This PhD thesis presents the design, development, and implementation of a loadlock platform tailored for next-generation quantum optics experiments. Quantum optics, a field at the forefront of both fundamental research and technological innovation, relies heavily on precise control over light-matter interactions. To advance this field, the thesis provides a comprehensive exploration of the theoretical and experimental foundations of quantum optics, followed by a detailed examination of the loadlock platform's role in enhancing experimental capabilities.
This PhD thesis presents the design, development, and implementation of a loadlock platform tailored for next-generation quantum optics experiments. Quantum optics, a field at the forefront of both fundamental research and technological innovation, relies heavily on precise control over light-matter interactions. To advance this field, the thesis provides a comprehensive exploration of the theoretical and experimental foundations of quantum optics, followed by a detailed examination of the loadlock platform's role in enhancing experimental capabilities.
Cavity quantum electrodynamics (QED), the study of the interaction between quantized emitters and photons confined in an optical cavity, is an important tool for quantum science in computing, networking, and synthetic matter. In atomic cavity QED, this approach typically relies upon an ultrahigh vacuum chamber that hosts a cold trapped atomic ensemble and an optical cavity. Upgrading the cavity necessitates a months-long laborious process of removing external optics, venting, replacing the resonator, baking, and replacing optics, constituting a substantial bottleneck to innovation in resonator design. In this work, we demonstrate that the flexibility of optical cavities and the quick turnaround time in switching between them can be restored with the vacuum loadlock technique-reducing the cycle time to install a cavity, bake it, and transport it into the science chamber for days, achieving 3 × 10-10 Torr pressure in the science chamber. By reducing vacuum limitations, this approach is particularly powerful for labs interested in quickly exploring novel optic cavities or any other atomic physics relying on in-vacuum optics.
In this Thesis we design radiation patterns capable of creating effective light-matter interactions suited to applications in quantum computing, quantum simulation and quantum sensing. On the one hand, we have used dynamical decoupling techniques to design quantum operations that are robust against errors in environmental and control fields, achieving high-fidelity quantum logic in trapped ions and energy-efficient nuclear magnetic resonance at the nanoscale with nitrogen-vacancy centers in diamond. On the other hand, we have studied generalised models of light-matter interaction, leading to the discovery of selective multi-photon interactions in the Rabi-Stark model and a proposal for preparing non-classical quantum states using the nonlinear quantum Rabi model. Finally, we have shown how the appropriate tailoring of interactions among ultracold atoms in optical lattices could lead to solve the boson sampling problem faster than the best supercomputers, thus demonstrating quantum supremacy. In this manner, we believe the results presented here significantly expand our knowledge on the control of light-matter interactions, and provide optimal scenarios for current quantum devices to generate the next-generation of quantum applications.
Quantum optics is the branch of physics that investigates the interaction of light with matter at the quantum level, where the discrete nature of photons and quantum states of atoms, molecules, and solid-state systems become dominant. Quantum optics systems provide the experimental and theoretical foundation for understanding nonclassical states of light, quantum coherence, entanglement, and measurement at the quantum limit. Over the past few decades, advances in laser technology, nonlinear optics, and precision measurement have transformed quantum optics from a fundamental discipline into a key enabler of quantum technologies, including quantum communication, quantum computing, quantum sensing, and quantum metrology. This review presents a comprehensive overview of the physical principles, system architectures, and experimental platforms of quantum optics. Emphasis is placed on light sources, atom–photon interaction systems, detection techniques, and emerging applications, along with current challenges and future research directions.
While the fundamental principles of light-matter interaction are well-understood and drive countless technologies, the world of multiphoton processes remains a fascinating puzzle, holding the potential to drastically alter our understanding of how light interacts with matter at its most basic level. This rich interplay of light and matter unveils novel phenomena that can be harnessed for sensing with exceptional precision, as exemplified by multiphoton quantum sensing. This thesis delves into the applications of multiphoton quantum protocols, particularly in imaging, communication, and plasmonic sensing, to surpass classical limitations and achieve enhanced sensitivity. We explore the potential of multiphoton quantum processes, particularly in the nanoscale regime and within subsystems of macroscopic systems, where novel and ultra-sensitive sensing methodologies emerge. Subsequent chapters of this thesis demonstrate the transformative potential of multiphoton quantum sensing, elucidating the design, implementation, and experimental results of specific sensing protocols tailored to diverse applications. Our analysis combines experimental observations and theoretical predictions to assess the sensitivity and performance of these protocols. Additionally, the thesis discusses potential future directions and advancements in the field, envisioning applications in biomolecule detection, environmental monitoring, and fundamental studies of light-matter interactions at the nanoscale. Concluding reflections highlight the implications of multiphoton quantum sensing across scientific disciplines and lay the groundwork for future research endeavors.
Space has always been a primary source of inspiration for the development of the scientific, technological, artistic, philosophical and religious thinking of the whole humankind. Space explorations marked the history of the XX century, bringing an incredible technological advancement and allowing to investigate the natural phenomena over scales and into details which are simply not available on Earth. Nowadays, the Space is the benchmark of the new quantum revolution, which promises to change the way we communicate, measure and calculate, thank to the exploitation and the control of what happens at the microscopic scale. Indeed, the quantum theory, born at the beginning of the XX century to describe the behavior of the elementary particles of Nature, has reached today an incredible reliability. As any scientific theory, Quantum Mechanics is valid within the limits in which it has been experimentally verified, and the Space is the main stage where to validate quantum predictions at large scales, in a domain that is completely different with respect to the microscopic one from which it moved. The technological advances in photonics, which allows the manipulation and the control of the single quanta of light, the photons, make today feasible fundamental tests of Quantum Mechanics in Space, experiments to investigate, for example, if entanglement is preserved along thousands of kilometers or if the wave-particle duality survives even after a Space trip. Furthermore, Space makes available relativistic regimes, in which the velocities and the distances could allow to experimentally investigate the unresolved puzzle of modern physics, that is, the interplay between Quantum Mechanics and gravitation. For these reasons, this thesis is dedicated to the Quantum Optics experiment in Space I have been involved during my PhD.
While the fundamental principles of light-matter interaction are well-understood and drive countless technologies, the world of multiphoton processes remains a fascinating puzzle, holding the potential to drastically alter our understanding of how light interacts with matter at its most basic level [1–4]. This rich interplay of light and matter unveils novel phenomena that can be harnessed for sensing with exceptional precision, as exemplified by multiphoton quantum sensing. This thesis delves into the applications of multiphoton quantum protocols, particularly in imaging, communication, and plasmonic sensing, to surpass classical limitations and achieve enhanced sensitivity. We explore the potential of multiphoton quantum processes, particularly in the nanoscale regime and within subsystems of macroscopic systems, where novel and ultra-sensitive sensing methodologies emerge. Subsequent chapters of this thesis demonstrate the transformative potential of multiphoton quantum sensing, elucidating the design, implementation, and experimental results of specific sensing protocols tailored to diverse applications. Our analysis combines experimental observations and theoretical predictions to assess the sensitivity and performance of these protocols. Additionally, the thesis discusses potential future directions and advancements in the field, envisioning applications in biomolecule detection, environmental monitoring, and fundamental studies of light-matter interactions at the nanoscale. Concluding reflections highlight the implications of multiphoton quantum sensing across scientific disciplines and lay the groundwork for future research endeavors.