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Springer eBooks

Orbital Angular Momentum Effects of Light on Atoms; A Density-Matrix Theory

V. E. Lembessis, L. Allen, M. Babiker

Published Jan 1, 1996• 0 citations
Publisher
DOI
10.1007/978-1-4757-9742-8_58

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arXiv:0807.0130•Physical Review A•Nov 6, 2008•92 citations
We theoretically study the generation of orbital angular momentum (OAM) based on the four-wave mixing process in a diamond-type homogeneously broadened 85 R b atomic system. We use density matrix formalism at a weak field limit to explain the origin of vortex translation between different optical fields and a generated signal. We show how the singularities, which are omnipresent in the phases of the input optical vortex beams, can be profoundly mapped to atomic coherence in the transverse plane, which holds the origin of OAM translation. This translation process works well even for a moderately intense probe and control field, which enhances medium nonlinearity. The generation and manipulation of OAM of the light beam in a nonlinear medium may have important applications in optical tweezers and quantum information processing systems.
A theory is developed that leads to the description of the internal and gross motions of an atom interacting with an arbitrary light field. The general results are then applied to the case of a Laguerre-Gaussian (LG) mode, one of a class of modes of electromagnetic radiation that possess orbital angular momentum. A number of effects are predicted, notably, an azimuthal shift in the atomic resonance, a modified radiation pressure force, and an associated torque on the atom. It is pointed out that the effects originate in the processes of the transfer of linear and orbital angular momentum from the field to the atomic gross motion. The strengths of the effects are assessed in relation to the normal axial Doppler shift and the linear light pressure force. The motion of atoms and ions subject to the LG pressure force is studied by solving the classical equation of motion. Trajectories clearly exhibiting the effects of orbital angular momentum are displayed for a free atom and for an ion in a two-dimensional trap and in a Paul trap.
In this paper, we experimentally demonstrate that the photon pairs generated via spontaneous four-wave mixing in a hot atomic ensemble are in entangled orbital angular momentum (OAM) states. The density matrix of the OAM states of the photon pair is reconstructed, from which the fidelity to the maximal entangled state and the concurrence are estimated to be about 0.89 and 0.81, respectively. The experimental result also suggests the existence of the entanglement concerned with spatial degrees of freedom between the hot atomic ensemble and the Stokes photon.