High-quality factor photonic eigenstates stemming from bound states in the continuum (BICs) significantly enhance the nonlinear-optical response, enabling many peculiar scenarios of light–light interaction in dielectric metasurfaces. We consider a quasi-BIC metasurface built of dimers of AlGaAs rods and model spontaneous parametric down-conversion, yielding pairs of quantum-entangled photons. We show that specific properties of the quasi-BIC—maximum extrinsic chirality along straight flatbands in the reciprocal space—allow for the emission of pairs of photons outgoing from different metasurface sides in slightly oblique directions and carrying maximum quantum entanglement. As the same quasi-BIC is linearly polarized for normal incidence, it can also generate co-polarized photons in unentangled product states. We simulate different regimes of generation of photon pairs, having a continuously variable degree of polarization entanglement, with and without frequency entanglement, all controlled by subtle changes in the pump and detection wavelengths.
High-quality factor photonic eigenstates stemming from bound states in the continuum (BICs) significantly enhance the nonlinear-optical response, enabling many peculiar scenarios of light–light interaction in dielectric metasurfaces. We consider a quasi-BIC metasurface built of dimers of AlGaAs rods and model spontaneous parametric down-conversion, yielding pairs of quantum-entangled photons. We show that specific properties of the quasi-BIC—maximum extrinsic chirality along straight flatbands in the reciprocal space—allow for the emission of pairs of photons outgoing from different metasurface sides in slightly oblique directions and carrying maximum quantum entanglement. As the same quasi-BIC is linearly polarized for normal incidence, it can also generate co-polarized photons in unentangled product states. We simulate different regimes of generation of photon pairs, having a continuously variable degree of polarization entanglement, with and without frequency entanglement, all controlled by subtle changes in the pump and detection wavelengths.
The efficient and controllable generation of entangled photon pairs is a cornerstone for advancing quantum technologies, including quantum computing, communication, and sensing. Traditional methods, primarily relying on spontaneous parametric down-conversion (SPDC) or spontaneous four-wave mixing (SFWM) in bulk nonlinear crystals or waveguides, often suffer from low efficiency, bulky form factors, and limited control over the spectral and spatial properties of the generated photons. This paper explores a transformative approach leveraging resonant Bound States in the Continuum (BICs) within nanophotonic structures to overcome these limitations. BICs are extraordinary optical resonances characterized by theoretically infinite quality (Q) factors, enabling extreme light localization and immense field enhancement within subwavelength volumes. By integrating nonlinear optical materials into BIC-supporting structures, such as photonic crystal slabs or metasurfaces, the local electric field strength experienced by the nonlinear medium can be dramatically increased, boosting the efficiency of entangled photon generation. Furthermore, the sharp, tailor-able spectral response of BICs offers unprecedented control over the joint spectral amplitude of the photon pairs, promising high degrees of spectral purity and entanglement fidelity. This work outlines the theoretical underpinnings, potential device architectures, and anticipated advantages of BIC-enhanced entangled photon sources, paving the way for compact, high-brightness, and spectrally engineered quantum light sources critical for next-generation quantum technologies.
Here we demonstrate the efficient photon-pair generation via spontaneous parametric down conversion from a semiconductor metasurface supporting dual quasibound states in the continuum (quasi-BICs). In a simple metasurface composed of AlGaAs elliptical nanocyclinders, the two high-Q quasi-BIC resonances that coincide with the generated signal and idler frequencies significantly boost the local electric field. This leads to a substantial enhancement in the reverse classical nonlinear process of sum-frequency generation and subsequently the remarkably high generation rate of photon pairs under the quantum-classical correspondence principle. Within a narrowband wavelength regime around the quasi-BIC resonances, the rate of pair production is enhanced up to $\ensuremath{\sim}{10}^{4}$ Hz, two orders of magnitude larger than that in the Mie resonant AlGaAs nanoantennas. Moreover, the photon pair emission is mainly concentrated in the normal direction with respect to the metasurface, and shows a tunable rate with the Q factor by engineering the rotation angle of nanocylinders. The presented work enables nanoscale sources of high-quality entangled photons which will find applications in advanced quantum imaging and communications.
spontaneous parametric down conversion from a metasurface supporting a quasi-bound state in the continuum (BIC) leading to remarkable emission directivities. The pair generation rate is enhanced 67 times compared to the case of an unpatterned film of the same thickness and material. At the wavelength of the quasi-BIC resonance, photons are mostly emitted backwards, while their partners, spectrally detuned by only 8 nm, are emitted forwards. This behavior demonstrates fine spectral splitting of entangled photons and their bi-directional emission, never before observed in nanoscale sources. We expect this work to be a starting point for the efficient demultiplexing of photons in nanoscale quantum optics.
Spontaneous parametric down conversion (SPDC) has proven to be a robust and prominent method for creating non-classical light sources of entangled single-photon pairs. However, such sources suffer from low efficiency due to the inherent weakness of the SPDC process. Moreover, there is no control of polarization in the generated photons. Circularly polarized SPDC-based sources with an efficient chiral response are currently missing, which severely precludes the realization of a wide range of practical applications in quantum computing and communications. The current work solves these inherent problems by demonstrating a novel chiral plasmonic metasurface that leverages a strong quasi-bound state in the continuum (qBIC) resonance, which significantly increases the SPDC photon generation efficiency and realizes circularly polarized (chiral) single-photon pairs. The presented metasurface design is ultrathin, supports efficient free space outcoupling of chiral classical and quantum radiation, and operates at room temperature. Hence, it offers the potential to realize a compact and integrable quantum source of circularly polarized entangled single-photon pairs.
Single-photon sources can be realized by spontaneous parametric down-conversion (SPDC), where a pair of entangled single photons is generated. However, SPDC is an inherently weak process and lacks control in the polarization of the generated photons. Increasing the efficiency and controlling the polarization of SPDC-based sources is critical for their practical use in quantum communications and computing. Here, we demonstrate a new chiral plasmonic metasurface leveraging a resonant quasi-bound state in the continuum (qBIC) response in reflection that significantly enhances single-photon pair generation rates and circularly polarizes the produced non-classical (quantum) light. The ultrathin design consists of a lithium niobate(LiNbO3)crystal overlaid by a chiral silver grating made of tilted nanorods responsible for the qBIC chiral response. When excited by sources of polarity and wavelength matching to the metasurface resonant conditions, a significant enhancement of the electric field can occur within theLiNbO3layer. With two incident circular polarized sources, the nonlinear sum frequency generation (SFG) efficiency is increased drastically over theLiNbO3layer alone leading to a substantially boosted rate of single photon-pairs created by SPDC due to the quantum-classical correspondence principle. The design presented here is ultrathin, relies on efficient free space coupling of chiral radiation, and operates in room temperature, resulting in a new quantum source of chiral single-photon pairs that can be easily integrated into a wide range of applications in quantum photonics.
Quantum state engineering, the cornerstone of quantum photonic technologies, mainly relies on spontaneous parametric downconversion and four-wave mixing, where one or two pump photons spontaneously decay into a photon pair. Both of these nonlinear effects require momentum conservation for the participating photons, which strongly limits the versatility of the resulting quantum states. Nonlinear metasurfaces have subwavelength thickness and allow the relaxation of this constraint; when combined with resonances, they greatly expand the possibilities of quantum state engineering. Here, we generated entangled photons via spontaneous parametric downconversion in semiconductor metasurfaces with high-quality factor, quasi-bound state in the continuum resonances. By enhancing the quantum vacuum field, our metasurfaces boost the emission of nondegenerate entangled photons within multiple narrow resonance bands and over a wide spectral range. A single resonance or several resonances in the same sample, pumped at multiple wavelengths, can generate multifrequency quantum states, including cluster states. These features reveal metasurfaces as versatile sources of complex states for quantum information.