we live in a many-body world. The new receiver incorporates an active polarization analyzer capable of switching between measurement bases on a microsecond time-scale through the use of a Pockels cell while maintaining measurements of a high fidelity. Some of the initial alignment and analysis results are detailed including the final measured contrasts of 1:25.2 and 1:22.6 in the rectilinear and diagonal bases respectively.
Quantum cryptography uses the quantum properties of individual photons to provide two or more users with means to communicate securely and efficiently. Specifically, quantum key distribution (QKD) focuses on the secure communication between two distant parties and guarantees the security of a transmitted message between them. Although QKD is the most mature application of quantum cryptography, applications of quantum mechanics in communication systems are not limited to QKD and other cryptographic protocols can be implemented as well. This thesis focuses on the implementation of quantum cryptographic systems over deployed fiber. A first QKD system was built and used to demonstrate the BB84 protocol over deployed fiber between the University of Calgary and SAIT. The system implemented a novel tool called quantum frames that allow for the quantum signals to be routed, for clock synchronization, and for channel stabilization in a network scenario. The same system was used to examine the scalability of the secret key generation rate in different steps of the process in order to detect potential bottlenecks for key generation rate of high speed systems. A second QKD system was developed to demonstrate the measurement-device independent QKD protocol. The system worked over deployed fiber between the University of Calgary, SAIT, and Foothills Hospital in the City of Calgary. The advantage of the measurement-device independent QKD protocol over previous QKD protocols is that it eliminates the possibility of side-channel attacks that target single photon detectors used in QKD systems. This demonstration also involved the first demonstration of a Bell state measurement over deployed fiber. Bell state measurements were further studied by using novel single photon detectors, which allowed demonstrating a highly efficient Bell measurement. Finally, a cryptographic protocol known as private queries was demonstrated between the University of Calgary and SAIT. Quantum private queries were demonstrated for the first time over deployed fiber by developing and implementing an error correction scheme to make the protocol noise and loss tolerant.
"Quantum communication is the art of transferring a quantum state from one place to another". The capability of distributing quantum states allows, for instance, provably secure communication and, in the near future, will enable the interconnection of quantum computers to establish a quantum internet. A convenient way to send quantum states from one place to another is to encode them into photons and distribute them using optical bres. The distance over which this can be achieved is still limited to a few hundred of kilometers. However, it can be extended in principle to arbitrary long distances by means of quantum repeaters. The realization of such quantum repeaters will require the engineering and interfacing of heterogeneous elements such as entangled photon-pair sources, quantum memories and entanglement swapping operations. The main goal of this thesis is to develop and study the compatibility of the main elements required to build a frequency multiplexed quantum repeater. This architecture requires a frequency multimode entangled photon pair source which, for example, could be implemented exploiting the process that involves the interaction of a strong light pulse with a non-linear crystal. Such a process is versatile and allows easy tailoring of the photon-pair spectral properties in order to match the requirements of the frequency multiplexed quantum repeater architecture. First, as a precursor of such a photon pair source, we developed a novel heralded single photon source that involves spectrally resolved single photon detection and on-demand frequency shifting. These capabilities are also essential tools in a frequency multiplexed quantum repeater. Next, we demonstrated the compatibility of such a sources with frequency multimode photonic quantum memories by performing spectrally multiplexed storage of single photons. We also tested the capability of high- delity storage of photons encoding quantum information in their polarization degree of freedom. Finally, we showed that entanglement swapping operations, i.e. Bell-state measurements, can be performed using photon pair sources compatible with quantum memories, quantum repeater architectures, and real-world scenarios. While a lot of e ort remains to be done, in the work presented in this thesis we demonstrated that all the key elements required to build a frequency multiplexed quantum repeater can be built and eventually be interfaced. The main obstacles towards that goal and possible ways to overcome them are also discussed.
Quantum theory admits correlations between distant parties that are stronger than those permitted by classical physics. Such correlations, which are termed nonlocal, have been studied extensively since their discovery by John Bell in 1964. This thesis makes progress on various aspects of quantum nonlocality both from a foundational and practical perspective. We begin by studying a foundational question on the relationship between nonlocality and quantum entanglement. We show that the strongest form of nonlocality, also called pseudo-telepathy or full nonlocality, can be demonstrated by non-maximally entangled states and prove that all pure entangled states can demonstrate full nonlocality in the many-copy scenario. We also provide non-trivial examples of fully nonlocal mixed states. We then turn to the study of another phenomenon in quantum theory which is essential in almost all demonstrations of non-classicality—measurement incompatibility. We generalise the notion of measurement incompatibility and show that our notion has strong operational relevance: it captures the randomness in the outcomes of an untrusted measurement device against a classical adversary. We use our formalism to derive new bounds on the experimental losses and noise that can be tolerated in quantum communication protocols before they become insecure. We then begin a systematic study of routed Bell experiments, a variant of standard Bell experiments that was introduced to demonstrate nonlocality over long distances in the presence of losses and noise. We formalize the notion of genuine long-range quantum correlations in routed Bell experiments and develop numerical and analytical tools to characterize them. We show that routed Bell experiments allow for the demonstration of long-range quantum correlations at arbitrarily large distances using only entangled qubit states. We then prove the security of fully device-independent (DI) quantum key distribution (QKD) protocols based on routed Bell tests and quantify the resulting improvement in key rate and distance compared to standard DI QKD protocols.