Light-matter Interactions for Memory-assisted Microwave-to-Optical Transducers
Ujjwal Gautam
Abstract
Quantum technologies harness superposition and entanglement for computation, communication, and sensing. Superconducting quantum circuits (SQCs) are promising for scalable quantum information processing, but networking distant SQC nodes is challenging: microwave photons suffer severe thermal noise and loss at room temperature, while optical photons travel through fiber with negligible loss. A quantum transducer bridges this gap by converting microwave photons to optical photons with minimal added noise. This thesis presents a memory-assisted microwave-to-optical (M2O) transducer using an ensemble of Yb-ions doped in Y2SiO5 (YSO). Yb:YSO offers zero-first-order Zeeman (ZEFOZ) transitions at zero field, giving long coherence times, and GHz-range hyperfine splittings that interface directly with SQCs without an external magnetic field. The platform integrates a custom loop-gap resonator (LGR) with a free-space optical setup at 30 mK in a dilution refrigerator. The LGR, designed via CAD and COMSOL simulation and machined from oxygen-free copper, concentrates the microwave field for strong coupling to the spin ensemble. A Python-based automation framework synchronizes instrumentation for high-throughput acquisition of pulse sequences. Coherence is characterized via optical excited-state lifetime, spin population time, and optical coherence time. Optically detected magnetic resonance reveals coherent microwave-spin dynamics, including Rabi oscillations with collapse-and-revival features from spin inhomogeneity and cavity photon-number statistics. Continuous-wave M2O transduction at 2623 MHz achieves an internal efficiency of 2e-8 over 200 kHz bandwidth. Avoided-crossing measurements confirm strong spin-microwave coupling, with cooperativity exceeding unity. A theoretical framework links efficiency to microwave, optical, and atomic cooperativities, projecting ~1e-4 efficiency through improved doping, beam diameter, detuning, and cavity integration. A memory-assisted M2O protocol integrates quantum storage via rapid adiabatic passage phase imprinting, enabling on-demand retrieval separated from the pump and suppressing pump noise without lossy filtering. At 460 μs storage, this achieves 4e-8 efficiency with 0.4 noise photons, among the lowest noise figures reported for M2O transducers. Interference measurements confirm coherent information transfer, and multiplexing of up to ten transduced modes is demonstrated, exploiting Yb:YSO's broad inhomogeneous linewidths. This work, the first memory-assisted M2O interface, enables photon synchronization for path-erasure entanglement between remote SQCs, advancing scalable quantum repeaters and distributed quantum computing.