This thesis is concerned with the collective dynamics in different spin chains and spin ensembles in solid-state materials. The focus is on the manipulation of electron spins, through spin-spin and spin-photon couplings controlled by voltage potentials or electromagnetic fields. A brief review of various systems is provided to describe the possible physical implementation of the ideas, and also outlines the basis of the adopted effective interaction models. The first two ideas presented explore the collective behaviour of non-interacting spin chains with external couplings. One focuses on mapping the identical state of spin-singlet pairs in two currents onto two distant, static spins downstream, creating distributed entanglement that may be accessed. The other studies a quantum memory consisting of an array of non-interacting, static spins, which may encode and decode multiple flying spins. Both chains could effectively 'enhance' weak couplings in a cumulative fashion, and neither scheme requires active quantum control. Moreover, the distributed entanglement generated can offer larger separation between the qubits than more conventional protocols that only exploit the tunnelling effects between quantum dots. The quantum memory can also 'smooth' the statistical fluctuations in the effects of local errors when the stored information is spread. Next, an interacting chain of static spins with nearest-neighbour interactions is introduced to connect distant end spins. Previously, it has been shown that this approach provides a cubic speed-up when compared with the direct coupling between the target spins. The practicality of this scheme is investigated by analysing realistic error effects via numerical simulations, and from that perspective relaxation of the nearest-neighbour assumption is proposed. Finally, a non-interacting electron spin ensemble is reviewed as a quantum memory to store single photons from an on-chip stripline cavity. It is then promoted to a full quantum processor, with major error effects analysed.
This thesis is concerned with the collective dynamics in different spin chains and spin ensembles in solid-state materials. The focus is on the manipulation of electron spins, through spin-spin and spin-photon couplings controlled by voltage potentials or electromagnetic fields. A brief review of various systems is provided to describe the possible physical implementation of the ideas, and also outlines the basis of the adopted effective interaction models. The first two ideas presented explore the collective behaviour of non-interacting spin chains with external couplings. One focuses on mapping the identical state of spin-singlet pairs in two currents onto two distant, static spins downstream, creating distributed entanglement that may be accessed. The other studies a quantum memory consisting of an array of non-interacting, static spins, which may encode and decode multiple flying spins. Both chains could effectively 'enhance' weak couplings in a cumulative fashion, and neither scheme requires active quantum control. Moreover, the distributed entanglement generated can offer larger separation between the qubits than more conventional protocols that only exploit the tunnelling effects between quantum dots. The quantum memory can also 'smooth' the statistical fluctuations in the effects of local errors when the stored information is spread. Next, an interacting chain of static spins with nearest-neighbour interactions is introduced to connect distant end spins. Previously, it has been shown that this approach provides a cubic speed-up when compared with the direct coupling between the target spins. The practicality of this scheme is investigated by analysing realistic error effects via numerical simulations, and from that perspective relaxation of the nearest-neighbour assumption is proposed. Finally, a non-interacting electron spin ensemble is reviewed as a quantum memory to store single photons from an on-chip stripline cavity. It is then promoted to a full quantum processor, with major error effects analysed.
Electron spins confined in quantum dots (QDs) are among the leading contenders for implementing quantum information processing. In this Thesis we address two of the most significant technological challenges towards developing a scalable quantum information processor based on spins in quantum dots: (i) decoherence of the electronic spin qubit due to the surrounding nuclear spin bath, and (ii) long-range spin-spin coupling between remote qubits. To this end, we develop novel strategies that turn the unavoidable coupling to the solid-state environment (in particular, nuclear spins and phonons) into a valuable asset rather than a liability. In the first part of this Thesis, we investigate electron transport through single and double QDs, with the aim of harnessing the (dissipative) coupling to the electronic degrees of freedom for the creation of coherence in both the transient and steady-state behaviour of the ambient nuclear spins. First, we theoretically show that intriguing features of coherent many-body physics can be observed in electron transport through a single QD. To this end, we first develop a master-equation-based formalism for electron transport in the Coulomb-blockade regime assisted by hyperfine (HF) interaction with the nuclear spin ensemble in the QD. This general tool is then used to study the leakage current through a single QD in a transport setting. When starting from an initially uncorrelated, highly polarized state, the nuclear system experiences a strong correlation buildup, due to the collective nature of the coupling to the central electron spin. We demonstrate that this results in a sudden intensity burst in the electronic tunneling current emitted from the QD system, which exceeds the maximal current of a corresponding classical system by several orders of magnitude. This gives rise to the new paradigm of electronic superradiance. Second, building upon the insight that the nuclear spin dynamics are governed by collective interactions giving rise to coherent effects such as superradiance, we propose a scheme for the deterministic generation of steady-state entanglement between the two nuclear spin ensembles in an electrically defined double quantum dot. Because of quantum interference in the collective coupling to the electronic degrees of freedom, the nuclear system is actively driven into a two-mode squeezedlike target state. The entanglement buildup is accompanied by a self-polarization of the nuclear spins towards large Overhauser field gradients. Moreover, the feedback between the electronic and nuclear dynamics is shown to lead to intriguing effects such as multistability and criticality in the steady-state solutions. In the second part of this Thesis, our focus turns towards the realization of long-range spin-spin coupling between remote qubits. We propose a universal, on-chip quantum transducer based on surface acoustic waves in piezo-active materials. Because of the intrinsic piezoelectric (and/or magnetostrictive) properties of the material, our approach provides a universal platform capable of coherently linking a broad array of qubits, including quantum dots, trapped ions, nitrogen-vacancy centers or superconducting qubits. The quantized modes of surface acoustic waves lie in the gigahertz range, can be strongly confined close to the surface in phononic cavities and guided in acoustic waveguides. We show that this type of surface acoustic excitations can be utilized efficiently as a quantum bus, serving as an on-chip, mechanical cavity-QED equivalent of microwave photons and enabling long-range coupling of a wide range of qubits. In summary, this thesis provides contributions towards developing a scalable quantum information processor based on spins in quantum dots in two different aspects. The first part is dedicated to a deeper understanding of the nuclear spin dynamics in quantum dots. In the second part we put forward a novel sound-based strategy to realize long-range spin-spin coupling between remote qubits. This completes a broad picture of spin-based quantum information processing which integrates different perspectives, ranging from the single-qubit level to a broader quantum network level.
This thesis discusses various schemes and protocols for quantum information processing in mesoscopic systems with particular focus on using the spin of a particle as the bearer of information. The first chapter introduce various aspects of the field of quantum information used in this thesis such as qubits, entanglement, its quantification, quantum logic gates and entanglement swapping. In this chapter concepts such as AKLT states, decoherence and adiabatic elimination are introduced as they will be relevant in the thesis. In chapter 2 we introduce the Quantum Dots as the solid state system that will primarily be used as the hardware for the development of Quantum Information Processing (QIP). The different properties of quantum dots depending on their size are discussed. The exchange interaction between tunnel coupled quantum dots and the background of quantum computation in quantum dots is described. The principal sources of decoherence and the measurement techniques for spin qubits are presented. In chapter 3, carbon nanowires filled with N@C60 dimers are studied to analyse the entanglement between nuclear spins. The dimer is modelled as a two coupled nuclear spin- electron spin pair with a Heisenberg interaction. The entanglement have been studied depending on the temperature and the intensity of an external magnetic field. Witnessing the entanglement, and particularly bound entanglement are discussed. In chapter 4, the way to extract a singlet from a quantum dot is explored. The system that we model will be consisting of a triple dot and analyse the best way to get the singlet out, with each electron in a separate dot. The chief motivation is to create a singlet between separate dots in a time-scale much faster than that given by spinspin exchange interactions. In chapter 5, quantum logic gates in a triple dot system has been studied. Such gates have been widely studied in double and single quantum dots. Motivated by the advent of experimental set ups of triple dots, we have studied the natural quantum gates that came out of a triple dot system. There are still two spin quantum bits in the three dots and there is an empty intervening dot, which imparts the scheme some advantages, as well as a substantial difference from the class of schemes studied so far. In chapter 6, we model a large square dot. As we describe in chapter 2, the properties of the large dots make them behave with some interesting properties such as hosting Wigner molecules of electrons inside. We explore the application of these structures for quantum information processing. We show here how to get singlet/triplet measurement, entanglement swapping, and how to prepare a 1D AKLT state, using the square dot as a construction block of the system. Finally in chapter 7 conclusions and further work. Here we indicate the further work that could be done with the knowledge present in this thesis and motivated by future advances in the technology.
Classical computation relies heavily on information manipulation. Each component of a hardware needs to communicate with others, and this is done by encoding information into strings of bits and application of logical operations. When dealing with quantum technologies, there arises a new set of paradigms and devices, based on manipulations of qubits, the quantum analogues of conventional bits. This work investigates the generation and distribution of quantum entanglement, a uniquely non-classical correlation, across spin chains, which serve as promising platforms for quantum information processing. We systematically compare two distinct entanglement generation protocols: Protocol 1 (P1), based on alternating weak and strong couplings that create a band structure enabling an effective trimer-model approximation, and Protocol 2 (P2), which employs symmetric boundary couplings and virtual excitations to establish a direct effective interaction between the chain ends. Our results demonstrate that a protocol based on virtual excitations and optimized boundary couplings consistently outperforms its counterpart in speed, achieved entanglement, and robustness against fabrication imperfections and noise. Furthermore, by employing effective model reductions and open quantum systems techniques we provide a comprehensive framework for understanding the resilience of distributed entanglement in solid-state quantum devices. The characteristics of the virtual-coupling protocol highlight its potential for experimental implementation in scalable quantum technologies.
Spins in a solid-state environment and photons are both promising physical systems regarding the implementation of qubits. Whereas electron and nuclear spins act very well as localized qubits that are able to store and process quantum information, photons are the primary candidates to transmit quantum information between distant locations. Entanglement, on the other hand, is a fundamental resource of quantum information processing enabling, e.g., secure communication over long distances. The generation and manipulation of entanglement are thus fundamental steps in order to leverage the benefits of quantum information processing. The aim of this dissertation is therefore to theoretically investigate entangling mechanisms for various physical systems. A functioning source of entangled photons is a basic hardware component required for quantum communication. To this end, we study a system composed of semiconductor quantum wells inside a microcavity, known as intersubband cavity system, in which the interaction of the electronic system with the cavity field can reach the ultrastrong coupling regime. The ground state contains a finite number of photons, and we find that these photons are entangled. The amount of entanglement is quantified analytically, and maximal entanglement is found to be possible. The technique of entanglement purification allows to restore maximal entanglement that has decreased, e.g. due to decoherence. Purification requires quantum memory, a role for which electron spins in electrically-defined quantum dots are well suited. However, existing purification protocols are rather unpractical in this case. Here, the concept of asymmetric bilateral two-qubit operations is introduced to purify spin entanglement by harnessing the typical interaction between electrons in neighboring quantum dots. As it turns out, this concept can be applied to a variety of qubit systems, e.g. superconducting qubits or spins in nitrogen-vacancy centers in diamond. The latter example offers several possibilities to implement a qubit, of which the intrinsic nitro- gen nuclear spin has proven its viability in many ways. We develop a scheme to deterministically couple two nuclear spin qubits, in which the interaction is mediated by an optical cavity. It is found that an entangling two-qubit gate, also required for universal quantum computation, can be implemented with operation times below 100 nanoseconds, i.e. several orders of magnitude faster compared to the decoherence time of the nuclear spin. The verification of entanglement, which is required e.g. in entanglement-based quantum com- munication to detect an eavesdropping attack, typically involves a measurement of qubit states. Using the input-output formalism, we derive a fully quantum-mechanical model of an optical readout scheme to measure the spin state of an electron in a self-assembled quantum dot.
Since the seminal work by Shor who proposed a quantum algorithm factorizing integers into prime factors, it has become manifest that the laws of quantum mechanics provide resources for computation that overpower classical physics. The computational advantages that quantum physics offers have stimulated a tremendous amount of theoretical and experimental research. In this context, spin systems have played a major role, given that the spin degree of freedom -- with the paradigmatic case of the spin-1/2 of electrons -- represents an obvious candidate for the encoding of an elementary bit of quantum information (qubit). \n \nOn the other hand, however, quantum objects are very fragile entities, being very susceptible to the environment they reside in. This fragility of qubits is one of the main obstacles in the realization of a quantum computer. \n \nIn this thesis, we mainly address the two following questions relevant to quantum computation. \n \ni) How is it possible to realize quantum gates both in a reliable and scalable way? \n \nii) How can we store quantum information in a way that is resilient to the errors caused by the thermal environment? \n \nWe focus on spin systems and demonstrate that long-range spin-spin interactions in the models considered can have beneficial effects. \n \nIn their pioneering work, Loss and DiVincenzo proposed a way to perform quantum computation in a semiconductor-based architecture where the spin state of an electron trapped in a quantum dot is chosen to encode the elementary qubit. In this proposal, the spins are required to lie spatially close to each other, and this might complicate the realization of a scalable architecture. \n \nIn the first part of the thesis we thus propose a scheme that allows the constraint on the positioning of the qubits to be relaxed. This is achieved by introducing a ferromagnetic coupler between the distant qubits, to which it is coupled via a dipolar interaction. Most importantly, our proposal is applicable to any type of spin qubits and in particular to the technologically very relevant silicon-based qubits and NV-centers in diamond to which previous coupling schemes do not apply. \n \nAs additional key element, a quantum computer needs a memory capable of reliably storing quantum information in the presence of thermal fluctuations. \n \nThis brings us to the second part of this thesis, where we consider self-correcting memories, for which the protection against thermal noise is built-in at the hardware level. We propose physical models that exhibit these self-correcting properties, using as a starting point the well known topologically ordered toric code. In particular, we investigate how to induce long-range interactions between the spins of the toric code, since such interactions help increase the memory lifetime. \n \nAs a first step, we study a honeycomb quantum spin model coupled to delocalized cavity modes. We investigate the properties of the low-energy toric code Hamiltonian and show that the coupling to cavity modes prolongs the lifetime of the memory and offers a method to detect the presence of excitations. \nWhile the introduction of extended bosonic modes makes the model non-local, we also propose a purely local model consisting of a toric code embedded in a three-dimensional cubic lattice of hopping bosons; the low-energy sector of a toric code coupled to a three-dimensional Heisenberg ferromagnet in a broken-symmetry state realizes this model. Our analysis leads to an energy penalty for the creation of defects that grows linearly with the size L of the memory and thus to a lifetime increasing exponentially with L. \n \nIn the third part of this thesis, we study spin systems that support anyons, i.e., particles with fractional statistics. Similar to the toric code, such systems are topologically ordered: they are immune to local perturbations and quantum gates are implemented by non-local operations, namely the exchange of anyons, whose outcomes depend only on the topology of the exchange. Here again the fault-tolerance is achieved at the level of the hardware and physical systems supporting non-abelian anyons are thus promising platforms for quantum computation. \n \nWe focus on spin systems that exhibit some of these properties and specifically on variations of the honeycomb quantum spin model. We first investigate the exact solution of the honeycomb model in detail and derive an explicit formula for the projector onto the physical subspace. We use this result to study inhomogeneous open spin ladders, related to the honeycomb model, which can be tuned between topological and non-topological phases. We test the robustness of Majorana end states (MES) which emerge at the boundary between sections in different topological phases. Furthermore, we present a trijunction setup where MES can be braided. This is of interest since MES in these spin ladders potentially follow non-abelian braiding statistics. Finally, we study the ground states of the aforementioned ladders and show that they are free of vortices when the signs of the spin couplings are all positive or negative. To prove this, we use exact reflection-positivity-based methods as well as approximate methods. \n \nIn the last part of the thesis, we provide an extension of the Mermin-Wagner theorem to a system of lattice spins that are spin-coupled to itinerant and interacting charge carriers. We prove that neither (anti-) ferromagnetic nor helical long-range order is possible in one and two dimensions at any finite temperature (in the absence of spin-orbit). The fundamental question whether spontaneous ordering of the lattice spins occurs in these systems is of interest in the context of quantum computation; the polarization of nuclear spins coupled to a two-dimensional electron gas is a possible route towards the reduction of decoherence induced by the fluctuating Overhauser field in gate-defined quantum dots. \n \n
The goal of this thesis is to investigate theoretically the generation and behaviour of multipartite entanglement for solid-state nanosystems, in particular electron spin quantum bits (so-called 'qubits') in quantum dots. A quantum dot is a tiny potential well where a single electron can be trapped. A quantum bit can be implemented in this system by applying a magnetic field, and thereby lifting the degeneracy of the spin states of the electron. These spins can then be used as single qubits, and engineering many of these quantum dots next to each other gives as a register of qubits. In this scheme, the so-called Loss-DiVincenzo quantum computer, the single spins can be rotated e.g. by applying a time dependent magnetic field, and two spins can interact through controlling the potential barrier between them. A qubit cannot only be in a superposition of the two computational states 0 and 1 at the same time, but an even stranger characteristic arises for multiple qubits: this phenomenon is called entanglement and refers to a strong correlation between two or more qubits, which can not be achieved within the framework of classical physics, and exponentially enlarges the possible states for a N-qubit system as compared to a classical N-bit system. In this thesis we devise algorithms how to generate multipartite entangled states in electron spin qubits in quantum dots. We compare which classes of entangled states can be generated efficiently in this system. Once the states are created, they decay due to a process called decoherence. We compare how entangled states can be generated and detected in a realistic experiment, and which classes of states are the most suitable. Furthermore, we compare which classes conserve the entanglement, and quantify the robustness of various classes of entangled states. In the last chapter, we devise a scheme of how to execute a simple quantum algorithm, the Deutsch-Jozsa algorithm, in a system containing another type of solid-state qubit, the so-called flux qubit.