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Interface between picosecond and nanosecond quantum light pulses

Ali Golestani, Michał Mikołajczyk, Filip Sośnicki

Published Jan 1, 2023• 0 citations
OpenAlex

Abstract

Light is a key information carrier, enabling worldwide, high-speed data transmission through a telecommunication fibre network. This information-carrying capacity can be extended to transmitting quantum information (QI) by encoding it in single photons—flying qubits. However, the various QI-processing platforms operate at vastly different timescales. QI-processing units in atomic media, operating within nanosecond to microsecond timescales, and high-speed quantum communication, at picosecond timescales, cannot be linked efficiently because of the orders-of-magnitude mismatch in the timescales or, correspondingly, spectral linewidths. Here we develop a large-aperture time lens using wide-bandwidth electro-optic phase modulation to bridge this gap. We demonstrate coherent, deterministic spectral bandwidth compression of quantum light pulses by more than two orders of magnitude with high efficiency. This will facilitate large-scale hybrid QI-processing by linking the ultrafast and quasi-continuous-wave experimental platforms, which until now, to a large extent, have been developing independently. To bridge the ultrafast and slow classes of quantum-information-processing systems, a Fresnel time lens is developed by using a wideband electro-optic phase modulator combined with a dispersion element. The single-photon spectral bandwidth is compressed from picosecond to nanosecond timescales.

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Light is a key information carrier, enabling worldwide, high-speed data transmission through a telecommunication fibre network. This information-carrying capacity can be extended to transmitting quantum information (QI) by encoding it in single photons—flying qubits. However, the various QI-processing platforms operate at vastly different timescales. QI-processing units in atomic media, operating within nanosecond to microsecond timescales, and high-speed quantum communication, at picosecond timescales, cannot be linked efficiently because of the orders-of-magnitude mismatch in the timescales or, correspondingly, spectral linewidths. Here we develop a large-aperture time lens using wide-bandwidth electro-optic phase modulation to bridge this gap. We demonstrate coherent, deterministic spectral bandwidth compression of quantum light pulses by more than two orders of magnitude with high efficiency. This will facilitate large-scale hybrid QI-processing by linking the ultrafast and quasi-continuous-wave experimental platforms, which until now, to a large extent, have been developing independently. To bridge the ultrafast and slow classes of quantum-information-processing systems, a Fresnel time lens is developed by using a wideband electro-optic phase modulator combined with a dispersion element. The single-photon spectral bandwidth is compressed from picosecond to nanosecond timescales.
Spectral-temporal manipulation of optical pulses has enabled numerous developments within a broad range of research topics, ranging from fundamental science to practical applications. Within quantum optics spectral-temporal degree of freedom of light offers a promising platform for integrated photonic quantum information processing. An important challenge in experimentally realizing spectral-temporal manipulation of quantum states of light is the need for highly efficient manipulation tools. In this context the intrinsically deterministic electro-optic methods show great promise for quantum applications. We experimentally demonstrate application of electro-optic platform for spectral-temporal manipulation of ultrashort pulsed quantum light. Using techniques analogous to serrodyne frequency shifting we show active spectral translation of few-picosecond single photon pulses by up to 0.5 THz. By employing an approach based on an electro-optic time lens we demonstrate up to 6-fold spectral compression of heralded single photon pulses with efficiency that enables us to significantly increase single photon flux through a narrow bandpass filter. We realize the required temporal phase manipulation by driving a lithium niobate waveguided electrooptic modulator with 33 dBm sinusoidal RF field at the frequency of either 10 GHz or 40 GHz. We use a phase lock loop to temporally lock the RF field to the 80 MHz repetition rate of approximately 1 ps long optical pulses. Heralded single photon wavepackets are generated by means of spontaneous parametric down-conversion in potassium dihydrogen phosphate (KDP) crystal, which enables preparation of spectrally pure single photon wavepackets without the need for spectral filtering. Spectral shifting is achieved by locking single-photon pulses to the linear slope of sinusoidal 40 GHz RF phase modulation. We verify the spectral shift by performing spectrally resolved heralded single photon counting, using frequency-to-time conversion by means of a highly dispersive chirped fiber Bragg grating. We verify the non-classicality of spectrally shifted single photons by measuring high-visibility Hong-Ou-Mandel interference using a reference single photon pulse. Spectral compression is based on the time lens principle, which requires locking optical pulses to approximately quadratic region of sinusoidal phase modulation. We utilize both 10 GHz and 40 GHz RF driving frequencies. Bandwidth compression is achieved by chirping the single photon pulse using an appropriate length of single-mode fibre and subsequently subjecting it to the action of the time lens. We verify spectral compression directly using the aforementioned spectrally-resolved heralded single photon counting method. We achieve 3-fold spectral compression of 2 nm bandwidth single photon pulses using 40 GHZ modulation frequency, and 6-fold spectral compression of 0.9 nm bandwidth single photon pulses using 10 GHz modulation frequency. Overall transmission of our set-up exceeding 30% enables practical usability of our spectral compression method which we demonstrate experimentally by showing an increased photon flux through a narrowband filter. Our results present an important contribution towards implementing quantum information processing in the spectral-temporal degree of freedom of a photon. In the context of quantum networks they present an enabling tool towards efficient photonic interfacing of different quantum information processing platforms.
Spectral-temporal shaping of quantum light has important applications in quantum communications and photonic quantum information processing. Electro-optic temporal lenses have recently been recognized as a tool for noise-free, efficient spectral bandwidth manipulation of single-photon wavepackets. However, standard electro-optic time lenses based on single-tone modulation exhibit, limited bandwidth modification factors due to material limitations on phase modulation amplitude. Here we numerically investigate the use of complex electro-optic temporal phase modulation patterns for bandwidth compression of light over multiple orders of magnitude and show the feasibility of their use in photonic interfaces for quantum network applications.
A promising approach towards implementation of large-scale quantum information and communication protocols is a multifunctional photonic quantum information processing system, where a variety of distributed components, such as quantum memories, trapped ions, or photonic quantum gates are coherently interconnected via photonic links. These components may exhibit a vast range of spectro-temporal properties. A key incompatibility is spectral bandwidth mismatch. For example the characteristic bandwidths of photonic communication channels and nonlinear-optical single-photon sources are in the 100 GHz range, whereas typical bandwidths associated with trapped ions or media exhibiting strong single photon nonlinearity, such as Rydberg atoms, are in the sub-GHz regime, reaching single MHz values. Single-photon-level bandwidth conversion has been experimentally demonstrated by techniques based on the temporal lensing principle, but only between multi-GHz bandwidth optical pulses [1, 2]. Here we present a numerical study of an electro-optic time-lens-based technique enabling bandwidth conversion from the 100 GHz bandwidth region towards single MHz bandwidths. We discuss progress towards experimental implementation and possible realizations using alternative temporal lensing platforms, such as three and four wave mixing.
A promising approach to realize a quantum internet [1] is to use a hybrid quantum network - a network composed of many different quantum devices, such as quantum emitters, quantum repeaters, or quantum gates, interconnected via photonic links. However, such a wide variety of quantum devices tends to be spectrally incompatible. Especially, the challenge arises to interface different single-photon spectral bandwidths with high efficiency. In particular, an important link is bridging the ultrafast optics with hundreds of GHz spectral bandwidths with nanosecond timescales of single-photon pulses, hence MHz-wide spectra. Such an interface corresponds, e.g., to coupling a single photon produced in a commonly used bulk spontaneous parametric down-conversion (SPDC) photon sources to atomic-based quantum memories. The already demonstrated spectral compression techniques, based mostly on optical nonlinearities, operate only in the above GHz regime and are not suitable for this task [2].
We experimentally demonstrate spectral manipulation of heralded single photons by electro-optic temporal phase modulation employing complex, Fresnel-like wide-band electronic waveforms. We show spectral compression of classical telecom light enhancing its maximal intensity by over 80, by compressing its full-width at half maximum (FWHM) bandwidth from 0.856 nm down to 3.1 pm (383 MHz), thus achieving a compression factor of over 270. We show a compression gain by increasing the aperture of a Fresnel time lens (temporal waveform duration). We demonstrate a similar compression on a single-photon level from ~1.5 nm (~190 GHz) down to the sub-2GHz regime. Our findings should significantly improve the performance of future quantum information processors based on hybrid quantum networks.
Manipulating the frequency and bandwidth of nonclassical light is essential for implementing frequency-encoded/multiplexed quantum computation, communication, and networking protocols, and for bridging spectral mismatch among various quantum systems. However, quantum spectral control requires a strong nonlinearity mediated by light, microwave, or acoustics, which is challenging to realize with high efficiency, low noise, and on an integrated chip. Here, we demonstrate both frequency shifting and bandwidth compression of heralded single-photon pulses using an integrated thin-film lithium niobate (TFLN) phase modulator. We achieve record-high electro-optic frequency shearing of telecom single photons over terahertz range (±641 GHz or ±5.2 nm), enabling high visibility quantum interference between frequency-nondegenerate photon pairs. We further operate the modulator as a time lens and demonstrate over eighteen-fold (6.55 nm to 0.35 nm) bandwidth compression of single photons. Our results showcase the viability and promise of on-chip quantum spectral control for scalable photonic quantum information processing.