Femtosecond hole burning storage by two-photon absorption
Alex Karotki, Mikhail A. Drobizhev, Alexander Rebane
Summary form only given. Spectral hole burning (SHB) is a promising technique for optical recording of information with a potential to store in excess of 10/sup 4/-10/sup 5/ bits per /spl lambda//sup 3/ volume (Moerner, 1988). Highest storage capacity is achieved when frequency- or time-domain addressing is combined with addressing in three spatial dimensions by using a bulk SHB medium. However, so far both bit-by-bit and holographic SHB storage experiments were restricted to two spatial dimensions. This is because focusing a laser beam to a small volume inside the SHB medium is hindered by one-photon absorption in SHB material layers. We propose that this problem may be overcome by burning holes via two-photon absorption (TPA) (Demtro/spl uml/der, 1982; Takeda et al, 2000). TPA has been used earlier for conventional spectrally nonselective recording in photo-chromic materials by focusing two perpendicularly directed laser beams (with photon energies /spl planck//spl omega//sub 1/ and /spl planck//spl omega//sub 2/) on to one spot (Parthenopoulos and Rentzepis, Science, vol. 245, pp. 843-845, 1989). Since the sample is transparent for each beam separately, TPA occurs only at the beam intersection point. In this paper, we investigate frequency-selective SHB by TPA in organic dye-doped polymers at low temperature. In our experiments, the SHB medium is essentially transparent for the writing beams, which allows unrestricted penetration and focusing in the depth of the sample.
Conference on Lasers and Electro-Optics•Jan 1, 2001•1 citation