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Fermat's Spiral-Based Characterization of Squeezed Nonlinear Motional States of Levitated Nanoparticles

Martin Duchaň, Alexandr Jonáš, Radim Filip, Jan Ježek, Petr Jákl, Pavel Zemánek, Martin Šiler

Published Jun 18, 2026• 0 citations
Publisher

Abstract

Abstract A nanoparticle optically levitated in vacuum represents a macroscopic mechanical oscillator that can be virtually decoupled from its thermal environment, providing a unique testbed for exploring the transition between classical and quantum dynamical regimes. It is generally assumed that such a levitated particle is confined and oscillates in a parabolic optical potential where its state is described by a Gaussian distribution in the phase space. However, real-world experiments are performed in optical potentials with weak nonlinear distortions that drive the motion into a non-Gaussian state. Such a state requires additional parameters for the full characterization, and direct quantitative comparison with the ideal Gaussian states is not straightforward. Here, we focus on the most common weak nonlinearity of Duffing type, in which the oscillation frequency decreases with the square of the amplitude of nanoparticle's oscillations. This dependence gives rise to spiral-shaped, squeezed non-Gaussian states. Given the particular observed symmetry of the phase-space distributions, we use the concept of Fermat's spiral and propose a nonlinear transformation of normalized phase-space coordinates that transforms this spiral state into a squeezed Gaussian-like state, which can be directly compared with the states of a stochastic harmonic oscillator. For comparison, we evaluate a nonlinear squeezing metric that can be used also in quantum regimes. The proposed approach can be extended to other nonlinearities of the confining potential with an explicit dependence of the oscillation frequency on the amplitude of the motion.

DOI
10.21203/rs.3.rs-9914417/v1

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Abstract A nanoparticle optically levitated in vacuum represents a macroscopic mechanical oscillator that can be virtually decoupled from its thermal environment, providing a unique testbed for exploring the transition between classical and quantum dynamical regimes. It is generally assumed that such a levitated particle is confined and oscillates in a parabolic optical potential where its state is described by a Gaussian distribution in the phase space. However, real-world experiments are performed in optical potentials with weak nonlinear distortions that drive the motion into a non-Gaussian state. Such a state requires additional parameters for the full characterization, and direct quantitative comparison with the ideal Gaussian states is not straightforward. Here, we focus on the most common weak nonlinearity of Duffing type, in which the oscillation frequency decreases with the square of the amplitude of nanoparticle's oscillations. This dependence gives rise to spiral-shaped, squeezed non-Gaussian states. Given the particular observed symmetry of the phase-space distributions, we use the concept of Fermat's spiral and propose a nonlinear transformation of normalized phase-space coordinates that transforms this spiral state into a squeezed Gaussian-like state, which can be directly compared with the states of a stochastic harmonic oscillator. For comparison, we evaluate a nonlinear squeezing metric that can be used also in quantum regimes. The proposed approach can be extended to other nonlinearities of the confining potential with an explicit dependence of the oscillation frequency on the amplitude of the motion.
Controlling the state of motion of optically levitated nanoparticles is crucial for the advancement of precision sensing, fundamental tests of physics, and the development of hybrid classical-quantum technologies. Experimentally, such control can be achieved by pulsed modifications of the optical potential confining the nanoparticle. Most frequently, the applied potential pulses are parabolic in nanoparticle position, and they expand/squeeze or displace the initial Gaussian state of motion to a modified Gaussian state. The time-dependent mean values and covariance matrix of the phase-space variables can fully characterize such a state. However, quasi-parabolic optical potentials with added weak Duffing-type nonlinearity, encountered in real-world experiments, can generally distort the state of motion to a non-Gaussian one, for which the description based solely on the mean values and covariance matrix fails. Here, we introduce a nonlinear transformation of the phase-space coordinates using the concept of Fermat's spiral, which effectively removes the state distortion induced by the Duffing-type nonlinearity and enables characterization of the state of motion by the standard Gaussian-state metrics. Comparisons of the experimental data with theoretical models show that the proposed coordinate transformation can recover the ideal behavior of a harmonic oscillator even after extended evolution of the system in the nonlinear potential. The presented scheme enables the separation of the effects of the applied state manipulation, the system's gradual thermalization, and the nonlinearity of the confinement on the experimentally observed dynamics of the system, thereby facilitating the design of advanced protocols for levitated optomechanics.
Abstract Processing quantum information on continuous variables requires a highly nonlinear element in order to attain universality. Noise reduction in processing such quantum information involves the use of a nonlinear phase state as a non-Gaussian ancilla. A necessary condition for a nonlinear phase state to implement a nonlinear phase gate is that noise in a selected nonlinear quadrature should decrease below the level of classical states. A reduction of the variance in this nonlinear quadrature below the ground state of the ancilla, a type of nonlinear squeezing, is the resource embedded in these non-Gaussian states and a figure of merit for nonlinear quantum processes. Quantum optomechanics with levitating nanoparticles trapped in nonlinear optical potentials is a promising candidate to achieve such resources in a flexible way. We provide a scheme for reconstructing this figure of merit, which we call nonlinear squeezing, in standard linear quantum optomechanics, analysing the effects of mechanical decoherence processes on the reconstruction and show that all mechanical states which exhibit reduced noise in this nonlinear quadrature are nonclassical.
ABSTRACT Levitodynamics, i.e., the levitation of objects of mesoscopic size has made huge progress in the last decade allowing to address some questions of fundamental physics for the first time. It has become possible to cool a levitated particle of mesoscopic size down to its motional ground state and to observe its motion driven by quantum fluctuations. This defines a quantum system that is ideally suited for an analysis within Nelson's stochastic mechanics approach to quantum mechanics, which allows for a dynamic description of individual particle paths. In good approximation, a levitated nanoparticle is a quantum harmonic oscillator. The coherent states of such an oscillator are superpositions of classical paths and the stochastic ground state process. They are exact solutions not only of the Schrödinger equation but also of the quantum Hamilton equations of Nelson's stochastic mechanics, and they are amenable to path simulations. All model parameters are typically available from experiment. Analyzing the quantum motion of the levitated nanoparticle in terms of the coherent states of a quantum harmonic oscillator allows for a quantitative prediction of the experimentally measured power spectral density of its position fluctuations and predicts new experimentally accessible measures for the mean number of phonons present in the center of mass motion. It also explains the observed phase space trajectory of the nano‐particle during cooling.
Abstract High-order quantum nonlinearity is an important prerequisite for the advanced quantum technology leading to universal quantum processing with large information capacity of continuous variables. Levitated optomechanics, a field where motion of dielectric particles is driven by precisely controlled tweezer beams, is capable of attaining the required nonlinearity via engineered potential landscapes of mechanical motion. Importantly, to achieve nonlinear quantum effects, the evolution caused by the free motion of mechanics and thermal decoherence have to be suppressed. For this purpose, we devise a method of stroboscopic application of a highly nonlinear potential to a mechanical oscillator that leads to the motional quantum non-Gaussian states exhibiting nonclassical negative Wigner function and squeezing of a nonlinear combination of mechanical quadratures. We test the method numerically by analyzing highly instable cubic potential with relevant experimental parameters of the levitated optomechanics, prove its feasibility within reach, and propose an experimental test. The method paves a road for experiments instantaneously transforming a ground state of mechanical oscillators to applicable nonclassical states by nonlinear optical force.
Optomechanics with levitated nanoparticles is a promising way to combine very different types of quantum non-Gaussian aspects induced by continuous dynamics in a nonlinear or time-varying potential with the ones coming from discrete quantum elements in dynamics or measurement. First, it is necessary to prepare quantum non-Gaussian states using both methods. The nonlinear and time-varying potentials have been widely analyzed for this purpose. However, feasible preparation of provably quantum non-Gaussian states in a single mechanical mode using discrete photon detection has not been proposed yet for optical levitation. We explore pulsed optomechanical interactions combined with non-linear photon detection techniques to approach mechanical Fock states and confirm their quantum non-Gaussianity. We also predict the conditions under which the optomechanical interaction can induce multiple-phonon addition processes, which are relevant for nnn-phonon quantum non-Gaussianity. The practical applicability of quantum non-Gaussian states for sensing phase-randomized displacements is shown. Besides such applications, generating quantum non-Gaussian states of levitated nanoparticles can help to study fundamental questions of quantum thermodynamics, and macroscopic quantum effects.