Two-photon emission

R. Stephen Berry

Jitendra K. Verma, Harmanpreet Singh, Pradyumna K. Pathak

We predict dominating cooperative two-photon emission from two quantum dots coupled with a single-mode photonic crystal cavity. The cooperative two-photon emission occurs when excitons in two off-resonantly coupled quantum dots decay simultaneously. The interaction with a common cavity field leads to cavity-induced two-photon emission which is strongly inhibited by electron-phonon coupling. The interaction with a common phonon bath produces phonon-induced two-photon emission which increases on increasing temperature. For identical quantum dots, cavity-induced two-photon emission is negligible, but phonon-induced two-photon emission could be large.

S. N. Biswas, S. N. Haque, Man Mohan

Two-Raman-photon emission in hydrogen atoms in the presence of an intense electromagnetic field has been calculated utilizing the method of Dalgarno and Lewis. We give a general formulation for ($n\ensuremath{-}2$)-photon absorption and two-photon emission and also give numerical results for two-photon emission in the $1s\ensuremath{-}2p$ transition in hydrogen atoms. It is found that the emission of two spontaneous Raman photons could become important when the energy of the intense photon approaches the ionization energy. Finally, in the spectrum of the emitted Raman photon, faint lines are expected corresponding to the resonant peaks in the cross section.

Stephen V. Kershaw

Shunfa Liu, Yangpeng Wang, Yasser Saleem +12 more

Abstract Spontaneous two-photon emission is a process in which the transition between two quantum states happens via simultaneous emissions of two identical photons. Such second-order quantum radiation is of paramount importance in astrophysics, atomic physics, and quantum technology. In particular, on-demand spontaneous two-photon emission from single quantum emitters has long been envisioned to revolutionize photonic quantum science and technology. To date, experimental realizations of two-photon emission at the single quanta level are still highly challenging yet elusive due to their low probabilities. In this work, we explore spontaneous two-photon emission from a single semiconductor quantum dot deterministically coupled to a high-quality microcavity in which the cavity resonances greatly enhance both excitation and emission processes. When the cavity is resonant to the half energy of the biexciton, the strong vacuum field in the cavity mode drives the biexciton to the ground state and simultaneously emits two photons into the cavity mode, resulting in two-photon emissions with a record brightness comparable to the competing single-photon process and sub-nanowatt power consumption. For the first time, the quantum nature associated with spontaneous two-photon emissions in the cavity quantum electrodynamics regime has been investigated via photon statistics measurements. Furthermore, spontaneous two-photon emission is exploited to build unconventional entangled quantum light sources with the unique advantage of combining the best of two worlds: near-unity entanglement fidelity for spontaneous parametric down-conversion source and on-demand photon emissions for atomic quantum emitters. Our work provides unprecedented insights into the two-photon process in the quantum regime and opens an unexplored avenue for pursuing optically reconfigurable quantum light sources with nonlinear quantum radiations.