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Chinese Optics Letters

Temporal self-modifying characteristics of pulse propagation in multiphoton absorbers

Kun Cheng Kun Cheng, Sujuan Zhang Sujuan Zhang, Wei Li, Wanjun Dai, Dongxia Hu, Feng Jing

Published Jan 1, 2015• 0 citations
Publisher

Abstract

In this Letter, temporal self-modifying behavior of amplitude modulation pulse propagation characteristics in multiphoton absorbers is presented by solving the underlying theoretical model coupling the propagation equation with the rate equations. The characteristics of the output temporal shapes are of primary concern and are discussed in detail. Amplitude modulation suppressing effects of multiphoton absorbers are numerically demonstrated; they have not been reported previously, to our knowledge. By taking a time resolved absorption coefficients, the corresponding physical mechanism is explicitly interpreted.

DOI
10.3788/col201513.070009

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In this Letter, temporal self-modifying behavior of amplitude modulation pulse propagation characteristics in multiphoton absorbers is presented by solving the underlying theoretical model coupling the propagation equation with the rate equations. The characteristics of the output temporal shapes are of primary concern and are discussed in detail. Amplitude modulation suppressing effects of multiphoton absorbers are numerically demonstrated; they have not been reported previously, to our knowledge. By taking a time resolved absorption coefficients, the corresponding physical mechanism is explicitly interpreted.
We develop an analytical approach to the dynamics of band populations of reverse saturable absorbers modeled by the three-level approximation of the five-level rate equations. We find high-accuracy approximate solutions to these rate equations, taking into account the temporal shape of the incident laser pulse for different regimes of excitation. The results obtained are confirmed by direct numerical integration of the rate equations and are verified by solution of the full system of the rate and the propagation equations. The validity ranges of the approximations are determined. We also prove that for input pulses that are much longer than the lifetime of the first excited state the ground-state depletion obeys the same functional dependence on the input fluence as in the case of rectangular input pulses. The dynamics of the excited states, however, explicitly depends on the pulse shape. We quantitatively estimate the effect of various parameters on the nonlinear absorption coefficient and discuss implementation of the approach by a beam propagation method to reduce the computational time.
Nonlinear effects in pulse propagation through a medium consisting of four-level double-$\ensuremath{\Lambda}$-type systems are studied theoretically. We apply three continuous-wave driving fields and a pulsed probe field such that they form a closed interaction loop. Due to the closed loop and the finite frequency width of the probe pulses, the multiphoton resonance condition cannot be fulfilled, such that a time-dependent analysis is required. By identifying the different underlying physical processes we determine the parts of the solution relevant to calculate the linear and nonlinear response of the system. We find that the system can exhibit a strong intensity-dependent refractive index with small absorption over a range of several natural linewidths. For a realistic example we include Doppler and pressure broadening and calculate the nonlinear self-phase modulation in a gas cell with sodium vapor and argon buffer gas. We find that a self-phase modulation of $\ensuremath{\pi}$ is achieved after the propagation of a few centimeters through the medium while the absorption and pulse shape distortion in the corresponding spectral range is small.
On-resonance self-action of a beam with periodically modulated amplitude in a two-level saturable absorber is studied numerically. When the period of modulation is comparable with relaxation times, one cannot describe the medium by means of susceptibility, and the response of the medium to the amplitude variation is not immediate. We solve the Bloch equations in each point of the medium to find this response correctly. Transient behavior followed by stable oscillations of population difference and polarization vector is shown to depend strongly on the frequency and amplitude of modulation. Beam propagation is considered using a simplified model of a thin absorber followed by free space, the propagation distance being small compared with the modulation wavelength. Manifestations of non-stationary response of the medium in the output intensity behavior are analyzed.
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Reverse-saturable absorbers are of considerable interest for optical limiting. Using the electric dipole perturbation, we derived the rate equation for a five-level system describing reverse-saturable absorbers. Traditional theories for the propagating laser beam in these materials are expressed in terms of the optical intensity. However, with the introduction of high-power short-pulsed lasers, the propagation of light in these materials may be subject to nonlinear phenomena such as self-focusing and self-phase modulation. Furthermore, conventional theories treat the laser light as a continuous wave or as a very broad temporal pulse in which dispersive effects are neglected. In order to incorporate these other nonlinear or dispersive effects, and therefore determine their influence in reverse-saturable absorbers, we derived an equation for the propagation of the electromagnetic field, rather than the intensity, coupled to the rate equations for a five-level system. We also coupled our theory to experimentally measurable parameters for these materials and detailed the various physical approximations used to obtain the rate equations.
Numerical modeling of self-action of a beam, whose amplitude is periodically modulated in time, in a two-level saturable absorbing medium is reported. For describe a beam self-action we solve numerically the full set of Maxwell-Bloch equations. We study the influence of the non-stationary self-action of the beam on the transmission of modulation signal through the medium. It is shown that in the time dependence of the polarization and population difference the nonlinear distortions of the modulation signal can be much stronger than in the output field intensity.