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Journal of Experimental and Theoretical Physics Letters

Capture of Thulium Atoms into a Magneto-Optical Trap and Their Detection Using the 530-nm Transition

Daniil I. Provorchenko, A. A. Dvurechenskii, B. A. Bessmertnykh, D. Mishin, Д. О. Трегубов, N. Kolachevsky, Artem A. Golovizin

Published Jun 1, 2026• 0 citations
Publisher

Abstract

The efficient capture of thulium atoms from an atomic beam into a magneto-optical trap at the spectrally narrow 530-nm transition with a natural linewidth of 350 kHz, avoiding the primary cooling stage that is standard in many experiments, has been demonstrated. To optimize the capture parameters, a machine learning method with automated control of the experimental setup and feedback has been used, which has made it possible to achieve more than 75% capture efficiency compared to the previously used configuration. In addition, the number of atoms has been measured using 530-nm probe radiation with the ability to achieve signal-to-noise levels comparable to those obtained with fluorescence detection on the strong 410-nm transition. This significantly reduces the requirements for the 410-nm laser system, which was previously used for primary cooling and detection of atoms, simplifying the experimental setup and paving the way toward transportable thulium optical clocks.

DOI
10.1134/s0021364026601314

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The efficient capture of thulium atoms from an atomic beam into a magneto-optical trap at the spectrally narrow 530-nm transition with a natural linewidth of 350 kHz, avoiding the primary cooling stage that is standard in many experiments, has been demonstrated. To optimize the capture parameters, a machine learning method with automated control of the experimental setup and feedback has been used, which has made it possible to achieve more than 75% capture efficiency compared to the previously used configuration. In addition, the number of atoms has been measured using 530-nm probe radiation with the ability to achieve signal-to-noise levels comparable to those obtained with fluorescence detection on the strong 410-nm transition. This significantly reduces the requirements for the 410-nm laser system, which was previously used for primary cooling and detection of atoms, simplifying the experimental setup and paving the way toward transportable thulium optical clocks.
We have developed a compact vacuum system for laser cooling and spectroscopy of neutral thulium atoms. Compactness is achieved by obviating a classical Zeeman slower section and placing an atomic oven close to a magneto-optical trap (MOT), specifically at the distance of 11 cm. In this configuration, we significantly gained in solid angle of an atomic beam, which is affected by MOT laser beams, and reached 1 million atoms loaded directly in the MOT with only 15 mW of MOT cooling beams net power. By exploiting Zeeman-like deceleration of atoms with an additional laser beam and tailoring the MOT magnetic field gradient with a small magnetic coil, we demonstrated trapping of up to 13 million atoms. These results show great perspective of the developed setup for realizing a compact high-performance optical atomic clock based on thulium atoms.
We propose to use the magnetic-dipole transition at coupling two ground state fine-structure components of thulium (Tm), as a 'clock transition' in optical clocks. We have demonstrated first stage laser cooling of Tm atoms down to a temperature of 25 K using a strong transition at and we have also shown preliminary results for second stage cooling using a weaker transition at (natural linewidth γ G = 350 kHz). Laser cooled atoms have been trapped in an optical dipole trap and in a 1D optical lattice operating near 532 nm.
Deep laser cooling of atoms, ions, and molecules facilitates the study of fundamental physics as well as applied research. In this work, we report on the narrow-line laser cooling of thulium atoms at the wavelength of 506.2nm with the natural linewidth of 7.8kHz, which widens the limits of atomic cloud parameters control. Temperatures of about 400nK, phase-space density of up to 3.5×10−4 and 2×106 number of trapped atoms were achieved. We have also demonstrated formation of double cloud structure in an optical lattice by adjusting parameters of the 506.2nm magneto-optical trap. These results can be used to improve experiments with BEC, atomic interferometers, and optical clocks.
Laser cooling is a necessary tool to generate ultracold atoms in magneto-optical traps (MOT), as atomic transitions can be excited with lasers to address different energy levels. As these transitions differ for each quantum system, flexibility in delivering the right wavelength and power at the atoms is key for viable quantum devices or experiments. In our work, we present custom laser systems at the edges of the thulium emission range for improving barium and strontium atoms trapping experiments [1]. Two of barium's narrow atomic transitions can be directly addressed with lasers at 1762 nm and 2052 nm, while third harmonic generation from 2067 nm and 2095 nm allows to address the red MOT cooling and the clock transitions in strontium at 689 nm and 698 nm.
Secondary laser cooling has been realised on the weak dipole transition 4f13(2Fo)6s2, J = 7/2, F=4 → 4f12(3H6) 5d5/26s2, J' = 9/2, F' = 5 with the wavelength of 530.7 nm and natural width of 350 kHz. The temperature of the atomic cloud in a magnetooptical trap (MOT) was 30 μK at the lifetime of 2 s and the number of atoms 105. Approximately 1% of atoms from the MOT have been reloaded to an optical dipole trap and to one-dimensional optical lattice at the wavelength of 532 nm. The atom lifetime in the optical lattice was 320 ms. We propose to employ thulium atoms captured in an optical lattice as an optical frequency reference.
Second-stage laser cooling of thulium atoms at the 530.7 nm transition with a natural linewidth of 350 kHz offers an interesting possibility to study different regimes of a magneto-optical trap (MOT). The intermediate value of the spectral linewidth of the cooling transition allows the observation of three distinct regimes depending on the intensity and detuning of the cooling beams, namely, the ``bowl-shaped'' regime when light pressure force competes with gravity, the ``double structure'' regime with interplay between the Doppler and polarization-gradient (sub-Doppler) cooling, and the ``symmetric'' regime when Doppler cooling dominates over sub-Doppler cooling and gravity. The polarization-gradient cooling manifests itself by a two-temperature momentum distribution of atoms resulting in a double-structure of the spatial MOT profile consisting of a cold central fraction surrounded by a hot halo. We studied the double structure regime at different saturation parameters and compared observations with calculations based on semiclassical and quantum approaches. The quantum treatment adequately reproduces experimental results if the MOT magnetic field is properly taken into account.