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Springer eBooks

Optical Measurements of Weak Absorption Beyond Shot-Noise Limit

Wang Hai, Xie Changde, Qing Pan, Chenyang Xue, Yun Zhang, Peng Kunchi

Published Jan 1, 1997• 0 citations
Publisher
DOI
10.1007/978-1-4615-5923-8_48

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Absorption spectroscopy is one of the most widely used spectroscopic methods. The signal-to-noise ratio in conventional absorption spectroscopy is ultimately limited by the shot noise, which arises from the statistical property of the light used for the measurement. Here we show that the noise in absorption spectra can be suppressed below the shot-noise limit when entangled photon pairs are used for the light source. By combining broadband entangled photon pairs and multichannel detection, we realize the acquisition of sub-shot-noise absorption spectra in the entire visible wavelength. Furthermore, we demonstrate the strength of sub-shot-noise absorption spectroscopy for the identification and quantification of chemical species, which are two primary aims of absorption spectroscopy. For highly diluted binary mixture solutions, sub-shot-noise absorption spectroscopy enables us to determine the concentration of each chemical species with precision beyond the limit of conventional absorption spectroscopy. That is, sub-shot-noise absorption spectroscopy achieves superresolution in concentration measurements.
Absorption measurements are routinely used in science and engineering, it is an exceptionally versatile tool for most applications. For absorption measurements using laser beams of light, the sensitivity is theoretically limited by the shot noise due to the fundamental Poisson distribution of photon number in laser radiation. In practice, the shot-noise limit can only be achieved when all other sources of noise are eliminated. Here, we use bright squeezed light to demonstrate direct absorption measurement can be performed with sensitivity beyond the shot-noise limit. We present a practically realizable scheme, where the bright squeezed light is in the continuous-variable regime generated by the four-wave mixing process in an atomic rubidium vapor. This is a direct sub-shot-noise measurement of absorption, and more than 1 dB quantum advantage for the measurement sensitivity is demonstrated at faint absorption levels. A theoretical model that yields excellent agreements with experimental observations is also provided.