The capability of controlling light at scales that are much smaller than the operating wave-length enables new optical functionalities, and opens up a wide range of applications. Such a capability is out of the realm of conventional optical approaches. This dissertation aims to explore the light-matter interactions at nanometer scale, and to investigate the novel scien-tific and industrial applications. In particular, we will explain how to detect nanoparticles using an ultra-sensitive nano-sensor; we will also describe a photonic diode which gener-ates a unidirectional flow of single photons; Moreover, in an one-dimensional waveguide QED system where the fermionic degree of freedom is present, we will show that strong photon-photon interactions can be generated through scattering means, leading to photonic bunching and anti-bunching with various applications. Finally, we will introduce a mecha-nism to achieve super-resolution to discern fine features that are orders of magnitude smaller than the illuminating wavelength. These research projects incorporate recent advances in quantum nanophotonics, nanotechnologies, imaging reconstruction techniques, and rigorous numerical simulations.
The capability of controlling light at scales that are much smaller than the operating wave-length enables new optical functionalities, and opens up a wide range of applications. Such a capability is out of the realm of conventional optical approaches. This dissertation aims to explore the light-matter interactions at nanometer scale, and to investigate the novel scien-tific and industrial applications. In particular, we will explain how to detect nanoparticles using an ultra-sensitive nano-sensor; we will also describe a photonic diode which gener-ates a unidirectional flow of single photons; Moreover, in an one-dimensional waveguide QED system where the fermionic degree of freedom is present, we will show that strong photon-photon interactions can be generated through scattering means, leading to photonic bunching and anti-bunching with various applications. Finally, we will introduce a mecha-nism to achieve super-resolution to discern fine features that are orders of magnitude smaller than the illuminating wavelength. These research projects incorporate recent advances in quantum nanophotonics, nanotechnologies, imaging reconstruction techniques, and rigorous numerical simulations.
Abstract Over the last few decades, the quantum aspects of light have been explored and major progress has been made in understanding the specific quantum aspects of the interaction between light and matter. Single photons are now routinely produced by single molecules on surfaces, vacancies in crystals, and quantum dots. The micrometre and nanometre scale is also the privileged range where fluctuations of electromagnetic fields manifest themselves through the Casimir force. The domain of classical optics has recently seen many exciting new developments, especially in the areas of nano-optics, nano-antennas, metamaterials, and optical cloaking. Approaches based on single-molecule detection and plasmonics have provided new avenues for exploring light–matter interaction at the nanometre scale. All these topics have in common a trend to consider and use smaller and smaller objects, down to the micrometre, nanometre, and even atomic range, a region where one gradually passes from classical physics to quantum physics. The summer school held in Les Houches in July 2013 treated all these subjects lying at the frontier between nanophotonics and quantum optics, in a series of lectures given by world experts in the domain and gathered together in the present volume.
The field of quantum nanophotonics has recently been attracting a great deal of interest. In quantum nanophotonics, fermionic degrees of freedom such as atoms or quantum dots are coupled to traditional nanophotonic systems. As the fermionic components can only absorb a finite number of photons at a time, the interplay between the fermionic and photonic degrees of freedom can fundamentally alter the transport properties of photons and their correlations. In many conventional photonic systems, however, atom-photon interactions are too weak to realize efficient devices at ultra-low power levels. We show that in properly designed quantum nanophotonic geometries, we can create strong photon-photon interaction and quantum interference to realize efficient devices operating down to the single-photon power level. In particular, quantum nanophotonic geometry allows us to establish quantum interference to provide efficient single-photon frequency conversion and long-term photonic storage. Moreover, we use strong photon-photon interactions in cavity-QED to produce strongly antibunched streams of photons with shot noise below the classical limit which can allow fundamentally secret communication over large distances.
This thesis encompasses a broad area of physics including linear and nonlinear optics, photonics and quantum physics. It combines the phenomena of nonlinearoptical frequency conversion with waveguiding and coupling, taking advantage of new opportunities presented by advances in fabrication technologies of micro- and nano-waveguides. In this dissertation an in-depth analysis of quantum and classical properties of light traveling in nonlinear optical waveguides, directional couplers and waveguide arrays is performed. The concepts of spatial and temporal dispersion, waveguiding in structures with subwavelength dimensions and nonlinear interactions between different frequencies of light are studied both theoretically and experimentally. Some sections of this thesis include development and implementation of novel physical ideas, while other sections are focused on comprehensive experimental and numerical analysis of advanced theoretical concepts. The results presented in this dissertation demonstrate new physical phenomena with potential applications in the areas of telecommunications and quantum information. The research performed in this thesis opens opportunities for frequency conversion with world-leading power efficiency, including operation with ultrashort pulses for a variety of wavelengths to suit a wide range of perspective application requirements. It also shows an approach for simple and energy efficient spatio-temporal optical signal control, which can find applications in next generation telecommunications networks. Furthermore, the results obtained in this dissertation demonstrate the possibility for flexible shaping of quantum statistics of photons generated in photonic waveguiding structures through spontaneous frequency conversion, contributing to the development of integrated quantum circuits. The new methods of frequency conversion in micro- and nano-scale waveguides and optical circuits have potential to advance the performance, energy efficiency, and security of future optical communication networks and computing systems.
Waveguide quantum electrodynamics (waveguide QED) describes the interaction between an electromagnetic field confined to a one-dimensional waveguide with atom-like quantum emitters close by. The characteristics of these kinds of systems are the possibility for strong and even ultrastrong interactions between the photonic and atom-like systems, and practically infinite range interactions between the emitters. These properties are valuable for a wide range of quantum optical applications, like quantum communication, quantum networks and quantum metrology. In this thesis we focus on two challenges in quantum optics, namely the generation and scattering of multiphoton states. In the first part of this thesis we demonstrate how waveguide QED systems can be exploited for the generation of multiphoton states, in particular of single-mode Fock states and superpositions thereof as well as multi-mode photonic states with metrological applications. The basic setup for this goal is an ensemble of quantum emitters coupled to a waveguide. In the so-called atomic mirror configuration symmetric Dicke states (or a superposition thereof) decay superradiantly to the ground state and emit the desired multiphoton state, which can be efficiently collected at the ends of the waveguide. We propose various protocols for the preparation of these Dicke states in waveguide QED systems and characterize the emitted photonic state. It turns out that in the low excitation regime, that is, if the number of photons is much lower than the ensemble size, the photonic state is emitted into a single mode. This single-mode structure is fundamental to current proposals for applications in quantum metrology with optical interferometers. Outside the low excitation regime, a multi-mode photonic state is generated, for which the metrological capabilities were unknown. We were able to show that these states still lead to quantum-enhanced optical interferometry. In the second part of this thesis we demonstrate how the scattering of multiphoton states on a single quantum emitter coupled to the waveguide can be used for testing the limits of the light-matter interaction strength. In particular, we investigate systems in the so-called ultrastrong coupling regime, where the coupling strength between the photonic and atom-like system is of the order of the emitter's transition energy. In this regime, many methods and approximations used in quantum optics, especially the Rotating Wave Approximation, break down and one needs to develop new analytical and numerical methods to study these systems. One approach is the so-called polaron Transformation. We show how this transformation can be applied for predicting the scattering amplitude of few photons scattering on the emitter. The comparison of these results with numerical simulations using matrix product states shows a good agreement for moderate coupling strengths. Both parts together show that waveguide QED systems are promising candidates for the generation of multiphoton states as well as for the investigation of fundamental limits probed through the scattering of multiphoton states. The latter also finds application in the implementation of photon-photon nonlinearities induced by the interaction with the quantum emitters. Apart from these and many other theoretical predictions, waveguide QED systems are also undergoing rapid progress in experiments. Therefore, we expect these kinds of systems to bring forth several advances in the field of quantum optics.
Abstract Complete control of light-matter interactions at a single quantum level is critical for quantum science applications such as precision measurement and information processing. Nanophotonic devices, developed with recent advancements in nanofabrication techniques, can be used to tailor the interactions between single photons and atoms. One example of such a nanophotonic device is the optical nanofibre, which provides an excellent platform due to the strongly confined transverse light fields, long interaction length, low loss, and diverse optical modes. This facilitates a strong interaction between atoms and guided light, revealing chiral atom-light processes and the prospect of waveguide quantum electrodynamics. This paper highlights recent advances, experimental techniques, and future perspectives of the optical nanofibre-atom hybrid quantum platform.
The aim of this thesis is to explore nonlinear nanostructures – photonic systems with one or more dimension with nanoscale feature size – as new platforms for parametric photon-pair generation. This is motivated by the need for photon-pair sources in many technological applications of quantum optics, such as quantum communication, imaging and computing. The initial hypothesis is that nonlinear nanostructures are a promising platform to complement established photon-pair source schemes based on bulk crystals or photonic integrated circuits in terms of quantum state-engineering, footprint, functional density etc. However, nonlinear pair generation, e.g. via spontaneous parametric down-conversion (SPDC), is a new subfield in nanophotonics with a very limited number of studies existing. This constitutes the knowledge-gap addressed in this thesis. Therefore, the objective is to provide first experimental demonstrations of SPDC in subwavelength-scale and nonlinear nanostructures. We investigate the ability of such systems to control the properties of two-photon quantum states such as frequency and angular spectrum or polarization entanglement. To this end we analyze nanostructures with different degrees of complexity, starting with an unstructured thin crystal with one nanoscale dimension, leading up to a 3D nano-scale resonator with subwavelength-sized features in all dimensions. Furthermore, we test different types of nonlinear materials such as lithium niobate, group III-V semiconductors and emerging, highly nonlinear materials such as molybdenum disulfide. Additionally, we also advance the theoretical understanding by developing a comprehensive model of the quantum process of nonlinear parametric pair-generation in photonic nanostructures.