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Delocalised Excitation and Conditional Negative Delays of Single Photons

Andrii Myshko

Published Jun 12, 2025• 0 citations
Publisher

Abstract

We analyse the recent experiment of Angulo et al. (arXiv:2409.03680), where single photons traversing an ultracold 87Rb cloud exhibit negative conditional group delays. By modelling the process with a Dicke-type delocalised excitation, we establish a quantitative link to the ∇U tired-light framework developed in “Revisiting Tired-Light Cosmology: Photon Ageing in a Single ∇U Field” (DOI 10.5281/zenodo.15648007). The laboratory delay (–35 ps) scales to an effective β ≈1.8×10⁻³¹ s, consistent in order of magnitude with the cosmological β=1.4×10⁻²⁹ s. We derive phase-dependent delay, recoil distribution and Hong–Ou–Mandel visibility as falsifiable predictions. The study shows how frequency drift can occur without geometric scattering, strengthening the physical intuition behind internal photon ageing.

DOI
10.5281/zenodo.15650171

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Negative Dwell Times as Resolvent Derivatives: A Structural Operator-Theoretic Explanation of 𝑻𝑻=𝒕𝒈

Ilkka Linnas

A structural operator-theoretic account of negative group delays and post-selected excitation times in resonant atomic media. Within a scalar Lorentzian propagation model, the excitation time and the optical delay are shown to be parameter derivatives of the same frequency-resolved transmission amplitude — the first with respect to the atomic transition frequency, the second with respect to the optical frequency. Because the internal resolvent R = (z − ω)⁻¹, z = ω₀ − iΓ/2, depends on these only through their difference, the two are linked by an exact identity. For a fixed detected frequency, T_T(ω) = Re[i ∂_{ω₀} ln t_med(ω)] (Theorem A); its difference from the local Wigner delay is exactly A Re R(ω), which vanishes at line centre (Corollary B). For an unresolved detector, coarse-graining gives T_T = t_g^det whenever the detected spectral weight is even in detuning — a condition of symmetry, not of bandwidth (Theorem C). Negativity is treated separately from the equality. Causality is established from the analyticity of the retarded response and the full two-pole susceptibility: negative delays are properties of the pulse centroid, and the front velocity remains c exactly. Appendices cover departures from the idealised model, and a Python script reproduces all quoted numerics. All identities are exact within the stated first-order propagation model. Version note. Supersedes the May 2026 deposit. The central derivation has been replaced: the earlier conditional-probability argument is withdrawn. Keywords: post-selected excitation time, weak value, group delay, resolvent, Feynman–Hellmann identity, Lorentzian resonance, anomalous dispersion, front velocity, causality, quantum optics

•May 17, 2026•0 citations
We analyse the recent experiment of Angulo et al. (arXiv:2409.03680), where single photons traversing an ultracold 87Rb cloud exhibit negative conditional group delays. By modelling the process with a Dicke-type delocalised excitation, we establish a quantitative link to the ∇U tired-light framework developed in “Revisiting Tired-Light Cosmology: Photon Ageing in a Single ∇U Field” (DOI 10.5281/zenodo.15648007). The laboratory delay (–35 ps) scales to an effective β ≈1.8×10⁻³¹ s, consistent in order of magnitude with the cosmological β=1.4×10⁻²⁹ s. We derive phase-dependent delay, recoil distribution and Hong–Ou–Mandel visibility as falsifiable predictions. The study shows how frequency drift can occur without geometric scattering, strengthening the physical intuition behind internal photon ageing.
Recent experiments at the University of Toronto (Angulo et al., 2024) have demonstrated negative group delay and negative dwell times for photons transmitted through ultracold rubidium-85 atomic clouds using weak measurement techniques.Within the framework of Cosmological Thermosynthesis Theory v3.2 (TTC v3.2), we reinterpret these phenomena as manifestations of topological phase interference in the primordial etherion superfluid. We derive formally that: (i) the negativegroup delay arises from coherent forward scattering mediated by etherion-induced phase gradients; (ii) weak values of atomic dwell time acquire negative contributions from entropic-gravitational coupling Γg · ∆S; and (iii) the observed coincidence between pulse advance and atomic excitation time reflects the underlying topological constraint L123 = L12 = 1/2 on the etherion field configuration. We update the model with observational constraints from ultracold quantum optics (2024–2026)and demonstrate quantitative consistency with TTC v3.2 predictions for phase-shift distributions, weak-value statistics, and coherence preservation in dispersive media. Falsifiable predictions for next-generation quantum interferometry and weakmeasurement protocols are presented.
When a single photon propagates through a cloud of two-level atoms, part of its energy is temporarily stored as a collective atomic excitation. This raises a fundamental question: is it possible to meaningfully quantify how long the photon spends in the form of an atomic excitation? If so, does this duration depend on whether the photon is ultimately transmitted through the cloud or scattered by the atoms? These questions motivated recent experimental work by some of us [Sinclair et al., PRX Quantum 3, 010314 (2022)], but until now there has been no theoretical prediction for these conditional durations. We answer these questions by extending the concept of a dwell time from quantum tunneling to light–matter interactions, introducing an experimentally measurable “atomic excitation time.” Using the weak-value formalism combined with quantum trajectory theory, we derive analytical expressions for this time conditioned on the photon being transmitted through the cloud or scattered into a side mode. We show that, for transmitted photons, this time is equal to the (spectrally averaged) group delay, even in regimes where the group delay is negative. For scattered photons, the time is given by the sum of an ensemble-averaged group delay and an always-positive Wigner time delay, well known in elastic scattering theory. Finally, we present a toy model that explains how such negative dwell times can arise as a result of quantum interference. This work provides new insight into the complex and surprising histories of photons traveling through absorptive media.
We consider the time delay of interfering single photons oppositely traveling in the Kerr metric of a rotating massive object. Classically, the time delay shows up as a phase difference between coherent sources of light. In quantum mechanics, the loss in visibility due to the indistinguishability of interfering photons is directly related to the time delay. We can thus observe the Kerr frame dragging effect using the Hong–Ou–Mandel dip, a purely quantum mechanical effect. By Einstein's equivalence principle, we can analogously consider a rotating turntable to simulate the Kerr metric. We look at the feasibility of such an experiment using optical fiber and note a cancellation in the second order dispersion but a direction dependent difference in group velocity. However, for the chosen experimental parameters, we can effectively assume light propagating through a vacuum.
Recent weak-measurement experiments performed by the University of Toronto reported an apparent negative transmission delay associated with photons propagating through a cold rubidium atomic cloud, raising fundamental questions concerning the physical interpretation of negative interaction time. In this work, we develop a second-quantized synchronization framework to describe resonant photon transmission through a collective atomic ensemble. Both the incident photon and the collective atomic excitation are treated as coupled quantum resonators interacting through an effective synchronization Hamiltonian with finite lifetime broadening. An analytical expression for the transmission amplitude and its phase response is derived, demonstrating that the apparent transmission delay naturally becomes negative on the resonance wings owing to coherent interference between direct transmission and resonant absorption–reemission pathways. In contrast, the microscopic excitation time, defined by the time integral of the atomic excitation-number operator, is rigorously proven to remain nonnegative. Numerical simulations using representative parameters for the Toronto cold-rubidium experiment reproduce the experimentally observed order of magnitude of the negative weak delay without introducing empirical fitting parameters. The calculations further show how the apparent delay depends systematically on frequency detuning and the effective collective coupling strength, providing experimentally testable predictions beyond the existing weak-value interpretation. The present synchronization framework therefore resolves the apparent paradox of negative transmission time by demonstrating that the observed temporal advance originates from phase synchronization and quantum interference rather than from a negative microscopic interaction time.
A structural operator-theoretic account of negative group delays and post-selected excitation times in resonant atomic media. Within a scalar Lorentzian propagation model, the excitation time and the optical delay are shown to be parameter derivatives of the same frequency-resolved transmission amplitude — the first with respect to the atomic transition frequency, the second with respect to the optical frequency. Because the internal resolvent R = (z − ω)⁻¹, z = ω₀ − iΓ/2, depends on these only through their difference, the two are linked by an exact identity. For a fixed detected frequency, T_T(ω) = Re[i ∂_{ω₀} ln t_med(ω)] (Theorem A); its difference from the local Wigner delay is exactly A Re R(ω), which vanishes at line centre (Corollary B). For an unresolved detector, coarse-graining gives T_T = t_g^det whenever the detected spectral weight is even in detuning — a condition of symmetry, not of bandwidth (Theorem C). Negativity is treated separately from the equality. Causality is established from the analyticity of the retarded response and the full two-pole susceptibility: negative delays are properties of the pulse centroid, and the front velocity remains c exactly. Appendices cover departures from the idealised model, and a Python script reproduces all quoted numerics. All identities are exact within the stated first-order propagation model. Version note. Supersedes the May 2026 deposit. The central derivation has been replaced: the earlier conditional-probability argument is withdrawn. Keywords: post-selected excitation time, weak value, group delay, resolvent, Feynman–Hellmann identity, Lorentzian resonance, anomalous dispersion, front velocity, causality, quantum optics
A structural operator-theoretic account of negative group delays and post-selected excitation times in resonant atomic media. Within a scalar Lorentzian propagation model, the excitation time and the optical delay are shown to be parameter derivatives of the same frequency-resolved transmission amplitude — the first with respect to the atomic transition frequency, the second with respect to the optical frequency. Because the internal resolvent R = (z − ω)⁻¹, z = ω₀ − iΓ/2, depends on these only through their difference, the two are linked by an exact identity. For a fixed detected frequency, T_T(ω) = Re[i ∂_{ω₀} ln t_med(ω)] (Theorem A); its difference from the local Wigner delay is exactly A Re R(ω), which vanishes at line centre (Corollary B). For an unresolved detector, coarse-graining gives T_T = t_g^det whenever the detected spectral weight is even in detuning — a condition of symmetry, not of bandwidth (Theorem C). Negativity is treated separately from the equality. Causality is established from the analyticity of the retarded response and the full two-pole susceptibility: negative delays are properties of the pulse centroid, and the front velocity remains c exactly. Appendices cover departures from the idealised model, and a Python script reproduces all quoted numerics. All identities are exact within the stated first-order propagation model. Version note. Supersedes the May 2026 deposit. The central derivation has been replaced: the earlier conditional-probability argument is withdrawn. Keywords: post-selected excitation time, weak value, group delay, resolvent, Feynman–Hellmann identity, Lorentzian resonance, anomalous dispersion, front velocity, causality, quantum optics