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Microwave Transitions and Synthetic Dimensions in Rydberg Atoms

Yi Lu

Published Mar 5, 2025• 0 citations
OpenAlex

Abstract

The marriage between Rydberg physics and ultracold atomic systems have hatched so many fascinating achievements. The exaggerated properties of Rydberg states, combined with the pristine environments provided by the ultracold atoms, can lead to realizations of exotic physical systems. One particularly innovative direction that emerged recently is to use microwave-frequency transitions between Rydberg levels to simulate the dynamics of a particle hopping between lattice sites. Such approach, referred to as Rydberg synthetic dimensions, falls under the broad scheme of quantum simulations. Here we present description of the infrastructure used for Rydberg excitation and coherent microwave transitions, which are essential to the realization of Rydberg synthetic dimensions. We will also present experimental results on simulating the Su-Schireffer-Heeger Hamiltonian, a canonical model with paradigmatic importance in topological physics.

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Rydberg-atom synthetic dimensions in the form of a lattice of $n^{3}S_{1}$ levels, $58\ensuremath{\le}n\ensuremath{\le}63$, coupled through two-photon microwave excitation are used to examine dynamics within the single-particle Su-Schrieffer-Heeger Hamiltonian. This paradigmatic model of topological matter describes a particle hopping on a one-dimensional lattice with staggered hopping rates. Tunneling rates between lattice sites and on-site potentials are set by the microwave amplitudes and detuning, respectively. An atom is first excited to a Rydberg state that lies within the lattice and then subject to the microwave dressing fields. After some time, the dressing fields are turned off and the evolution of the population distribution in the different final lattice sites monitored using field ionization. The measurements show the existence of long-lived symmetry-protected edge states and reveal the existence of direct long-distance tunneling between the edge states. The results are in good agreement with model calculations and further demonstrate the potential of Rydberg-atom synthetic dimensions to simulate and faithfully reproduce complex Hamiltonians.

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Synthetic dimensions are powerful tools for quantum simulation and computation. They are realized by harnessing internal or external degrees of freedom of an atom or molecule, which can mimic the motion of an electron in a real-space lattice potential. Such degrees of freedom are highly tunable and can be engineered to create configurations difficult to access or realize in real space. Some of the exciting possibilities include realizing higher dimensions systems[1, 2, 3], nontrivial real space[4, 5] and band structure[6, 7] topologies and artificial gauge fields[8, 9]. Experiments have utilized various degrees of freedom to create synthetic dimensions, such as motional[10, 11], spin[8, 12, 13, 14] and rotational[15] levels of atoms and molecules, and frequency modes, spatial modes, and arrival times in photonic systems[16]. Atomic synthetic dimensions have demonstrated artificial gauge fields, spin-orbit coupling, chiral edge states using Raman-coupled ground magnetic sublevels[8, 12, 17] of atoms, and phenomena such as Anderson localization using two-photon Bragg transitions by coupling free-particle momentum states[18]. Here, we harness the Rydberg levels of 84Sr to realize a synthetic lattice for studying quantum matter. Resonant millimeter-wave (mm-wave) radiation coupling Rydberg levels |i⟩ and |j⟩ with amplitude Ωij (Rabi frequency) are described by the same Hamiltonian as a particle tunneling between lattice sites |i⟩ and |j⟩ with tunneling amplitude Jij = Ωij /2. The mathematical equivalence to particles moving in a real-space lattice enables Rydberg levels to function as a synthetic spatial dimension. Rydberg-atom synthetic dimensions offer control over connectivity, tunneling rates and on-site potentials, which allows for the creation of a broad range of synthetic dimensional system. The capabilities of such a system are demonstrated by realizing the famous Su-Schrieffer-Heeger (SSH) model[19] and studying its topologically protected edge states(TPS).

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Rydberg-atom synthetic dimensions in the form of a lattice of n$^3S_1$ levels, $58\leq n \leq 63$, coupled through two-photon microwave excitation are used to examine dynamics within the single-particle Su-Schrieffer-Heeger (SSH) Hamiltonian. This paradigmatic model of topological matter describes a particle hopping on a one-dimensional lattice with staggered hopping rates. Tunneling rates between lattice sites and on-site potentials are set by the microwave amplitudes and detuning, respectively. An atom is first excited to a Rydberg state that lies within the lattice and then subject to the microwave dressing fields. After some time, the dressing fields are turned off and the evolution of the population distribution in the different final lattice sites monitored using field ionization. The measurements show the existence of long-lived symmetry-protected edge states and reveal the existence of direct long-distance tunneling between the edge states. The results are in good agreement with model calculations and further demonstrate the potential of Rydberg-atom synthetic dimensions to simulate and faithfully reproduce complex Hamiltonians.

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Abstract A discrete degree of freedom can be engineered to match the Hamiltonian of particles moving in a real-space lattice potential. Such synthetic dimensions are powerful tools for quantum simulation because of the control they offer and the ability to create configurations difficult to access in real space. Here, in an ultracold 84 Sr atom, we demonstrate a synthetic-dimension based on Rydberg levels coupled with millimeter waves. Tunneling amplitudes between synthetic lattice sites and on-site potentials are set by the millimeter-wave amplitudes and detunings respectively. Alternating weak and strong tunneling in a one-dimensional configuration realizes the single-particle Su-Schrieffer-Heeger (SSH) Hamiltonian, a paradigmatic model of topological matter. Band structure is probed through optical excitation from the ground state to Rydberg levels, revealing symmetry-protected topological edge states at zero energy. Edge-state energies are robust to perturbations of tunneling-rates that preserve chiral symmetry, but can be shifted by the introduction of on-site potentials.

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Probing topological edge states in a molecular synthetic dimension

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Engineering synthetic dimensions, where the physics of additional spatial dimensions is simulated within the internal states of a quantum system, allows the realisation of phenomena not otherwise accessible in experiments. Ultracold ground-state polar molecules are an ideal platform to encode synthetic dimensions, offering access to large Hilbert spaces of long-lived internal states associated with the rotational and hyperfine degrees of freedom, that can be coupled together with microwave fields to simulate tunnelling. Here, to benchmark the advantages of ultracold molecules, we encode a 1D synthetic lattice in the rotational states of ultracold RbCs molecules and use it to investigate the well-known Su-Schrieffer-Heeger (SSH) model, a minimal model displaying topological properties. To probe the system, we perform spectroscopy using an auxiliary rotational state and study the time dynamics after deterministic state preparation. We demonstrate long coherence times, typically ~500 times the lattice tunnelling period, even for a synthetic lattice using 8 rotational states. Observations of dynamics at long times with full site-resolved readout of the synthetic dimension allow us to test the effects of chiral and non-chiral perturbations on the topologically protected edge states. Our work lays the foundation for further quantum simulations using the rich internal structure of molecules, including dipolar string phases in interacting samples of molecules, and adiabatic state preparation of many-body Hamiltonians.

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The marriage between Rydberg physics and ultracold atomic systems have hatched so many fascinating achievements. The exaggerated properties of Rydberg states, combined with the pristine environments provided by the ultracold atoms, can lead to realizations of exotic physical systems. One particularly innovative direction that emerged recently is to use microwave-frequency transitions between Rydberg levels to simulate the dynamics of a particle hopping between lattice sites. Such approach, referred to as Rydberg synthetic dimensions, falls under the broad scheme of quantum simulations. Here we present description of the infrastructure used for Rydberg excitation and coherent microwave transitions, which are essential to the realization of Rydberg synthetic dimensions. We will also present experimental results on simulating the Su-Schireffer-Heeger Hamiltonian, a canonical model with paradigmatic importance in topological physics.
Rydberg-atom synthetic dimensions in the form of a lattice of n3S1n^{3}S_{1}n3S1​ levels, $58\ensuremath{\le}n\ensuremath{\le}63$, coupled through two-photon microwave excitation are used to examine dynamics within the single-particle Su-Schrieffer-Heeger Hamiltonian. This paradigmatic model of topological matter describes a particle hopping on a one-dimensional lattice with staggered hopping rates. Tunneling rates between lattice sites and on-site potentials are set by the microwave amplitudes and detuning, respectively. An atom is first excited to a Rydberg state that lies within the lattice and then subject to the microwave dressing fields. After some time, the dressing fields are turned off and the evolution of the population distribution in the different final lattice sites monitored using field ionization. The measurements show the existence of long-lived symmetry-protected edge states and reveal the existence of direct long-distance tunneling between the edge states. The results are in good agreement with model calculations and further demonstrate the potential of Rydberg-atom synthetic dimensions to simulate and faithfully reproduce complex Hamiltonians.
Synthetic dimensions are powerful tools for quantum simulation and computation. They are realized by harnessing internal or external degrees of freedom of an atom or molecule, which can mimic the motion of an electron in a real-space lattice potential. Such degrees of freedom are highly tunable and can be engineered to create configurations difficult to access or realize in real space. Some of the exciting possibilities include realizing higher dimensions systems[1, 2, 3], nontrivial real space[4, 5] and band structure[6, 7] topologies and artificial gauge fields[8, 9]. Experiments have utilized various degrees of freedom to create synthetic dimensions, such as motional[10, 11], spin[8, 12, 13, 14] and rotational[15] levels of atoms and molecules, and frequency modes, spatial modes, and arrival times in photonic systems[16]. Atomic synthetic dimensions have demonstrated artificial gauge fields, spin-orbit coupling, chiral edge states using Raman-coupled ground magnetic sublevels[8, 12, 17] of atoms, and phenomena such as Anderson localization using two-photon Bragg transitions by coupling free-particle momentum states[18]. Here, we harness the Rydberg levels of 84Sr to realize a synthetic lattice for studying quantum matter. Resonant millimeter-wave (mm-wave) radiation coupling Rydberg levels |i⟩ and |j⟩ with amplitude Ωij (Rabi frequency) are described by the same Hamiltonian as a particle tunneling between lattice sites |i⟩ and |j⟩ with tunneling amplitude Jij = Ωij /2. The mathematical equivalence to particles moving in a real-space lattice enables Rydberg levels to function as a synthetic spatial dimension. Rydberg-atom synthetic dimensions offer control over connectivity, tunneling rates and on-site potentials, which allows for the creation of a broad range of synthetic dimensional system. The capabilities of such a system are demonstrated by realizing the famous Su-Schrieffer-Heeger (SSH) model[19] and studying its topologically protected edge states(TPS).
Rydberg-atom synthetic dimensions in the form of a lattice of n3S1^3S_13S1​ levels, 58≤n≤6358\leq n \leq 6358≤n≤63, coupled through two-photon microwave excitation are used to examine dynamics within the single-particle Su-Schrieffer-Heeger (SSH) Hamiltonian. This paradigmatic model of topological matter describes a particle hopping on a one-dimensional lattice with staggered hopping rates. Tunneling rates between lattice sites and on-site potentials are set by the microwave amplitudes and detuning, respectively. An atom is first excited to a Rydberg state that lies within the lattice and then subject to the microwave dressing fields. After some time, the dressing fields are turned off and the evolution of the population distribution in the different final lattice sites monitored using field ionization. The measurements show the existence of long-lived symmetry-protected edge states and reveal the existence of direct long-distance tunneling between the edge states. The results are in good agreement with model calculations and further demonstrate the potential of Rydberg-atom synthetic dimensions to simulate and faithfully reproduce complex Hamiltonians.
Abstract A discrete degree of freedom can be engineered to match the Hamiltonian of particles moving in a real-space lattice potential. Such synthetic dimensions are powerful tools for quantum simulation because of the control they offer and the ability to create configurations difficult to access in real space. Here, in an ultracold 84 Sr atom, we demonstrate a synthetic-dimension based on Rydberg levels coupled with millimeter waves. Tunneling amplitudes between synthetic lattice sites and on-site potentials are set by the millimeter-wave amplitudes and detunings respectively. Alternating weak and strong tunneling in a one-dimensional configuration realizes the single-particle Su-Schrieffer-Heeger (SSH) Hamiltonian, a paradigmatic model of topological matter. Band structure is probed through optical excitation from the ground state to Rydberg levels, revealing symmetry-protected topological edge states at zero energy. Edge-state energies are robust to perturbations of tunneling-rates that preserve chiral symmetry, but can be shifted by the introduction of on-site potentials.
Synthetic dimension approach has emerged as a versatile and powerful technique in cold-atom toolbox for quantum simulation, serving as a complementary alternative to conventional optical lattice platforms. By mapping internal or external atomic states into discrete lattice sites, this method provides precise control over local tunneling amplitudes, phases, and on-site potentials, enabling flexible engineering of tight-binding Hamiltonians. Such capabilities have facilitated the experimental exploration of topology, synthetic gauge fields, disorder-induced phenomena, and exotic time-dependent dynamics across a range of platforms, including hyperfine and Rydberg states, momentum lattices, and harmonic-trap modes. In this review, we summarize the underlying principles of the key experimental synthetic dimension platforms, and their recent advances in quantum simulation. We also discuss the advantages and current limitations of the synthetic method, and provide a perspective on future directions, including hybrid-dimensional architectures and the study of high-dimensional many-body physics.
Engineering synthetic dimensions, where the physics of additional spatial dimensions is simulated within the internal states of a quantum system, allows the realisation of phenomena not otherwise accessible in experiments. Ultracold ground-state polar molecules are an ideal platform to encode synthetic dimensions, offering access to large Hilbert spaces of long-lived internal states associated with the rotational and hyperfine degrees of freedom, that can be coupled together with microwave fields to simulate tunnelling. Here, to benchmark the advantages of ultracold molecules, we encode a 1D synthetic lattice in the rotational states of ultracold RbCs molecules and use it to investigate the well-known Su-Schrieffer-Heeger (SSH) model, a minimal model displaying topological properties. To probe the system, we perform spectroscopy using an auxiliary rotational state and study the time dynamics after deterministic state preparation. We demonstrate long coherence times, typically ~500 times the lattice tunnelling period, even for a synthetic lattice using 8 rotational states. Observations of dynamics at long times with full site-resolved readout of the synthetic dimension allow us to test the effects of chiral and non-chiral perturbations on the topologically protected edge states. Our work lays the foundation for further quantum simulations using the rich internal structure of molecules, including dipolar string phases in interacting samples of molecules, and adiabatic state preparation of many-body Hamiltonians.