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Acta Physica Polonica A

Phonon-Induced Pure Dephasing of Two-Electron Spin States in Vertical Quantum Dot Molecules

Katarzyna Roszak, Paweł Machnikowski

Published Nov 1, 2009• 1 citation
Publisher

Abstract

Phonon-induced dephasing of two-electron spin states in two vertically stacked self-assembled GaAs/InGaAs quantum dots is studied.A pure dephasing process due to elastic phonon scattering is found to dominate at low temperatures.This process is independent of the spin-orbit coupling and does not require the presence of a magnetic field.It relies on interdot tunneling and the Pauli principle, which make the double quantum dot gate for spin based quantum computing possible, and therefore cannot be avoided.

DOI
10.12693/aphyspola.116.877

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Phonon-induced dephasing of two-electron spin states in two vertically stacked self-assembled GaAs/InGaAs quantum dots is studied.A pure dephasing process due to elastic phonon scattering is found to dominate at low temperatures.This process is independent of the spin-orbit coupling and does not require the presence of a magnetic field.It relies on interdot tunneling and the Pauli principle, which make the double quantum dot gate for spin based quantum computing possible, and therefore cannot be avoided.
We show that singlet-triplet superpositions of two-electron spin states in a double quantum dot undergo a phonon-induced pure dephasing which relies only on the tunnel coupling between the dots and on the Pauli-exclusion principle. As such, this dephasing process is independent of spin-orbit coupling or hyperfine interactions. The physical mechanism behind the dephasing is elastic phonon scattering, which persists to much lower temperatures than real phonon-induced transitions. Quantitative calculations performed for a lateral GaAs/AlGaAs gate-defined double quantum dot yield microsecond dephasing times at sub-Kelvin temperatures, which is consistent with experimental observations.
Phonon-assisted tunneling of electrons between nonidentical quantum dots in a magnetic field has been recently shown to be affected by a spin pure dephasing.The process is due to the mismatch of the Zeeman splittings caused by the difference of effective electron g-factors in the two dots.Based on both analytical estimation and an accurate numerical modeling of a double quantum dot system, we show that this dephasing can be canceled by applying an appropriately tuned magnetic-field gradient that compensates for the built-in inequality of the Zeeman splittings.
We study theoretically the phonon-induced relaxation (T1{T}_{1}T1​) and decoherence times (T2{T}_{2}T2​) of singlet-triplet qubits in lateral GaAs double quantum dots (DQDs). When the DQD is biased, Pauli exclusion enables strong dephasing via two-phonon processes. This mechanism requires neither hyperfine nor spin-orbit interaction and yields ${T}_{2}\ensuremath{\ll}{T}_{1}$, in contrast to previous calculations of phonon-limited lifetimes. When the DQD is unbiased, we find ${T}_{2}\ensuremath{\simeq}2{T}_{1}$ and much longer lifetimes than in the biased DQD. For typical setups, the decoherence and relaxation rates due to one-phonon processes are proportional to the temperature TTT, whereas the rates due to two-phonon processes reveal a transition from T2{T}^{2}T2 to higher powers as TTT is decreased. Remarkably, both T1{T}_{1}T1​ and T2{T}_{2}T2​ exhibit a maximum when the external magnetic field is applied along a certain axis within the plane of the two-dimensional electron gas. We compare our results with recent experiments and analyze the dependence of T1{T}_{1}T1​ and T2{T}_{2}T2​ on system properties such as the detuning, the spin-orbit parameters, the hyperfine coupling, and the orientation of the DQD and the applied magnetic field with respect to the main crystallographic axes.
We have theoretically studied phonon-mediated spin-flip processes of electrons in a GaAs double quantum dot (DQD) holding two spins, under a phonon temperature gradient over the DQD. Transition rates of interdot phonon-assisted tunnel processes and intradot spin-flip processes involving spin triplet states are formalized by the electron-phonon interaction accompanied with the spin-orbit interaction. The calculations of the spin-flip rates and the occupation probabilities of the spin-states in the two-electron DQD with respect to the phonon temperature difference between the dots are quantitatively consistent with our previous experiment. This theoretical study on the temperature gradient effect onto spins in coupled QDs would be essential for understanding spin-related thermodynamic physics.
We study electron-phonon interaction induced decoherence between two-electron singlet and triplet states in a semiconductor double quantum dot using a spin-boson model. We investigate the onset and time evolution of this dephasing, and study its dependence on quantum dot parameters such as dot size and double dot separations, as well as the host materials (GaAs and Si). At the short time limit, electron-phonon interaction only causes an incomplete initial Gaussian decay of the off-diagonal density matrix element in the singlet-triplet Hilbert space; a complete long-time exponential decay due to phonon relaxation would eventually dominate over two-spin decoherence. We analyze two-spin decoherence in both symmetric and biased double quantum dots, identifying their difference in electron-phonon coupling and the relevant consequences.
We predict a spin pure dephasing channel in electron relaxation between states with unequal Zeeman splittings, exemplified by a spin-preserving electron tunneling between quantum dots in a magnetic field. The dephasing is caused by a mismatch in electron ggg factors in the dots leading to distinguishability of phonons emitted during tunneling with opposite spins. Combining multiband $\mathbit{k}\ifmmode\cdot\else\textperiodcentered\fi{}\mathbit{p}$ modeling and dynamical simulations via a master equation, we show that this fundamental effect of spin measurement effected by the phonon bath may be widely controlled by the size and composition of the dots or on demand via tuning of external fields. By comparing the numerically simulated degree of dephasing with the predictions of general theory based on distinguishability of environment states, we show that the proposed mechanism is the dominant phonon-related spin dephasing channel and may limit spin coherence time in tunnel-coupled structures at cryogenic temperatures.