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Quantum Rabi Model Beyond the Electric Dipole Approximation

S. Zarrinkamar

Published Oct 28, 2026• 0 citations
Publisher

Abstract

We investigate a controlled beyond-electric-dipole extension of the quantum Rabi model in which the leading electric-dipole interaction is supplemented by an electric-quadrupole contribution. A central issue is the parity selection rule: for two exact atomic parity eigenstates of opposite parity, an electric-quadrupole transition matrix element vanishes. We therefore do not interpret the additional longitudinal coupling as an E2 transition between an opposite-parity pair. Instead, we consider an inversion-asymmetric (or parity-mixed) two-level system for which the two retained states may have different diagonal quadrupole moments. Projection of the multipolar interaction then produces a state-dependent term proportional to σz(a + a†), while the ordinary transition dipole produces the transverse term proportional to σx(a + a†). A state-independent quadrupolar contribution is removed by a bosonic displacement, leaving the effective Hamiltonian H =ωa†a+∆σz/2+gσx(a+a†)+gQσz(a+a†). This construction connects the beyond-dipole physical problem to the well-studied class of Rabi models with simultaneous transverse and longitudinal coupling, including asymmetric or biased Rabi models. We make this relation explicit by a constant spin rotation, which maps the model to a biased Rabi Hamiltonian with effective coupling κ = √g2 +g2Q and bias δ = ∆gQ/(2κ). We then derive the corresponding second-order Bargmann differential equation and solve its exceptional polynomial sector using a Zhang-type functional Bethe ansatz. The resulting Bethe equations, root-sum constraint, exceptional energy branches, and the first nontrivial parameter condition are obtained explicitly. In the limit gQ → 0, the construction continuously recovers the ordinary Rabi exceptional sector. From an experimental perspective, the connection with demonstrated quadrupolar light--matter coupling in engineered quantum systems suggests that the present framework may have relevance for spectroscopic studies of beyond-electric-dipole interactions, although a direct experimental realization of the specific effective model considered here remains to be established [20].

DOI
10.1364/opticaopen.34750764

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We investigate a controlled beyond-electric-dipole extension of the quantum Rabi model in which the leading electric-dipole interaction is supplemented by an electric-quadrupole contribution. A central issue is the parity selection rule: for two exact atomic parity eigenstates of opposite parity, an electric-quadrupole transition matrix element vanishes. We therefore do not interpret the additional longitudinal coupling as an E2 transition between an opposite-parity pair. Instead, we consider an inversion-asymmetric (or parity-mixed) two-level system for which the two retained states may have different diagonal quadrupole moments. Projection of the multipolar interaction then produces a state-dependent term proportional to σz(a + a†), while the ordinary transition dipole produces the transverse term proportional to σx(a + a†). A state-independent quadrupolar contribution is removed by a bosonic displacement, leaving the effective Hamiltonian H =ωa†a+∆σz/2+gσx(a+a†)+gQσz(a+a†). This construction connects the beyond-dipole physical problem to the well-studied class of Rabi models with simultaneous transverse and longitudinal coupling, including asymmetric or biased Rabi models. We make this relation explicit by a constant spin rotation, which maps the model to a biased Rabi Hamiltonian with effective coupling κ = √g2 +g2Q and bias δ = ∆gQ/(2κ). We then derive the corresponding second-order Bargmann differential equation and solve its exceptional polynomial sector using a Zhang-type functional Bethe ansatz. The resulting Bethe equations, root-sum constraint, exceptional energy branches, and the first nontrivial parameter condition are obtained explicitly. In the limit gQ → 0, the construction continuously recovers the ordinary Rabi exceptional sector. From an experimental perspective, the connection with demonstrated quadrupolar light--matter coupling in engineered quantum systems suggests that the present framework may have relevance for spectroscopic studies of beyond-electric-dipole interactions, although a direct experimental realization of the specific effective model considered here remains to be established [20].
We investigate a controlled beyond-electric-dipole extension of the quantum Rabi model in which the leading electric-dipole interaction is supplemented by an electric-quadrupole contribution. A central issue is the parity selection rule: for two exact atomic parity eigenstates of opposite parity, an electric-quadrupole transition matrix element vanishes. We therefore do not interpret the additional longitudinal coupling as an E2 transition between an opposite-parity pair. Instead, we consider an inversion-asymmetric (or parity-mixed) two-level system for which the two retained states may have different diagonal quadrupole moments. Projection of the multipolar interaction then produces a state-dependent term proportional to σz(a + a†), while the ordinary transition dipole produces the transverse term proportional to σx(a + a†). A state-independent quadrupolar contribution is removed by a bosonic displacement, leaving the effective Hamiltonian H =ωa†a+∆σz/2+gσx(a+a†)+gQσz(a+a†). This construction connects the beyond-dipole physical problem to the well-studied class of Rabi models with simultaneous transverse and longitudinal coupling, including asymmetric or biased Rabi models. We make this relation explicit by a constant spin rotation, which maps the model to a biased Rabi Hamiltonian with effective coupling κ = √g2 +g2Q and bias δ = ∆gQ/(2κ). We then derive the corresponding second-order Bargmann differential equation and solve its exceptional polynomial sector using a Zhang-type functional Bethe ansatz. The resulting Bethe equations, root-sum constraint, exceptional energy branches, and the first nontrivial parameter condition are obtained explicitly. In the limit gQ → 0, the construction continuously recovers the ordinary Rabi exceptional sector. From an experimental perspective, the connection with demonstrated quadrupolar light--matter coupling in engineered quantum systems suggests that the present framework may have relevance for spectroscopic studies of beyond-electric-dipole interactions, although a direct experimental realization of the specific effective model considered here remains to be established [20].
The Rabi Hamiltonian, describing the interaction between a two-level atomic system and a single-cavity mode of the electromagnetic field, is one of the fundamental models in quantum optics. The model becomes exactly solvable by considering an atom without permanent dipole moments, whose excitation energy is quasiresonant with the cavity photon energy, and by neglecting the nonresonant (counter-rotating) terms. In this case, after including the decay of either the atom or the cavity mode to a continuum, one can derive the well-known phenomenology of quasiresonant transitions, including the fluorescence triplets. In this work we consider the most general Rabi model, incorporating the effects of permanent atomic electric dipole moments. Based on a perturbative analysis, we compare the intensities of emission lines induced by rotating terms, counter-rotating terms, and parity-symmetry-breaking terms in order to identify the parameter regimes in which these different contributions play a significant role. The analysis reveals that the emission strength related to the existence of permanent dipoles may surpass the one due to the counter-rotating interaction terms but is usually much weaker than the emission due to the main, resonant coupling. This ratio can be modified in systems with a reduced dimensionality or by engineering the energy spectral density of the continuum.
We have studied the two-qubit quantum Rabi model in the asymmetric case and its generalizations with dipole and Heisenberg-type qubit-qubit interactions. The solutions are obtained analytically with eigenstates given in terms of the extended coherent states or photon number states. For identical qubit-photon couplings, a novel type of quasi-exact solution which exists for all coupling values with constant eigenenergy is found, leading to level crossings within the same parity subspace even for non-identical qubits. In contrast to the quasi-exact eigenstates of the single-qubit model, these exceptional eigenstates are formed by just a few Fock states (photon number bounded from above at one or three), and the condition for them depends only on a fine-tuning of the qubit level splittings with respect to the photon energy, but not on the coupling to the photon field if the qubit-qubit interaction is not taken into consideration. This makes them excellent candidates for direct experimental observation within circuit quantum electrodynamics (QED) and application in single photon experiments. Besides, exceptional solutions with finite photon numbers N are also found.
We formulate and solve an effective spin-one quantum Rabi model motivated by the physical spin-one sector of the ten-component Duffin--Kemmer--Petiau (DKP) theory. After the constrained DKP components are separated from the three physical spin projections, the internal sector is represented as a qutrit. Under a single-mode and magnetic-dipole approximation, its coupling to a quantized electromagnetic field has the spin-one Rabi form g(a+a†)Sx. We derive the regular spectrum of this model in the Bargmann representation. The exact parity symmetry reduces the three-component problem to independent scalar three-term recurrences, from which parity-resolved spectral functions are obtained as continued fractions. The pole energies generated by eliminating the outer spin components are treated separately, allowing exceptional finite-polynomial states to be identified without confusing them with regular zeros of the continued fractions. Numerical comparison with direct Fock-space diagonalization confirms the regular spectral construction to better than 5×10−13 for a representative parameter set. The result establishes an exact spectral framework for a qutrit generalization of the quantum Rabi model and states explicitly the assumptions required for its connection with spin-one DKP dynamics.
We formulate and solve an effective spin-one quantum Rabi model motivated by the physical spin-one sector of the ten-component Duffin--Kemmer--Petiau (DKP) theory. After the constrained DKP components are separated from the three physical spin projections, the internal sector is represented as a qutrit. Under a single-mode and magnetic-dipole approximation, its coupling to a quantized electromagnetic field has the spin-one Rabi form g(a+a†)Sx. We derive the regular spectrum of this model in the Bargmann representation. The exact parity symmetry reduces the three-component problem to independent scalar three-term recurrences, from which parity-resolved spectral functions are obtained as continued fractions. The pole energies generated by eliminating the outer spin components are treated separately, allowing exceptional finite-polynomial states to be identified without confusing them with regular zeros of the continued fractions. Numerical comparison with direct Fock-space diagonalization confirms the regular spectral construction to better than 5×10−13 for a representative parameter set. The result establishes an exact spectral framework for a qutrit generalization of the quantum Rabi model and states explicitly the assumptions required for its connection with spin-one DKP dynamics.
The quantum Rabi model (QRM), describing a two-level system coupled to a quantum harmonic oscillator, is one of the simplest and most ubiquitous interaction models in quantum mechanics. Despite its simplicity, the QRM has found applications in various fields of physics. The most exciting realization of the QRM nowadays is arguably the circuit quantum electrodynamics (QED) system, where an on-chip artificial atom (or a qubit) is coupled to a transmission line or a waveguide. The qubits in circuit QED systems contain a bias term, which breaks the Z_2 symmetry in the QRM. Therefore, the precise model realized in circuit QED systems is referred to as the asymmetric quantum Rabi model (AQRM). This thesis explores theoretical methods to treat the AQRM and develops a complete approach to describe its energy landscape. The hidden symmetry of the AQRM is investigated in detail, and seen to be a rather general phenomenon in light-matter interaction models. The equivalence between the generalised Poschl-Teller potential and the spectrum of the AQRM is also established. Chapter 1 is dedicated to reviewing the analytic solutions and conventional approximations to the QRM/AQRM. Regarding the analytic solutions, the analytic results in terms of the transcendental functions determining the eigenspectrum of the AQRM are collected. Special emphasis is placed on the isolated closed-form exceptional solutions to the AQRM. Due to the lack of simple closed-form expressions for the general eigenvalues, some well-known approximations are considered. In Chapter 2, a generalised adiabatic approximation (GAA) is developed to calculate the eigenvalues of the excited states of the QRM and apply it to the AQRM. The GAA is based on the similarity between the exact exceptional solutions and the Laguerre polynomials. By construction, the GAA always has exact exceptional energy and approximates the regular spectrum with rather good agreement in a large parameter regime. Furthermore, the GAA is applied to the AQRM and shown to correctly recover the conical intersections in the energy landscape. The geometric phases around these conical intersections are calculated analytically as an illustrative example. In Chapter 3, a physically motivated variational wave function is presented for the ground state of the AQRM. The wave function is a weighted superposition of squeezed coherent states entangled with non-orthogonal qubit states and relies only on three variational parameters in the regimes of interest. The variational expansion describes the ground state remarkably well in almost all parameter regimes, especially with arbitrary bias. The results show that the variational expansion is a significant improvement over the existing approximations for the AQRM. In Chapter 4, the hidden symmetry and tunnelling dynamics in the AQRM and several related models are analysed in detail. The AQRM has a broken Z_2 symmetry, with generally a non-degenerate eigenvalue spectrum. In some special cases of the related models, stable level crossings typical of the Z_2-symmetric quantum Rabi model are recovered. It is thus shown that this hidden symmetry is not limited to the AQRM, but exists in various related light-matter interaction models. In Chapter 5, starting with the Gaudin-like Bethe ansatz equations associated with the quasi-exactly solved (QES) exceptional points of the AQRM, a spectral equivalence is established with QES hyperbolic Schrodinger potentials. This leads to particular QES Poschl-Teller potentials. The complete spectral equivalence is then established between the AQRM and generalised Poschl-Teller potentials. Conclusions and future directions are presented in the final Chapter 6.