Detection of Exchange Interaction Through Fano-Like Interference Effects

Jonas Fransson, Alexander V. Balatsky

Zoe Scott, Shafi Muhammad, Tigran V. Shahbazyan

We present an analytical model describing the transition to a strong coupling regime for an ensemble of emitters resonantly coupled to a localized surface plasmon in a metal-dielectric structure. The response of a hybrid system to an external field is determined by two distinct mechanisms involving collective states of emitters interacting with the plasmon mode. The first mechanism is the near-field coupling between the bright collective state and the plasmon mode, which underpins the energy exchange between the system components and gives rise to exciton-induced transparency minimum in scattering spectra in the weak coupling regime and to emergence of polaritonic bands as the system transitions to the strong coupling regime. The second mechanism is the Fano interference between the plasmon dipole moment and the plasmon-induced dipole moment of the bright collective state as the hybrid system interacts with the radiation field. The latter mechanism is greatly facilitated by plasmon-induced coherence in a system with the characteristic size below the diffraction limit as the individual emitters comprising the collective state are driven by the same alternating plasmon near field and, therefore, all oscillate in phase. This cooperative effect leads to scaling of the Fano asymmetry parameter and of the Fano function amplitude with the ensemble size, and therefore, it strongly affects the shape of scattering spectra for large ensembles. Specifically, with increasing emitter numbers, the Fano interference leads to a spectral weight shift toward the lower energy polaritonic band.

W. Baltensperger

Joachim Keßler, J. Lorenz

K. L. Litvinenko, Nguyen H. Le, Britta Redlich +5 more

The ordinary Fano effect occurs in many-electron atoms and requires an autoionizing state. With such a state, photo-ionization may proceed via pathways that interfere, and the characteristic asymmetric resonance structures appear in the continuum. Here we demonstrate that Fano structure may also be induced without need of auto-ionization, by dressing the continuum with an ordinary bound state in any atom by a coupling laser. Using multi-photon processes gives complete, ultra-fast control over the interference. We show that a line-shape index q near unity (maximum asymmetry) may be produced in hydrogenic silicon donors with a relatively weak beam. Since the Fano lineshape has both constructive and destructive interference, the laser control opens the possibility of state-selective detection with enhancement on one side of resonance and invisibility on the other. We discuss a variety of atomic and molecular spectroscopies, and in the case of silicon donors we provide a calculation for a qubit readout application.

Wei Yan, Junle Qu, Hongsheng Niu

We perform a time-dependent analysis of the formation and stable propagation of an ultraslow optical soliton pair, and four-wave mixing (FWM) via tunable Fano interference in double-cascade type semiconductor multiple quantum wells (SMQWs). By using the probability amplitude method to describe the interaction of the system, we demonstrate that the electromagnetically induced transparency (EIT) can be controlled by Fano interference in the linear case and the strength of Fano interference has an important effect on the group velocity and amplitude of the soliton pair in the nonlinear case. Then, when the signal field is removed, the dynamic FWM process is analyzed in detail, and we find that the strength of Fano interference also has an important effect on the FWM's efficiency: the maximum FWM efficiency is ~28% in appropriate conditions. The investigations are promising for practical applications in optical devices and optical information processing for solid systems.