This thesis details the development of a new ultracold atom experiment hosting (bosonic) ³⁹K, from the drawing board to its eventual utilisation in studying atom-light scattering in a uniform system of ultracold atoms with tunable interactions. This work is conceptually divided into three parts. The first part (Inferno), covering Chapters 1 - 3, establishes the theoretical framework for ultracold Bose gases and details the design philosophy and construction of the machine at the heart of this work. The primary benchmarks of the experiment include the production of harmonically trapped condensates of up to 1.2×10⁶ atoms in ≈ 12 s, uniform 3D degenerate gases of 0.8×10⁶ atoms in ≈ 14 s, and uniform 2D systems of 1.5×10⁵ atoms in ≈ 20 s. The second part (Purgatorio), covering Chapters 4 and 5, builds upon the machine's established capabilities. First, we detail the process by which we generate a uniform condensate used for our atom-light scattering experiments. Second, we demonstrate an alternative, all-optical route to quantum degeneracy that bypasses the usage of a magnetic trap in the sequence which is a central component of conventional methods (such as the one in Chapter 3). This technique is an intermediate step between sub-Doppler cooling and optical dipole trap (ODT) loading, designed to optimise the initial conditions for optical evaporation in the ODT. In particular, our method uses the simultaneous compression and cooling of a sub-Doppler cloud within a dynamically tunable blue-detuned tube trap, thereby enhancing the atom loading fraction into the ODT, where the final evaporation towards degeneracy occurs. The improvement of the initial conditions is the critical step that allows this all-optical sequence to successfully reach quantum degeneracy. The third and final part (Paradiso), covering Chapter 6, presents the main scientific result of this thesis. Here, we study the scattering between off-resonant light and a uniform Bose gas with tunable interactions, and illustrate the extreme sensitivity of atom-light scattering to local atomic correlations. We begin by showing that for the (quasi-)ideal (non-interacting) gas, the observed enhancement in atom-light scattering is captured by quantum statistical effects. This picture changes dramatically however, once we introduce atomic interactions. We find that due to the presence of local correlation effects, even weak repulsive interactions can completely suppress the enhancement in atom-light scattering, while attractive ones increase it above the ideal-gas level. Moreover, by studying the dynamics after an interaction quench, we show that the post-quench correlation dynamics are orders of magnitude faster than the dynamics associated with changes to momentum-space occupations or the density distribution. Our results thus establish off-resonant light scattering as a powerful and sensitive probe of equilibrium and non-equilibrium many-body physics.
This thesis details the development of a new ultracold atom experiment hosting (bosonic) ³⁹K, from the drawing board to its eventual utilisation in studying atom-light scattering in a uniform system of ultracold atoms with tunable interactions. This work is conceptually divided into three parts. The first part (Inferno), covering Chapters 1 - 3, establishes the theoretical framework for ultracold Bose gases and details the design philosophy and construction of the machine at the heart of this work. The primary benchmarks of the experiment include the production of harmonically trapped condensates of up to 1.2×10⁶ atoms in ≈ 12 s, uniform 3D degenerate gases of 0.8×10⁶ atoms in ≈ 14 s, and uniform 2D systems of 1.5×10⁵ atoms in ≈ 20 s. The second part (Purgatorio), covering Chapters 4 and 5, builds upon the machine's established capabilities. First, we detail the process by which we generate a uniform condensate used for our atom-light scattering experiments. Second, we demonstrate an alternative, all-optical route to quantum degeneracy that bypasses the usage of a magnetic trap in the sequence which is a central component of conventional methods (such as the one in Chapter 3). This technique is an intermediate step between sub-Doppler cooling and optical dipole trap (ODT) loading, designed to optimise the initial conditions for optical evaporation in the ODT. In particular, our method uses the simultaneous compression and cooling of a sub-Doppler cloud within a dynamically tunable blue-detuned tube trap, thereby enhancing the atom loading fraction into the ODT, where the final evaporation towards degeneracy occurs. The improvement of the initial conditions is the critical step that allows this all-optical sequence to successfully reach quantum degeneracy. The third and final part (Paradiso), covering Chapter 6, presents the main scientific result of this thesis. Here, we study the scattering between off-resonant light and a uniform Bose gas with tunable interactions, and illustrate the extreme sensitivity of atom-light scattering to local atomic correlations. We begin by showing that for the (quasi-)ideal (non-interacting) gas, the observed enhancement in atom-light scattering is captured by quantum statistical effects. This picture changes dramatically however, once we introduce atomic interactions. We find that due to the presence of local correlation effects, even weak repulsive interactions can completely suppress the enhancement in atom-light scattering, while attractive ones increase it above the ideal-gas level. Moreover, by studying the dynamics after an interaction quench, we show that the post-quench correlation dynamics are orders of magnitude faster than the dynamics associated with changes to momentum-space occupations or the density distribution. Our results thus establish off-resonant light scattering as a powerful and sensitive probe of equilibrium and non-equilibrium many-body physics.
This thesis includes both experimental and theoretical investigations, presented in a series of eight papers. The experimental part ranges from the construction procedures of an apparatus for Bose-Einstein condensates, to full scale experiments using three different set-ups for ultracold atoms in optical lattices. As one of the main themes of the thesis, an experimental apparatus for production of Bose-Einstein Condensates is under construction. A magneto-optically trapped sample, hosting more than 200 million 87Rb atoms, have successfully been loaded into a magnetic trap with high transfer rate. The lifetime of the sample in the magnetic trap is in the range of 9 s, and the atoms have been shown to respond to evaporative cooling. The experiment is ready for optimization of the magnetic trap loading, and evaporative cooling parameters, which are the final steps for reaching Bose-Einstein condensation. The set-up is designed to host experiments including variable geometry optical lattices, and includes the possibility to align laser beams with high angular precision for this purpose. The breakdown of Bloch waves in a Bose-Einstein condensate is studied, attributed to the effect of energetic and dynamical instability. This experimental study is performed using a Bose-Einstein condensate in a moving one-dimensional optical lattice at LENS, Florence Italy. The optical lattice parameters, and the thermal distribution of the atomic sample required to trigger the instabilities, are detected, and compared with a theoretical model developed in parallel with the experiments. In close connection with these one-dimensional lattice studies, an experimental survey to characterize regimes of superradiant Rayleigh scattering and Bragg scattering is presented. Tunneling properties of repulsively bound atom pairs in double well potentials are characterized in an experiment at Johannes Gutenberg University, Mainz Germany. A three-dimensional optical lattice, producing an array of double wells with tunable properties is let to interact with a Bose-Einstein condensate. Pairs of ultracold atoms are produced on one side in the double wells, and their tunneling behavior, dependent on potential barrier and repulsion properties, is studied. A theoretical study of the crossover between one- and two-dimensional systems has been performed. The simulations were made for a two-dimensional array of atoms, where the behavior for different tunneling probabilities and atom-atom repulsion strengths was studied. Scaling relations for systems of variable sizes have been examined in detail, and numerical values for the involved variables have been found.
Atom chips are an excellent tool for studying ultracold degenerate quantum gases, due to the high degree of controllability afforded by the precise potentials generated from the current-carrying microfabricated wires on the chip surface. The geometries of the trapping potentials are inherently capable of realising extreme aspect ratios, and therefore creating model systems with effectively reduced dimensionality, particularly the theoretically-tractable one-dimensional Bose gas. In addition, the temporal tunability makes it possible to impart non-adiabatic changes on the trapping potentials, allowing experimental investigation of samples which have been brought out of equilibrium - a situation which is not fully theoretically understood. This thesis describes the implementation, development and characterisation of an experimental system for producing the first Bose-Einstein condensates of atomic rubidium 87 gas trapped on the surface of an atom chip in Nottingham. Such an apparatus is very complex and requires careful characterisation in order to run in a stable and reliable way. Details of the experimental setup are thoroughly outlined, including the vacuum system, lasers, electronics, computer control and timing, and the optical imaging system. A newly installed compact two-dimensional magneto-optical trap provides an loading rate of 5e7 atoms per second for loading a three-dimensional mirror-magneto-optical trap with 1.5e8 atoms, at a temperature of 300uK within 10s. The cloud is then sub-Doppler cooled to 50uK, and spin-polarised with 96% purity into the |F=2,mF=+2> ground state within 5ms, in preparation for loading a purely magnetic trap. A millimeter sized copper Z-shaped conductor located beneath the atom chip surface creates a Ioffe-Pritchard magnetic trap, into which the laser cooled cloud is loaded with 70% efficiency, and can be held with a vacuum-limited lifetime of 40s. Evaporative cooling then pre-cools the sample to below 20uK within 10s, to allow the subsequent loading into potentials created by the atom chip with 100% efficiency. A final evaporation stage then cools the cloud below the phase transition temperature of 800nK, resulting finally in pure BECs with 105 atoms confined using the atom chip. Key measurements of various properties of the trapped condensates are presented, which are important in order to characterise the system fully, and to compare with theoretical expectations. In particular, included are the variation of condensate fraction with temperature, the BEC expansion dynamics, and the condensate lifetime in the trap, for example. Finally, it is demonstrated how BECs can be produced on the atom chip without the use of external macroscopic coils, achieved by using novel, integrated sheet structures located beneath the chip surface - unique to this experimental system - to create the necessary bias fields.
Research on degenerate quantum gases of dilute atomic gases has become a well established field in modern physics and revealed many astonishing phenomena. The first experiments on Bose and Fermi gases at low temperatures aimed to prove the predictions of quantum mechanics on a macroscopic scale. Since then we make use of Bose and Fermi gases and mixtures of any combination to model other many body systems. A property of Bose Einstein condensates is superfluidity which we want to investigate further in toroidal potentials with a new apparatus which can produce an all-optical BEC. This means trapping thermal atoms in an optical dipole trap and cooling the sample by evaporation into the quantum degenerate regime. This new technique was first successfully demonstrated by M.D. Barrett et al. in 2001 and promises to be faster and simpler than the well established and common way of evaporation in magnetic traps. A new apparatus was built by the author and we report on the experimental details of the trapping of 87Rb atoms from a hot vapour and cooling them in a magneto-optical trap, and further evaporation to quantum degeneracy in a crossed optical dipole trap operating at a wavelength of l = 1064nm, with accurate control of the power in both beams via a feedback loop. The evaporation of neutral atoms of 87Rb in far red detuned optical dipole traps using linearly polarised laser light is spin independent, and mixed spinor condensates of the F=1 manifold can be formed. As an empirical technique we found by applying a magnetic gradient field during the final evaporation that we can selectively populate mF spin states or prepare mixtures. This intriguing mechanism was found earlier as well by M. S. Chang, but is yet not fully understood and subject of our future research. We can now routinely prepare an almost pure condensate containing up to 7000 atoms in the condensed phase purely in the mF = 0 spin state. This thesis contains the theoretical framework of Bose-Einstein condensation with in mean-field theory, the concepts of cooling of atoms in magneto-optical traps, the trapping and evaporation in optical dipole traps and the experimental realisation. In the future this experiment will be extended by a fast scanning dipole trap to apply arbitrary time averaged potentials of more complex geometries, such as toroidal traps to study the effects of superfluidity in a periodic potential. The production of toroidal traps and cold atoms in such a trap are outlined in this thesis.
This thesis presents the development of an experimental apparatus to produce Bose-Einstein condensates (BECs) with tunable interparticle interactions. The ability to precisely control the strength of these interactions, and even to switch them from repulsive to attractive, allows one to probe novel regimes of condensate physics, from the collapse of attractively interacting BECs and the formation of solitary matter-waves to the observation of beyond mean-field effects in strongly repulsive condensates. The construction and characterisation of both a single and crossed beam optical dipole trap is presented. In the single beam case we develop a technique allowing the guided transport of atoms along the beam and up to a room-temperature surface; a technique which can be used to evaporatively cool the trapped atomic cloud. We produce Bose-Einstein condensates of 87Rb in the F=1, mF=-1 state in this trap, comparing the effect of beam waist on the evaporation trajectory. In the crossed beam trap Bose-Einstein condensation of 87Rb is realised in three distinct trapping configurations, along with a 1D optical lattice formed by changing the polarisation of the beams. A method of direct cooling of 85Rb atoms in the crossed trap is developed using a magnetic Feshbach resonance to precisely tune both the elastic and inelastic scattering properties of the atoms. The resonance used for this work occurs at 155G in collisions between atoms in the F=2, mF=-2 state of 85Rb. Bose-Einstein condensates of up to 40,000 85Rb atoms are formed in this trap and we demonstrate the presence of tunable interatomic interactions, exploring the collapse phenomenon associated with attractive condensates. By loading the 85Rb condensate into a quasi-1D waveguide we show that stable attractive condensates can be created, taking the form of bright solitary matter-waves. We observe a solitary wave of ~2,000 atoms which propagates, without dispersion, along the waveguide over a distance of ~1.1mm. The particle-like nature of the solitary wave is demonstrated by classical reflection of the wavepacket from a repulsive Gaussian barrier.
The three experiments described in this thesis investigate fundamental properties of ultracold atoms. Using laser cooling and evaporative cooling, a dilute gas of sodium atoms is cooled to ~100 nK. Under these circumstances a Bose-Einstein condensate (BEC) forms, where millions of atoms collapse into the lowest energy state of the system and share a macroscopic wavefunction. The experiments are done in an ultrahigh vacuum and the atoms are manipulated remotely using laser beams, magnetic fields, and RF-fields. Using ultracold atoms allows unprecedented control over the internal and external degrees of freedom of the system, making it very suitable for precision measurements. Ultracold atoms also serve as a model system for more complicated or remote fields such as solid-state physics and cosmology. In the first experiment the refractive index of an ultracold bosonic gas is studied. The atomic clouds are analyzed for temperature and number of particles using nearly non-destructive phase-contrast imaging. After each pulse of probe light a small fraction of the atoms is lost, while the cloud is simultaneously slightly heated. This makes it possible to study the scattering rate as a function of temperature using only a single sample. It is observed that the scattering rate increases below the critical temperature for BEC by more than a factor of 3 compared to the classical value. This enhancement is in good agreement with the predictions by theoretical work that takes two-body correlation and the Lorentz-Lorenz correction into account. The method is also used to perform calorimetry on the Bose gas and directly measure the heat capacity of the BEC. The second chapter deals with magnetism in ultracold gases. When cooling an ultracold gas containing different spin components below the critical temperature for BEC, stable magnetic domains form. The appearance of these domains and the dynamics of the domain walls are studied. The spin mixture is prepared by performing an RF-sweep on ground state atoms in the presence of a magnetic field. Spin dynamics are induced by applying magnetic gradients. Spin drag, which is the transport coefficient responsible for damping spin currents, was measured in a two-component system. Furthermore a new method for spin resolved phase contrast imaging is presented, which is used to study time evolution in situ non-destructively. The last experiment focuses on spontaneous symmetry breaking. When passing a continuous phase transition, spontaneous symmetry breaking causes the development of domains with an independently chosen order parameter. The domains are separated by boundary defects. In this experiment the spontaneous creation of solitons was observed, which are boundary defects in the phase of the condensate, as well as magnetic domain walls, which are the boundary defects in the magnetization. Through the Kibble-Zurek mechanism it is possible to determine the critical exponents that characterize the phase transition. The critical exponents are predicted to be universal, i.e. do not depend on the microphysics of the system, so the results from our ultracold atoms lab can help answer universal questions for example from cosmology and from the early universe.
This thesis covers most of my work in the field of ultracold atoms loaded in optical lattices. It makes a route through the physics of cold atoms in periodic potentials starting from the simple noninteracting system and going into the many-body physics that describes the strongly correlated Mott insulator regime. Even though this thesis is a theoretical work all the chapters are linked either with experiments already done or with ongoing experimental efforts. This thesis can be divided into four different parts. The first part comprises chapters 1 to 3. In these chapters, after a brief introduction to the field of optical lattices I review the fundamental aspects pertaining to the physics of systems in periodic potentials. The second part deals with the superfluid weakly interacting regime where standard mean field techniques can be applied. This is covered in chapters 4 and 5. Specifically, chapter 4 introduces the discrete nonlinear Schroedinger equation (DNLSE) and uses it to model some experiments. In chapter 5 I go one step further and include the small quantum fluctuations neglected in the DNLSE by studying quadratic approximations of the Bose-Hubbard Hamiltonian. Chapters 6 to 8 can be grouped as the third part of the thesis. In them I adopt an effective action formalism, the so called two particle irreducible effective action (2PI) together with the closed time path (CTP) formalism to study far-from-equilibrium dynamics. The many-body techniques discussed in these chapters systematically include higher order quantum corrections, not included in the quadratic approximations of the Hamiltonian, which we show are crucial for a correct description of the quantum dynamics outside the very weakly interacting regime. Finally, chapter 9 to 11 are devoted to study the Mott insulator phase. In these chapters using perturbation theory I study the Mott insulator ground state and its excitation spectrum, the response of the system to Bragg spectroscopy, and propose a mechanism to correct for the residual quantum coherences inherent to the Mott insulator ground state. Even though small these are not ideal for the use of neutral atoms in optical lattice as a tool for quantum computation.