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Nano Letters

Entangled Telecom Photons Generation Using Twisted van der Waals Crystals

Nidhin Prasannan, Konstantinos Mourzidis, Vishwas Jindal, Hanting Li, Di Lin, Wenchen Yang, Deng Hu, Liu Yang, A. Balocchi, Delphine Lagarde, P. Renucci, Zhiwei Wang, Gang Wang, X. Marie

Published Aug 18, 2026• 0 citations
Publisher

Abstract

Nanoscale quantum light sources are essential building blocks for integrated quantum photonic systems. Here, we report a wavelength-scale entangled-photon source based on van der Waals-engineered NbOBr2 and benchmark its performance for telecom-wavelength quantum light generation. By exploiting the material's second-order nonlinearity, we generate quantum-correlated photon pairs via spontaneous parametric down-conversion. We then use a 90° twisted stacking to induce quantum interference in photon-pair generation, yielding polarization-entangled photons. This approach enables tunability of the quantum optical state via control of the excitation laser polarization. We experimentally obtain entanglement fidelities exceeding 95% for Bell states, along with a high coincidence-to-accidental ratio of ∼335 and a brightness approximately 1 order of magnitude higher than recently reported telecom sources based on transition metal dichalcogenide two-dimensional materials. These results establish twisted van der Waals engineering as a powerful platform for highly tunable, high-brightness quantum light sources at telecom wavelengths.

DOI
10.1021/acs.nanolett.6c02461

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Nanoscale quantum light sources are essential building blocks for integrated quantum photonic systems. Here, we report a wavelength-scale entangled-photon source based on van der Waals-engineered NbOBr2 and benchmark its performance for telecom-wavelength quantum light generation. By exploiting the material's second-order nonlinearity, we generate quantum-correlated photon pairs via spontaneous parametric down-conversion. We then use a 90° twisted stacking to induce quantum interference in photon-pair generation, yielding polarization-entangled photons. This approach enables tunability of the quantum optical state via control of the excitation laser polarization. We experimentally obtain entanglement fidelities exceeding 95% for Bell states, along with a high coincidence-to-accidental ratio of ∼335 and a brightness approximately 1 order of magnitude higher than recently reported telecom sources based on transition metal dichalcogenide two-dimensional materials. These results establish twisted van der Waals engineering as a powerful platform for highly tunable, high-brightness quantum light sources at telecom wavelengths.
Nanoscale quantum light sources are essential building blocks for integrated quantum photonic systems. Here, we report a wavelength-scale entangled-photon source based on van der Waals-engineered NbOBr2_22​, and benchmark its performance for telecom-wavelength quantum light generation. By exploiting the material's second-order nonlinearity, we generate quantum-correlated photon pairs via spontaneous parametric down-conversion. We then use a 90∘^{\circ}∘ twisted stacking to induce quantum interference in photon-pair generation, yielding polarization-entangled photons. This approach enables tunability of the quantum optical state via control of the excitation laser polarization. We experimentally obtain entanglement fidelities exceeding 95% for Bell states, along with a high coincidence-to-accidental ratio of $\sim$335, and a brightness approximately one order of magnitude higher than recently reported telecom sources based on transition metal dichalcogenide (TMD) 2D materials. These results establish twisted van der Waals engineering as a powerful platform for highly tunable, high-brightness quantum light sources at telecom wavelengths.
We present a tunable, single-mode-optical-fiber-based source of polarization entangled photon pairs for the near-infrared telecommunication band that is deployable in standard infrastructure. The photon pairs are generated via spontaneous parametric down-conversion (SPDC) in a submicron-scale thin film of the inversion-broken rhombohedral polytype of the transition metal dichalcogenide molybdenum disulfide (3R-MoS2_22​), located between two fiber connectors. By exploiting the intrinsic symmetries of the second-order nonlinear susceptibility tensor of 3R-MoS2_22​, this hybrid approach offers control over the generated two-photon polarization state through the incident pump polarization. Most notably, two of the four maximally entangled Bell states, as well as fully co-polarized pairs can be produced. This represents a substantial improvement in terms of tunability and simplicity over established fiber-integrated sources, which require additional optical elements, precise alignment, or careful engineering of design parameters. Additionally, a nonlinear drop in the background photoluminescence signal of 3R-MoS2_22​ is observed at low pump powers, allowing us to reach a coincidences-to-accidentals ratio (CAR) of (8.3±1.8)×103(8.3\pm1.8)\times10^{3}(8.3±1.8)×103, the highest value recorded for SPDC in van der Waals materials to date.
Abstract Ultracompact entangled photon sources are pivotal to miniaturized quantum photonic devices. Van der Waals (vdW) nonlinear crystals promise efficient photon-pair generation and on-chip monolithic integration with nanophotonic circuitry. However, it remains challenging to generate maximally entangled Bell states of photon pairs with high purity, generation rate, and fidelity required for practical applications. Here, we realize a polarization-entangled photon-pair source based on spontaneous parametric down conversion in an ultrathin rhombohedral tungsten disulfide (3R-WS 2 ) crystal. This vdW entangled photonic source exhibits a high photon-pair purity with a coincidence-to-accidental ratio of above 800, a generation rate of 31 Hz, and two maximally polarization-entangled Bell states with fidelities exceeding 0.93 and entanglement degree over 0.97. These results stem from scalable optical nonlinearity, enhanced second-order susceptibility by electronic transitions, and a well-defined symmetry-enabled selection rule inherent in 3R-WS 2 . Our polarization entangled photon source can be integrated with photonic structures for generating more complex entangled states, thus paving an avenue for advanced quantum photonic systems toward computation and metrology.
Polarization-entangled photon pairs are essential resources for quantum information technologies, yet realizing compact sources with intrinsically controllable entanglement remains challenging. Van der Waals (vdW) nonlinear materials such as NbOCl2 provide atomically thin platforms for quantum light generation, yet their native crystalline anisotropies as natural materials impose limitations on accessible quantum states. Here, we develop a resonant vdW nonlinear metasurface based on NbOCl2 that exploits its intrinsic optical anisotropy to engineer polarization-dependent nonlinear responses. The anisotropic optical dispersion enables selective manipulation of resonant modes, resulting in a three-order-of-magnitude enhancement of the nonlinear response along the c axis. By further tailoring these resonant modes, we redistribute the effective second-order nonlinear susceptibility tensor between orthogonal polarization channels, balancing the spontaneous parametric down-conversion pathways along the b and c axes. This enables polarization-entangled photon generation with a measured fidelity of up to 92%. Our work establishes metasurface-enabled nonlinear optical engineering as a strategy for enhancing and controlling quantum light generation in vdW materials, providing a pathway toward scalable quantum photonic platforms.
Bright entangled photon sources with on-demand quantum state control are essential for advancing quantum science and technologies. However, simultaneously achieving high brightness and state tunability remains challenging, as this necessitates a dual-phase control mechanism that facilitates both longitudinal phase matching and transverse polarization modulation. Here, we report a twin-twisted two-dimensional (2D) van der Waals (vdW) crystal architecture that enables spontaneous parametric down-conversion (SPDC) with both high generation efficiency and continuously tunable quantum states. The designed crystal comprises two sections of twisted 2D GaSe vdW flakes with opposite chiral handedness, in which interflake twist angle induces phase matching in SPDC, and intersection twisting provides an additional degree of freedom on tunability. We demonstrate that the twin-twisted GaSe crystals achieve a record-high photon-pair generation rate exceeding 13 200 Hz and a Bell state fidelity above 99% within 2D material family, and enable unprecedented tunability of quantum states from the maximally polarization entangled states to the fully separable states. This study opens a practical avenue toward twist-engineered quantum states, and paves the way for developing compact quantum photonic systems with tailored properties.
Entangled photon pairs play a major role in various modern technologies such as quantum imaging, communication, and computing. Conventional photon-pair sources are often based on spontaneous parametric down-conversion in bulk nonlinear crystals. Recent advances have also shown entangled photon-pairs from transition metal dichalcogenide thin-films, however, these materials are not widely available and are not compatible with existing fabrication capabilities. We present a new thin-film lithium niobate source of polarization-entangled photon pairs at the telecom wavelength that requires no additional optical elements for entanglement generation and allows for easy application using the existing lithium niobate fabrication technologies. We demonstrate tunable entanglement generation using the three-fold rotational crystal symmetry of lithium niobate, allowing the generation of different maximally entangled Bell states or completely separable states depending on the polarization of the pump beam.