Microscopic quantum electrodynamics origin of spin entanglement

Jeffrey Scott Pratt

Moslem Zarei

We study effective spin interactions arising from quantum electrodynamics (QED) scattering between localized fermionic spins. By integrating out photon and mediator fields, the dynamics reduce to an effective spin Hamiltonian. For two qubits in the nonrelativistic regime, the resulting interaction takes a tensor dipolar form with an asymptotic decay proportional to \(R^{-3}\). We obtain analytical expressions for the entanglement negativity, highlighting its dependence on coupling strength and spatial configuration. We then examine a setup in which two bath spins interact via a sequential exchange with an intermediate fermionic mediator. At the perturbative order considered, the mediator remains unentangled and induces an effective bath--bath interaction with stronger spatial suppression than in the photon-mediated case. Extending the construction to an \(N\)-spin setting yields an effective interaction network mediated by virtual exchange processes, which can support the generation of multipartite entanglement across the system.

Wenbo Sun

Quantum light-matter interactions, described by the theory of quantum electrodynamics (QED), have motivated numerous scientific discoveries and technological developments over the past few decades. Considerable effort has been made to develop different QED platforms, e.g., free space, waveguides, cavities, and photonic crystals, for engineering quantum light-matter interactions. This thesis explores a new frontier, deep microscopic QED, which leverages the deep microscopic response of materials to reveal new topological, quantum, and thermal photonic phenomena with applications to quantum sensing and information processing. In the first part of this thesis, we investigate unique topological photonic effects arising in the deep microscopic QED regime. Previous efforts focused on topological photonic phases and edge states arising from artificial spatial structures of materials (e.g., photonic crystals or metamaterials). One fundamental question is whether topological photonic states can also arise from the intrinsic response of many-body systems and do not rely on materials' macroscopic structures. Here, we first discuss a new topological electromagnetic phase - ‘optical N-phase’ arising in two-dimensional (2D) viscous hydrodynamic electrons in graphene, which originates from the microscopic response of 2D materials and does not rely on materials' macroscopic structures. We then introduce the associated edge states, optical N-plasmons, which are topologically protected ultra-subwavelength edge magneto-plasmons. We further show how these topological plasmons can be harnessed to design chiral radio-frequency nonreciprocal circuit components, topological hydrodynamic circulators, that interface quantum and classical hardware.In the second part of this thesis, we focus on collective atom-photon interactions in the deep microscopic QED regime. In atom interactions with photonic environments, there exist two non-unitary processes -- pure dephasing and spontaneous emission. Despite considerable interest in collective effects in spontaneous emission since the 1950s, one long-standing problem is whether collective effects in pure dephasing can arise in atom-photon interactions. This question is particularly important in the quantum information era since pure dephasing is the main obstacle in current quantum information technologies. Here, we first introduce a new collective quantum phenomenon, ‘nanophotonic superdephasing,’ occurring in atom/spin ensembles in nanoscale photonic environments. This nanophotonic superdephasing phenomenon originates from low-frequency photonic environment correlations, and leads to collectively accelerated disentanglement without photon emission, in stark contrast to conventional collective spontaneous emission/superradiance effects. We further reveal the effects of nanophotonic environment mediated correlated dynamics on quantum computing and sensing. We demonstrate that correlations of nanoscale EM environments in spin qubit quantum computing devices can induce correlated errors and limit quantum gate fidelity. Meanwhile, based on nanophotonic collective dephasing, we also propose a multiqubit quantum sensing protocol that exploits spatially correlated noise near materials to enable order parameter symmetry characterization of materials beyond single-qubit methods.In the final part, we explore thermal photonic phenomena in the deep microscopic regime. Conventional techniques in engineering near-field radiative heat transfer typically rely on phonons, plasmons, and electromagnetic modes in structured materials. Here, we reveal a new approach to enhance near-field thermal radiation: leveraging intrinsic quantum coherence in superconducting materials. We reveal the quantum fingerprint of superconductivity in thermal photonics, ‘superconducting coherence peak’ in near-field thermal radiation, which originates from quantum coherence of Bogoliubov quasiparticles, with potential applications in thermal engineering in superconducting circuits.Overall, the thesis establishes a deep microscopic QED platform for new quantum, topological, and thermal photonic phenomena in many-body systems, with applications in quantum sensors and devices.

Ana María Rey

Saeed Rahmanian Koshkaki, Ding Xu, Michael Fowler +2 more

Optical spin-orbit interactions (SOI), demonstrated experimentally in optical cavities, enable the polarization degrees of freedom of light to be described and controlled as an effective pseudospin, providing a foundation for spintronic-like control of light and the development of next-generation optical technologies. However, prior works describe this emergent effect using phenomenological models that fail to uncover its microscopic quantum origins, and as a result, a rigorous connection between material electronic structure and the optical SOI remains elusive. In this work, we address this fundamental challenge by developing a microscopic quantum theory starting from the non-relativistic quantum electrodynamical (QED) description of light-matter interactions. We show that this effect arises from virtual interactions between confined photons and material excitations. Crucially, our theoretical framework provides microscopic material-design principles for tuning the distinct components of optical SOI, which include the optical birefringence, photonic self-energies, TE-TM splitting, and optical Zeeman splitting, enabling precise engineering of effective magnetic fields, diabolical points, and pseudospin textures. We anticipate that the predictive capability of our microscopic theory will enable systematic screening and design of material systems for photonic spintronics and optical technologies.

Cuixia Wang, Ding Xiong, Guoqiang Huang +1 more