This thesis describes experimental and theoretical work towards a novel dual species platform for Rydberg quantum information processing employing ultracold samples of potassium (K) and rubidium (Rb) atoms. The dual-species setup combined with the possibility of deploying arrays of ultracold atomic ensembles trapped in optical tweezers will pave the way for a new generation of Rydberg single-photon optical transistors with high input photon rate. Firstly, by using degenerate fermionic 40K samples as the storage medium one can take advantage of the Pauli exclusion principle which offers protection against loss and dephasing mechanisms of Rydberg polaritons, while the bosonic 87Rb species can be used as a benchmark. Secondly, simultaneously trapping nearby ensembles of the two species opens up the possibility of creating strong interactions between photons of different ”colours”, as well as the independent control of parameters of the atomic storage medium. A theoretical study conducted in the first part of this thesis reveals multiple experimentally accessible pair combinations of K and Rb atoms in their respective Rydberg states which have high interaction strength. These K-Rb pair states offer long-range interaction suitable for such a spatially isolated transistor setup. The subsequent part presents experimental work towards a dual species Rydberg optical transistor. This includes the establishment of a laser system to access Rydberg states in both species, and a feedback system to reduce atom number fluctuations. Lastly, non-destructive measurements of Rydberg states, using electromagnetically induced transparency and the newly established setup, are presented for ultracold samples of 40K and 87Rb.
This thesis describes experimental and theoretical work towards a novel dual species platform for Rydberg quantum information processing employing ultracold samples of potassium (K) and rubidium (Rb) atoms. The dual-species setup combined with the possibility of deploying arrays of ultracold atomic ensembles trapped in optical tweezers will pave the way for a new generation of Rydberg single-photon optical transistors with high input photon rate. Firstly, by using degenerate fermionic 40K samples as the storage medium one can take advantage of the Pauli exclusion principle which offers protection against loss and dephasing mechanisms of Rydberg polaritons, while the bosonic 87Rb species can be used as a benchmark. Secondly, simultaneously trapping nearby ensembles of the two species opens up the possibility of creating strong interactions between photons of different ”colours”, as well as the independent control of parameters of the atomic storage medium. A theoretical study conducted in the first part of this thesis reveals multiple experimentally accessible pair combinations of K and Rb atoms in their respective Rydberg states which have high interaction strength. These K-Rb pair states offer long-range interaction suitable for such a spatially isolated transistor setup. The subsequent part presents experimental work towards a dual species Rydberg optical transistor. This includes the establishment of a laser system to access Rydberg states in both species, and a feedback system to reduce atom number fluctuations. Lastly, non-destructive measurements of Rydberg states, using electromagnetically induced transparency and the newly established setup, are presented for ultracold samples of 40K and 87Rb.
Large-scale Rydberg atom arrays are used for highly coherent analogue quantum simulations and for digital quantum computations. However, advanced quantum protocols, such as quantum error correction, require midcircuit qubit operations, including the replenishment, reset and read-out of a subset of qubits. A compelling strategy for unlocking these capabilities is a dual-species architecture in which a second atomic species is controlled independently and entangled with the first through Rydberg interactions. Here, we realize a dual-species Rydberg array consisting of rubidium and caesium atoms and explore regimes of interactions and dynamics not accessible in single-species architectures. We achieve enhanced interspecies interactions by electrically tuning the Rydberg states close to a Förster resonance. In this regime, we demonstrate an interspecies Rydberg blockade and implement a quantum state transfer from one species to another. We then generate a Bell state between Rb and Cs hyperfine qubits through an interspecies controlled-phase gate. Finally, we combine interspecies entanglement with a native midcircuit read-out to achieve quantum non-demolition measurements. Rydberg atoms in optical tweezers are a promising platform for quantum information science. A platform composed of dual-species Rydberg arrays has been realized, offering access to unexplored interaction regimes and crosstalk-free midcircuit control.
Over the past decade, quantum information science has progressed from few-qubit demonstrations to experiments with hundreds of qubits. Neutral atom processors based on individual atoms trapped in arrays of optical tweezers have emerged as a leading candidate due to their inherent scalability and flexible connectivity. Advanced protocols like measurement-based state preparation and quantum error correction, however, require efficient crosstalk-free mid-circuit operations for the readout, reset, and replenishment of a subset of qubits. In typical single-species atom arrays, where all atoms are identical and on-resonance, such operations necessitate complex overheads from single-site addressing, coherent transport, or shielding techniques, to mitigate the qubit decoherence induced from photons scattered by neighboring atoms. To address this challenge of engineering scalable quantum architectures compatible with efficient control techniques, we introduce and implement the first dual-species atom array platform, and explore new dynamics inaccessible in single-species arrays. In this approach, two atomic species are addressed independently due to the spectral separation between their control wavelengths. We engineer two-dimensional arrays from individual rubidium (Rb) and cesium (Cs) atoms in up to 512 optical tweezers, and show that the two species can be independently trapped, cooled, and imaged with state-of-the-art performance metrics. Harnessing this intrinsic crosstalk-free control, we establish the key primitives of mid-circuit readout, real-time processing and feed-forward, and coherent mid-circuit reloading. By integrating these capabilities, we realize in-sequence, real-time correction of correlated phase errors via a spectator qubit protocol. Next, we excite atoms to Rydberg states in the Förster regime, accessing hitherto unobserved enhanced interspecies Rydberg interactions, and program them to implement the first interspecies CNOT gate. We combine this multispecies entanglement with mid-circuit readout to achieve quantum non-demolition measurement of a Rb-qubit using an auxiliary Cs-qubit, circumventing physical qubit transport. Finally, leveraging the two qubit modalities, we present the first experimental demonstration of quantum cellular automata in atom arrays using only global addressing, and prepare a 17-qubit Cs cluster state with Rb-mediated interactions. The dual-species platform and techniques established in this thesis pave the way toward measurement-based algorithms and real-time feedback control in large-scale quantum systems.
High optical nonlinearities can be achieved at the single photon level by coupling the photon states to strongly interacting Rydberg excitations under the conditions of electromagnetically induced transparency. The nonlinear response in Rydberg quantum optics comes as a direct result of the long range dipole-dipole interactions via Rydberg blockade and interaction induced dephasing. In this thesis, Rydberg quantum optics experiments are performed with two spatially separated mediums with a nonlinear response at the single photon level. Two ultracold rubidium atomic clouds are tightly confined by a pair of in-vacuo aspheric lenses such that only a few Rydberg excitations can exist in each one of the clouds simultaneously. The long range character of the dipole-dipole interactions leads to the generation of quantum states of light. The effective photon-photon interactions are directly observed as an anti-correlation in the simultaneous photon retrieval as a result of the non resonant van der Waals interactions. The collective Rydberg excitations, stored in the non-overlapping mediums, experience an additional spatial non-uniform phase. In addition, we experimentally characterize the cooperative optical response of a cold atomic medium at a single photon level. This aims to exploit the enhancement of the spontaneous emissions decay rate (superradiance) as a dependence of the number of atoms involved in the ensemble. The observed atomic response in two different regimes gives a further understanding of the system dynamics and unlocks a promising potential route towards the implementation in scalable, multichannel quantum optical devices.
Optical tweezer arrays of neutral atoms have emerged as a promising platform for studying quantum physics. These individual atoms can be carefully prepared in single quantum states, and easily manipulated with microwaves and lasers. MHz scale interactions are accessible at several micron scale distances by exciting these atoms to Rydberg states. These arrays can also be created in arbitrary 2D geometries with the use of a spatial light modulator. Adding the capability of a second species opens new possibilities in non-destructive measurement and quantum simulation of bipartite systems with widely tunable parameters. In this thesis, we describe our efforts to build a flexible platform for studying quantum phenomena utilizing two species of atoms, sodium and cesium. In particular, we discuss the laser technology and setups required to create dual species optical tweezer arrays. These arrays are made defect-free with real-time rearrangement of atoms using a separate set of tweezers created with acousto-optical deflectors. We then describe how to excite these atoms coherently to the Rydberg state with coherence times in Cs as long as 20 microseconds. With these techniques established, we are able to probe an Ising critical point in 1D and 2D systems with up to 81 atoms. In particular, we measure and confirm the value of the universal critical exponent, η, via adiabatic preparation of the ground state at the critical point. Then, we measure the interactions between sodium and cesium atoms setting the stage for future experiments. Lastly, a theoretical proposal is presented where Rydberg atoms can be used to enhance the interaction rates of ultracold polar molecules, as well as measure their states non-destructively.
Quantum simulation offers the possibility to study quantum mechanical problems which are untraceable on classical computers. This thesis introduces a novel platform for quantum simulation and presents the first experimental realisation of single potassium atoms trapped in optical tweezers. Interactions between individual atoms are induced by strong energy shifts of atoms excited to states with large principal quantum number, so-called Rydberg states. Either direct excitation to Rydberg states or off-resonant dressing can be used to induce these interactions. We argue that potassium is well-suited for the implementation of Rydberg dressing, enabling simultaneous dressing of both ground states to engineer complex interactions. Using techniques to cool and trap cold atoms, single potassium atoms are prepared in arrays of optical tweezers. Raman sideband cooling reduces vibrational excitations and prepares the atoms close to the motional ground state. This cooling technique mitigates severe limitations for Rydberg dressing, arising from thermal broadening and inhomogeneous light shifts in the array of atoms. To directly excite atoms to Rydberg states, a high power laser setup with two cavity-enhanced frequency doubling stages is constructed, generating up to one Watt of ulta-violet light at 286 nm. By exciting atoms to Rydberg states we observe Rabi oscillations with Rabi frequencies of up to 1 MHz, demonstrating coherent control of Rydberg atoms. Finally, we combine these techniques to observe interactions in two ways: First, we create a so-called superatom of up to four individual atoms using direct excitation and Rydberg-blockade and observe coherent oscillations to this collective state. We measure the expected square root scaling of the effective Rabi frequency with the number of individual atoms, confirming the creation of a many-body entangled state. Secondly, we off-resonantly dress the atoms prepared in a one-dimensional chain and measure correlated interaction shifts over multiple sites. In summary, we have developed a platform for quantum simulation with single atoms in optical tweezers. The presented results show coherent control of single atoms and interactions induced by Rydberg states. We have thus demonstrated that the system is well-suited for quantum simulation of many-body systems.
Interacting Rydberg excitations in cold atomic ensembles can exhibit large quantum nonlinearities that enable engineering of strong interactions between individual photons. Consequently, Rydberg ensembles are a promising platform for quantum information applications and the study of more fundamental physics of few- and many-body phenomena with interacting photons. This thesis presents a series of experiments that study and exploit different regimes of Rydberg-mediated interactions. We report the realization of an efficient on-demand single-photon source. The strong long-range Rydberg interactions allow the excitation of only a single collective Rydberg state within the entire atomic medium. The collective excitation can be subsequently retrieved as a single-photon. We use this scheme to generate highly pure and highly indistinguishable photons, which are suitable for scalable quantum information applications. These photons can be compatible with other atomic systems due to their narrow bandwidth, which makes building practical hybrid quantum systems feasible. Here, we demonstrate high visibility two-photon quantum interference between our Rydberg-produced photons, and photons emitted by a remote single-trapped ion. We also study Rydberg atoms under electromagnetically induced transparency conditions, where coherent superpostions of photons and Rydberg excitations propagate through the atomic medium as lossless dark-state polaritons. In the experiment, we use the external control fields to tune the interactions to a many-body regime where we can observe resonant scattering of dark-state polaritons to lossy channels. We show that the enhanced scattering process arises as a pure three-body effect.