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Springer series in chemical physics

Spontaneous Emission and Ultrafast Dephasing in Front of a Mirror

Karel E. Drabe, Gerard Cnossen, D. A. Wiersma

Published Jan 1, 1990• 0 citations
Publisher
DOI
10.1007/978-3-642-84269-6_41

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Spontaneous Emission and Ultrafast Dephasing in front of a Mirror.

Karel E. Drabe, Gerard Cnossen, Douwe A. Wiersma

We report a new technique to probe femtosecond dephasing processes in solids, requiring only low excitation intensities. The method is based on the measurement of the spontaneous emission spectrum of a thin sample (about 2µm) in front of a mirror, excited by 40 fs pulses from a colliding pulse modelocked (CPM) laser. Fig. 1A shows the simplified level scheme of a prototype molecule, and fig.1B gives the schematics of the experimental arrangement.

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