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EPJ Quantum Technology

Floquet analysis of coherence in periodically driven diamond nitrogen-vacancy ensemble systems

Cuong Manh Nguyen, Uijin Ko, Seong-Joo Lee, Hyeonsu Kim, Hosung Seo, Sangwon Oh

Published Sep 21, 2026• 0 citations
Publisher

Abstract

Abstract High-density nitrogen-vacancy (NV) ensembles are promising platforms for solid-state quantum sensing, but their performance is limited by dipolar interactions and inhomogeneous dephasing. Periodic decoupling sequences such as Waugh-Huber-Haeberlen (WAHUHA) can extend the observed stroboscopic decay time, but a longer fitted lifetime does not necessarily imply improved magnetic-field sensitivity. Here, we experimentally demonstrate this disconnect experimentally. WAHUHA increases the fitted stroboscopic decay time from $T_{2}^{*}$ T 2 ∗ of 0.9 μs to $T_{2,\mathit{eff}}^{*}$ T 2 , eff ∗ of 31 μs, while producing little improvement in dc magnetic-field sensitivity. Using detuning-resolved stroboscopic spectroscopy and finite-pulse Floquet analysis, we show that the long-lived signal arises from phase wrapping and quasienergy branch folding of the one-cycle unitary. These effects reshape the stroboscopic spectrum, and the experimentally relevant folded branches exhibit a reduced local detuning-to-phase transduction slope, $d\Phi /d\Delta $ d Φ / d Δ , which governs the dc magnetic-field response. Our results demonstrate that, under periodic driving, an extended effective dephasing time does not necessarily translate into enhanced dc sensitivity and establish finite pulse Floquet analysis as a practical framework for evaluating coherence in spin ensembles.

DOI
10.1140/epjqt/s40507-026-00571-2

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Abstract High-density nitrogen-vacancy (NV) ensembles are promising platforms for solid-state quantum sensing, but their performance is limited by dipolar interactions and inhomogeneous dephasing. Periodic decoupling sequences such as Waugh-Huber-Haeberlen (WAHUHA) can extend the observed stroboscopic decay time, but a longer fitted lifetime does not necessarily imply improved magnetic-field sensitivity. Here, we experimentally demonstrate this disconnect experimentally. WAHUHA increases the fitted stroboscopic decay time from T2∗T_{2}^{*}T2∗​ T 2 ∗ of 0.9 μs to T2,eff∗T_{2,\mathit{eff}}^{*}T2,eff∗​ T 2 , eff ∗ of 31 μs, while producing little improvement in dc magnetic-field sensitivity. Using detuning-resolved stroboscopic spectroscopy and finite-pulse Floquet analysis, we show that the long-lived signal arises from phase wrapping and quasienergy branch folding of the one-cycle unitary. These effects reshape the stroboscopic spectrum, and the experimentally relevant folded branches exhibit a reduced local detuning-to-phase transduction slope, dΦ/dΔd\Phi /d\Delta dΦ/dΔ d Φ / d Δ , which governs the dc magnetic-field response. Our results demonstrate that, under periodic driving, an extended effective dephasing time does not necessarily translate into enhanced dc sensitivity and establish finite pulse Floquet analysis as a practical framework for evaluating coherence in spin ensembles.
High-density nitrogen-vacancy (NV) ensembles are promising platforms for solid-state quantum sensing, but their performance is limited by dipolar interactions and inhomogeneous dephasing. Periodic decoupling sequences such as Waugh-Huber-Haeberlen (WAHUHA) can extend the observed stroboscopic decay time, but a longer fitted lifetime does not necessarily imply improved magnetic-field sensitivity. Here, we experimentally demonstrate this disconnect experimentally. WAHUHA increases the fitted stroboscopic decay time from T2∗T_{2}^*T2∗​ of 0.9 μμμs to T2,eff∗T_{2,eff}^*T2,eff∗​ of 31 μμμs, while producing little improvement in dc magnetic-field sensitivity. Using detuning-resolved stroboscopic spectroscopy and finite-pulse Floquet analysis, we show that the long-lived signal arises from phase wrapping and quasienergy branch folding of the one-cycle unitary. These effects reshape the stroboscopic spectrum, and the experimentally relevant folded branches exhibit a reduced local detuning-to-phase transduction slope, dΦ/dΔdΦ/dΔdΦ/dΔ, which governs the dc magnetic-field response. Our results demonstrate that, under periodic driving, an extended effective dephasing time does not necessarily translate into enhanced dc sensitivity and establish finite pulse Floquet analysis as a practical framework for evaluating coherence in spin ensembles.
In quantum science applications, ranging from many-body physics to quantum metrology, dipolar interactions in spin ensembles are controlled via Floquet engineering. However, this technique typically reduces the interaction strength between spins, and effectively weakens the coupling to a target sensing field, limiting the metrological sensitivity. In this work, we develop and demonstrate a method for direct tuning of the native interaction in an ensemble of nitrogen-vacancy (NV) centers in diamond. Our approach utilizes dressed-state qubit encoding under a magnetic field perpendicular to the crystal lattice orientation. This method leads to a 3.2×3.2\times3.2× enhancement of the dimensionless coherence parameter JT2JT_2JT2​ compared to state-of-the-art Floquet engineering, and a 2.6×2.6\times2.6× (8.3 8.3~8.3 dB) enhanced sensitivity in AC magnetometry. Utilizing the extended coherence we experimentally probe spin transport at intermediate to late times. Our results provide a powerful Hamiltonian engineering tool for future studies with NV ensembles and other interacting higher-spin (S>12S>\frac{1}{2}S>21​) systems.
Abstract Nitrogen-vacancy (NV) center ensembles in diamond are one of the most promising solid-state quantum platforms for various sensing applications. Achieving ultimate sensitivity requires simultaneously long spin dephasing times ( T2∗{T}_{2}^{* }T2∗​ T 2 * ) and high NV center concentrations. In this work, we propose a systematic measurement approach to quantify the electron spin dephasing in NV center ensembles and analyze the contributions of various sources to the dephasing time, including NV-NV interactions, strain and electric field distributions, 13 C nuclear spins, and P1 electron spins. Our method is validated using a series of high-performance diamond samples, providing a comprehensive understanding of dephasing mechanisms and revealing correlations between NV concentration and different dephasing sources. Building on these insights, we outline strategies to further enhance the achievable sensitivity for DC magnetic field measurements.
Abstract Negatively charged nitrogen-vacancy (NV − ) center ensembles in diamond have proved to have great potential for use in highly sensitive, small-package solid-state quantum sensors. One way to improve sensitivity is to produce a high-density NV − center ensemble on a large scale with a long coherence lifetime. In this work, the NV − center ensemble is prepared in type-Ib diamond using high energy electron irradiation and annealing, and the transverse relaxation time of the ensemble— T 2 —was systematically investigated as a function of the irradiation electron dose and annealing time. Dynamical decoupling sequences were used to characterize T 2 . To overcome the problem of low signal-to-noise ratio in T 2 measurement, a coupled strip lines waveguide was used to synchronously manipulate NV − centers along three directions to improve fluorescence signal contrast. Finally, NV − center ensembles with a high concentration of roughly 10 15 mm −3 were manipulated within a ~10 µ s coherence time. By applying a multi-coupled strip-lines waveguide to improve the effective volume of the diamond, a sub-femtotesla sensitivity for AC field magnetometry can be achieved. The long-coherence high-density large-scale NV − center ensemble in diamond means that types of room-temperature micro-sized solid-state quantum sensors with ultra-high sensitivity can be further developed in the near future.
In this work, we optimize a dynamical decoupling (DD) protocol to improve the spin coherence properties of a dense ensemble of nitrogen-vacancy (NV) centers in diamond. Using liquid nitrogen-based cooling and DD microwave pulses, we increase the transverse coherence time T2 from ∼ 0.7 ms up to ∼ 30 ms. We extend previous work of single-axis (Carr-Purcell-Meiboom-Gill) DD towards the preservation of arbitrary spin states. After performing a detailed analysis of pulse and detuning errors, we compare the performance of various DD protocols. We identify that the concatenated XY8 pulse sequences serves as the optimal control scheme for preserving an arbitrary spin state. Finally, we use the concatenated sequences to demonstrate an immediate improvement of the AC magnetic sensitivity up to a factor of two at 250 kHz. For future work, similar protocols may be used to increase coherence times up to NV-NV interaction time scales, a major step toward the creation of quantum collective NV spin states.
Diamond-based quantum magnetometers are more sensitive to oscillating (ac) magnetic fields than static (dc) fields because the crystal impurity-induced ensemble dephasing time T2∗{T}_{2}^{*}T2∗​, the relevant sensing time for a dc field, is much shorter than the spin coherence time T2{T}_{2}T2​, which determines the sensitivity to ac fields. Here we demonstrate measurement of dc magnetic fields using a physically rotating ensemble of nitrogen-vacancy centers at a precision ultimately limited by T2{T}_{2}T2​ rather than T2∗{T}_{2}^{*}T2∗​. The rotation period of the diamond is comparable to T2{T}_{2}T2​ and the angle between the nitrogen-vacancy (NV) axis and the target magnetic field changes as a function of time, thus upconverting the static magnetic field to an oscillating field in the physically rotating frame. Using spin-echo interferometry of the rotating NV centers, we are able to perform measurements for over 100 times longer compared to a conventional Ramsey experiment. With modifications our scheme could realize dc sensitivities equivalent to demonstrated NV center ac magnetic field sensitivities of order $0.1\phantom{\rule{0.28em}{0ex}}\mathrm{nT}\phantom{\rule{0.16em}{0ex}}{\mathrm{Hz}}^{\ensuremath{-}1/2}$.