Ultracold neutral plasmas (UNPs), which are formed by photoionizing a cloud of cold atoms, have been a powerful platform for studying a wide variety of plasma phenomena. Two areas of interest include expansion into vacuum and the development of shockwaves. Previous UNP experiments have used plasmas with an initial Gaussian density distribution. UNPs with a radially exponentially decaying density distribution, or exponential UNPs, can be formed by photoionizing atoms out of a purely magnetic trap. This dissertation studies the expansion in free space of exponential UNPs as well as the development and characterization of shockwaves in exponential UNPs. The free space expansion of an exponential UNP is compared to the well-known self-similar hydrodynamic expansion of a Gaussian plasma. Similar scaling laws describe the size evolution well for both cases. The evolution of the plasma size and velocity show a characteristic ion acoustic time scale, indicating that the plasma is generally well-described by a hydrodynamic description. While the exponential UNP is predominantly in the hydrodynamic regime, heating at the central peak for low-density, high-electron temperature suggests significant local non-neutrality at early times. This thesis presents the first observation of a shockwave in a UNP. The evolution of the density and velocity for exponential UNPs show signs of wave steepening. A significant density and velocity jump over a narrow region develops. These occur at the same location in the plasma. Additionally, a large spike in the ion temperature occurs at this front. The relative ion velocity across the front modestly surpasses the local sound speed. The initial conditions were varied to characterize the development of shockwaves. Varying the density and electron temperature did not impact shock formation for the ranges used. Changing the shape caused the shocks to disappear as the density gradient decreased. This suggests that the electron thermal pressure gradient plays a significant role in the shock formation. The establishment of shock formation in UNPs opens a new avenue of research for UNPs.
Ultracold neutral plasmas (UNPs), which are formed by photoionizing a cloud of cold atoms, have been a powerful platform for studying a wide variety of plasma phenomena. Two areas of interest include expansion into vacuum and the development of shockwaves. Previous UNP experiments have used plasmas with an initial Gaussian density distribution. UNPs with a radially exponentially decaying density distribution, or exponential UNPs, can be formed by photoionizing atoms out of a purely magnetic trap. This dissertation studies the expansion in free space of exponential UNPs as well as the development and characterization of shockwaves in exponential UNPs. The free space expansion of an exponential UNP is compared to the well-known self-similar hydrodynamic expansion of a Gaussian plasma. Similar scaling laws describe the size evolution well for both cases. The evolution of the plasma size and velocity show a characteristic ion acoustic time scale, indicating that the plasma is generally well-described by a hydrodynamic description. While the exponential UNP is predominantly in the hydrodynamic regime, heating at the central peak for low-density, high-electron temperature suggests significant local non-neutrality at early times. This thesis presents the first observation of a shockwave in a UNP. The evolution of the density and velocity for exponential UNPs show signs of wave steepening. A significant density and velocity jump over a narrow region develops. These occur at the same location in the plasma. Additionally, a large spike in the ion temperature occurs at this front. The relative ion velocity across the front modestly surpasses the local sound speed. The initial conditions were varied to characterize the development of shockwaves. Varying the density and electron temperature did not impact shock formation for the ranges used. Changing the shape caused the shocks to disappear as the density gradient decreased. This suggests that the electron thermal pressure gradient plays a significant role in the shock formation. The establishment of shock formation in UNPs opens a new avenue of research for UNPs.
We present observations of wave steepening and signatures of shock formation during expansion of ultracold neutral plasmas formed with an initial density distribution that is centrally peaked and decays exponentially with distance. The plasma acceleration and velocity decrease at large distance from the plasma center, leading to central ions overtaking ions in the outer regions and the development of a steepening front that is narrow compared to the size of the plasma. The density and velocity change dramatically across the front, and significant heating of the ions is observed in the region of steepest gradients. For a reasonable estimate of electron temperature, the relative velocity of ions on either side of the front modestly exceeds the local sound speed (Mach number M≳1). This indicates that by sculpting steep density gradients, it is possible to create the conditions for shock formation, or very close to it, opening a new avenue of research for ultracold neutral plasmas.
We present a study of the expansion of an ultracold neutral plasma (UCNP) with an initial density distribution that decays exponentially in space, created by photoionizing atoms shortly after their release from a quadrupole (or biconic cusp) magnetic trap. A characteristic ion acoustic timescale is evident in the evolution of the plasma size and velocity, indicating that the dynamics are reasonably well described by a model of hydrodynamic expansion of a quasi-neutral plasma. However, for low plasma density and high initial electron temperature, excess ion kinetic energy in the vicinity of the central density peak suggests significant local non-neutrality at early times. Observations are compared to the well-understood self-similar expansion of a UCNP with an initial Gaussian density distribution, and a similar scaling law describes the evolution of plasma size for both cases.
This thesis describes the measurements of collective effects in strongly coupled ultra-cold neutral plasmas (UNPs). It shows the implementation of experimental techniques that perturb either the density or velocity distribution of the plasma and it describes the subsequent excitation, observation and analysis of the aforementioned collective phenomena. UNPs are interesting in that they display physics of strongly coupled systems. For most plasma systems, collective effects are well described with classical hydrodynamic or kinetic descriptions. However, for strongly coupled systems, the Coulomb interaction energy between nearest neighbors exceeds the kinetic energy, and these descriptions must be modified as the plasma crosses over from a gas-like to liquid-like behavior. Strongly coupling can be found in exotic plasma systems found astrophysics, dusty plasmas, non-neutral trapped ion plasmas, intense-laser/matter interactions and inertial confinement fusion experiments. Compared to other strongly coupled plasmas, UNPs are ideal for studying collective effects in this regime since they have lower timescales, precisely controllable initial conditions and non-invasive diagnostics. Previous studies of UNPs concentrated on plasma expansion dynamics and some collective effects such as disorder induced heating, but little work had been done in relaxation or collision rates and collective modes in UNPs. This thesis presents a method for measuring collision rates by perturbing the velocity distribution of the plasma, observing plasma relaxation and measuring the relaxation rate. It also presents a new technique for observing collective modes in the plasma by perturbing the initial density of the plasma and how this results in the excitation of ion acoustic waves and a measurement of its dispersion relation. Finally, this thesis presents how this last technique can be used to create a gap in the center of the plasma and how this leads to hole propagation and plasma streaming and presents a characterization of both phenomena. The result of these experiments will be valuable for predicting the behavior of collective effects in other strongly coupled plasmas and for comparison with theories that describe them.
This work describes the evolution of an ultracold neutral plasma as it expands freely in vacuum. It presents a comprehensive study of the electron temperature evolution under different initial conditions. Ultracold neutral plasmas are created by photoionizing laser-cooled neutral atoms in ultrahigh vacuum. The ions are typically at a temperature of ∼ 1K while the electron temperature can be set from 1--1000 K. After photoionization, some of the highly energetic electrons escape from the cloud, leaving a net positive charge in the cloud. This creates a Coulomb well which traps the rest of the electrons, and a plasma is formed. Since the electrons have a lot of kinetic energy, they tend to leave the cloud, however, the Coulomb force from the ion pulls the electrons back into the cloud. This exerts a recoil force on the ions, and the whole plasma starts expanding radially outwards. Since the expansion is caused by the thermal pressure of the electrons, a study of the plasma expansion unravels the complicated electron temperature evolution, under different initial conditions. Many collisional processes become significant as a plasma expands. These physical processes tend to heat or cool the ions and electrons, leading to very different kinds of evolution depending on the initial conditions of the plasma. This work demonstrates three different regions of parameter space where the degree of significance of these physical processes is different during the ultracold neutral plasma evolution. The experimental results are verified by theoretical simulations, performed by Thomas Pohl, which untangle the complicated electron temperature evolution.
Ultracold neutral plasmas (UNPs) are created in a vacuum by photoionizing laser-cooled atoms. The expansion of UNPs begins as a non-equilibrium system that quickly relaxes to a local equilibrium state [1] . We aim to quantify and compare the transport processes that govern the relaxation to equilibrium in the expanding UNP. Using a 1D-1V kinetic code in spherical coordinates, we model the radial expansion of an UNP. We compare our simulation results against analytic expressions to determine where the expansion of the UNP is adiabatic or isothermal. We carry out simulations for various initial density distributions such as an exponentially decaying density distribution [2] . We ultimately aim to extend this approach to a 1D-3V multi-component kinetic code that incudes collisions [3] .
Ultracold neutral plasmas (UNPs) are highly correlated, charged-particle systems studied in standard atomic-molecular optical physics laboratories. Advances in ultracold physics techniques have led to the development of magneto-optical traps that permit the localization of micro-Kelvin temperature atomic samples (10⁸ - 10¹⁰ cm -³ that can be photoionized with a defined excess laser energy. Magneto-optical trapping of molecules proves difficult, and to date, lags in reaching conditions attainable for atoms. Molecules possess additional degrees of freedom where energy can flow during laser trapping and cooling. Alternatively, elastic collisions with inert gases offer another route to low temperatures. Super-sonic expansions of target molecules seeded in a noble gas can reduced the translational temperature to values as low as 0.1 K. Here I report on the formation of a molecular ultracold plasma in a molecular beam of nitric oxide seeded in an inert gas. Our method does not directly form a plasma, but instead, I create a Rydberg gas that spontaneously evolves to a plasma. I have verified the transition to a collective plasma state by applying pulsed-fields to the field-free flight region, and observe a signal that persists well beyond classical field amplitudes required to ionize individual Rydberg states. Electric field screening is a collective effect occurring over a characteristic distance, quantified by the Debye length, λ_D. Molecular ultracold plasmas described here exhibit Debye lengths smaller than the overall size, λ_D<<σ. Plasmas of this nature offer an exotic environment for which to study fundamental phenomena. While plasmas are generally thought of as hot, UNPs exist at low enough temperatures that electrostatic interaction energy between particles is greater than their kinetic energy. At this point, charged particles begin to find themselves in local potential energy minima. Over the entire sample this translates to long-range order, or correlation. It is of great interest for researchers studying UNPs to maximize particle correlation, which requires UNPs to remain very cold, and dense through their lifetime.