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Journal of Experimental and Theoretical Physics Letters

On Measurement of the Second-Order Coherence of Light–Matter Bose–Einstein Condensates with a Single Detector

Ivan V. Panyukov, E. S. Andrianov

Published Jun 1, 2026• 0 citations
Publisher

Abstract

The second-order autocorrelation function, $${{g}^{{(2)}}}(0)$$ , measured in the Hanbury Brown–Twiss scheme is the strong indicator separating the thermal (incoherent) from the coherent state of light emitted by lasers or photon or polariton condensates. Consequently, $${{g}^{{(2)}}}(0)$$ can be used to determine if the Bose–Einstein condensate forms in the system. The fast dynamics of non-equilibrium light–matter Bose–Einstein condensate make implementing the Hanbury Brown–Twiss scheme challenging and expensive. A good time resolution requires single-photon detectors operating at cryogenic temperatures. An alternative approach to measuring $${{g}^{{(2)}}}(0)$$ , taken in many experiments, is to rely on the scheme with a single detector and measure the intensity fluctuations to directly obtain $${{g}^{{(2)}}}(0)$$ . In this paper, we show that the Hanbury Brown–Twiss scheme and the single detector scheme are not equivalent in the general case because we cannot directly use the intensity fluctuations measured in the single detector scheme to obtain $${{g}^{{(2)}}}(0)$$ of light emitted by a multi-mode system. Nevertheless, we develop a method allowing for the reconstruction of $${{g}^{{(2)}}}(0)$$ from the measurements in the single detector scheme for a multi-mode system with fast thermalization and illustrate it for a special case of non-equilibrium light–matter Bose–Einstein condensate.

DOI
10.1134/s0021364026601016

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This thesis features fundamental experiments on the coherence properties of Bose-Einstein condensates (BEC) and atom lasers, made possible by a newly developed apparatus combining a Bose-Einstein condensate with an ultrahigh nesse optical cavity.Using the cavity as a single atom detector, atoms extracted from a trapped cloud are detected with unprecedented sensitivity, and the rst time-resolved counting of single atoms from a quantum degenerate source was demonstrated.O-diagonal long-range order is a dening property of a BEC and equivalent to longrange phase coherence.Its formation is a complex process accompanied by spontaneous symmetry breaking.We witnessed this formation in an ultracold cloud of 87 Rb atoms crossing the phase transition of BEC.Two overlapping atomic beams originating from dierent positions inside the condensate propagated downwards into the cavity.They showed a matter wave interference pattern with a visibility determined by the coherence of the probed regions.The modulation of the ux of atoms, recorded with single-atom resolution, yields the visibility, whereas its mean value gives information about the density of the sample.By shock cooling, a cloud of atoms was prepared in a highly nonequilibrium state slightly above the phase transition.While the ensemble subsequently relaxed, it crossed the phase transition into an equilibrium with a small condensate fraction.Employing our minimally invasive measurement method, the growth of both the rst-order coherence and the density of the sample was tracked in real time while the system crossed the phase transition.The growth of the coherence was found to start later, proceed faster and nish earlier than the increase in density.The coherent region increased at one fth of the speed of sound.Employing time-resolved single atom counting with the cavity detector, the full counting statistics of an atom laser beam was recorded.In a Hanbury Brown and Twiss type experiment, the second-order correlation function was found to be constant g (2) (τ ) = 1.00±0.01,proving the atom laser's second-order coherence and the absence of excess intensity uctuations that were observed in a pseudothermal beam.An analysis of the time interval distributions of atoms in the beam conrmed these ndings.The iii

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A new method to measure true two-photoncorrelation of soft X-ray synchrotronradiation

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Two-photon correlation measurement provides a promising way to experimentally demonstrate the statistical nature of a light source, which is very significant for the deep understanding of the photon-generating process and the diagnosing of the coherence property. Quantitatively two- photon correlation is described by second-order coherence. Usually the behavior of the second-order coherence against any of the parameters defining the phase volume is different for different photon statistics. The Poisson photon statistics for coherent light gives its second-order coherence as a flat response; The Bose-Einstein photon statistics for chaotic light gives its second-order coherence as a bunching effect; While the Sub-Poisson photon statistics for non-classical light gives its second-order coherence as an anti-bunching effect. 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High-order photon correlations of light fields are important for characterizing the quantum nature. Since Hanbury Brown and Twiss conducted the pioneering experiments in the 1950s, the HBT effect has inspired extensive research on high-order photon correlation in quantum optics, quantum information, and quantum imaging. The Single-photon counting module is one of the most widely used single-photon detectors. Due to its high detection efficiency and low dark counts in the visible and near-infrared region, it is reasonably chosen for basic research on quantum mechanics. Many researches have demonstrated that the maximum value of second-order photon correlation g(2)(τ) at zero delay (τ = 0) can be used to distinguish different light fields. Therefore, the HBT scheme containing two single photon detectors have been widely used in many advanced studies, such as space interference, ghost imaging, single photon detection with high efficiency, etc. However, higher-order photon correlations g(n) (n > 2) can reveal more measurable characteristics of light fields, such as information about the non-Gaussian scattering process, the skewness and kurtosis of photon number distribution, etc. When the extended HBT scheme is used to measure higher-order photon correlations, the experimental conditions including quantum efficiency and background noise greatly affect the photon correlation measurement. The influences of the counting rate and resolution time of the detection system on the measurements are also very important and cannot be ignored. Therefore, the comprehensive considering of various influence factors is necessary for accurately measuring the high-order photon correlations and also a challenge. In this paper, we present a method based on double Hanbury Brown-Twiss scheme for the accurate measuring of high-order photon correlations g(n) (n > 2). The system consists of four single photon counting modules and is used to detect and analyze the joint distribution probability of temporal photon correlation. Considering the effects of the background noise and overall efficiency, theoretically, we analyze the correlations of the third- and fourth-order photon with the incident light intensity, squeezing parameter and photon number respectively for thermal state, coherent state, squeezed vacuum state, and Fock state. Meanwhile, experimentally we study the influences of resolution time and counting rate on correlations of the coherent state and thermal state with third- and fourth-order photon. On condition that the resolution time is 210 ns and the counting rate is 80 kc/s, the correlations of third and fourth-order photon with the thermal state at zero time delay are accurately measured, and the relative statistical deviations of the measured vales from the theoretical values are 0.3% and 0.8%, respectively. In addition, the third- and fourth-order photon correlations of the thermal state at different delay times are also observed. It is demonstrated that the high-order photon correlations of light fields are measured accurately by comprehensively analyzing various influencing factors. This technique provides a promising and useful tool to investigate quantum correlated imaging and quantum coherence of light fields.

Acta Physica Sinica•Jan 1, 2020•3 citations
The second-order autocorrelation function, g(2)(0){{g}^{{(2)}}}(0)g(2)(0) , measured in the Hanbury Brown–Twiss scheme is the strong indicator separating the thermal (incoherent) from the coherent state of light emitted by lasers or photon or polariton condensates. Consequently, g(2)(0){{g}^{{(2)}}}(0)g(2)(0) can be used to determine if the Bose–Einstein condensate forms in the system. The fast dynamics of non-equilibrium light–matter Bose–Einstein condensate make implementing the Hanbury Brown–Twiss scheme challenging and expensive. A good time resolution requires single-photon detectors operating at cryogenic temperatures. An alternative approach to measuring g(2)(0){{g}^{{(2)}}}(0)g(2)(0) , taken in many experiments, is to rely on the scheme with a single detector and measure the intensity fluctuations to directly obtain g(2)(0){{g}^{{(2)}}}(0)g(2)(0) . In this paper, we show that the Hanbury Brown–Twiss scheme and the single detector scheme are not equivalent in the general case because we cannot directly use the intensity fluctuations measured in the single detector scheme to obtain g(2)(0){{g}^{{(2)}}}(0)g(2)(0) of light emitted by a multi-mode system. Nevertheless, we develop a method allowing for the reconstruction of g(2)(0){{g}^{{(2)}}}(0)g(2)(0) from the measurements in the single detector scheme for a multi-mode system with fast thermalization and illustrate it for a special case of non-equilibrium light–matter Bose–Einstein condensate.
The advent of controlled experimental accessibility of Bose-Einstein condensates, as realized with e.g. cold atomic gases, exciton-polaritons, and more recently photons in a dye-filled optical microcavity, has paved the way for new studies and tests of a plethora of fundamental concepts in quantum physics. We here describe recent experiments studying a transition between laser-like dynamics and Bose-Einstein condensation of photons in the dye microcavity system. Further, measurements of the second-order coherence of the photon condensate are presented. In the condensed state we observe photon number fluctuations of order of the total particle number, as understood from effective particle exchange with the photo-excitable dye molecules. The observed intensity fluctuation properties give evidence for Bose-Einstein condensation occurring in the grand-canonical statistical ensemble regime.
Abstract We present an experimental technique that can accurately measure the high-order photon correlations of various light fields based on double Hanbury Brown–Twiss scheme. The system consists of four conventional binary response single-photon counting modules which are non-photon-number-resolving detectors. We theoretically analyze the effects of the experimental conditions on the high-order photon correlations of coherent, chaotic thermal, Fock and squeezed vacuum states with considering the overall efficiency and background noise. In experiment, we determine the proper resolution time from 2 9 = 512 ns to 2 11 = 2048 ns and counting rate from 10 kc s −1 to 100 kc s −1 for characterizing the exact second-, third- and fourth-order photon correlations of chaotic thermal state. At complete time delays, we also observe the third- and fourth-order photon correlations of chaotic thermal state, with the maximum high-order correlation values of 5.99 ± 0.02 and 23.9 ± 0.2 respectively, which are in good agreement with the theoretical values of 6 and 24. The demonstrated experimental technique with high accuracy is a promising tool for investigating quantum optical coherence and ghost imaging.
This thesis features fundamental experiments on the coherence properties of Bose-Einstein condensates (BEC) and atom lasers, made possible by a newly developed apparatus combining a Bose-Einstein condensate with an ultrahigh nesse optical cavity.Using the cavity as a single atom detector, atoms extracted from a trapped cloud are detected with unprecedented sensitivity, and the rst time-resolved counting of single atoms from a quantum degenerate source was demonstrated.O-diagonal long-range order is a dening property of a BEC and equivalent to longrange phase coherence.Its formation is a complex process accompanied by spontaneous symmetry breaking.We witnessed this formation in an ultracold cloud of 87 Rb atoms crossing the phase transition of BEC.Two overlapping atomic beams originating from dierent positions inside the condensate propagated downwards into the cavity.They showed a matter wave interference pattern with a visibility determined by the coherence of the probed regions.The modulation of the ux of atoms, recorded with single-atom resolution, yields the visibility, whereas its mean value gives information about the density of the sample.By shock cooling, a cloud of atoms was prepared in a highly nonequilibrium state slightly above the phase transition.While the ensemble subsequently relaxed, it crossed the phase transition into an equilibrium with a small condensate fraction.Employing our minimally invasive measurement method, the growth of both the rst-order coherence and the density of the sample was tracked in real time while the system crossed the phase transition.The growth of the coherence was found to start later, proceed faster and nish earlier than the increase in density.The coherent region increased at one fth of the speed of sound.Employing time-resolved single atom counting with the cavity detector, the full counting statistics of an atom laser beam was recorded.In a Hanbury Brown and Twiss type experiment, the second-order correlation function was found to be constant g (2) (τ ) = 1.00±0.01,proving the atom laser's second-order coherence and the absence of excess intensity uctuations that were observed in a pseudothermal beam.An analysis of the time interval distributions of atoms in the beam conrmed these ndings.The iii
Introduction The degree of first-order temporal coherence, a function denoted by g (1) ( τ ), provides information about the coherence length and the power spectral density of a light source. However, without additional information, g (1) ( τ ) has no bearing on intensity fluctuations and higher-order statistics of the emitted light. A quasi-monochromatic laser beam and the beam of light from an incandescent light bulb, provided that the latter is properly filtered to match the spectral line-shape of the former, will have identical degrees of first-order coherence. Any interferometric experiment involving the splitting and superposition of amplitudes would yield identical results for the laser beam and the (properly filtered) thermal light. Therefore, on the basis of such experiments alone, there is no way to distinguish the two light sources. It turns out, however, that the intensity fluctuations of laser light are fundamentally different from those of thermal light. The two sources can, therefore, be distinguished based on their second-order coherence properties. An ideal photodetector produces an electrical signal proportional to the “cycle-averaged intensity” of the E -field (or B -field) of the light beam at the location of the detector. Assuming that the electrical bandwidth of the detector (including all associated circuitry) is greater than the bandwidth of the incident light wave by at least a factor of 2, the output of the detector should accurately represent the intensity fluctuations of the light beam as a function of time.
Two-photon correlation measurement provides a promising way to experimentally demonstrate the statistical nature of a light source, which is very significant for the deep understanding of the photon-generating process and the diagnosing of the coherence property. Quantitatively two- photon correlation is described by second-order coherence. Usually the behavior of the second-order coherence against any of the parameters defining the phase volume is different for different photon statistics. The Poisson photon statistics for coherent light gives its second-order coherence as a flat response; The Bose-Einstein photon statistics for chaotic light gives its second-order coherence as a bunching effect; While the Sub-Poisson photon statistics for non-classical light gives its second-order coherence as an anti-bunching effect. Therefore the measurement of two-photon correlation is proved to be a good finger print to check whether light is in coherent state or incoherent state such as thermal state or non-classical state. Historically the measurement of two-photon correlation was first performed by Hanbury-Brown and Twiss (HBT) in 1956. They used a linear mixer to realize the correlation of the two currents from the photoelectric detectors illuminated by a stationary thermal light souece, a mercury arc, and the photo-bunching effect was first successfully observed in the visible region of 435.8 nm. HBT method is no doubt a good way to extract the small excess two-photon correlation for a stationary light because the background, that is the DC components, has been cut off automatically by the broad band amplifiers, which is in fact the key of the success of HBT experiment. However there exists a general problem, to which no attention has ever been paid, in measuring the two-photon correlation of non-stationary light such as synchrotron radiation (SR) by the HBT method. Here the "non-stationary" means a sense of classical mechanics that the observed intensity has some deterministic time structure. The systematic time structure of SR decided by the bunch distribution of the electric current in a storage ring will give rise to a large amount of unexpected accidental correlation, which in fact has nothing to do with the inherent photon statistics of light source and usually l000～l0000 times larger than the true two-photon correlation due to the short bunch separation length (2ns) and the short coherence time (～0.1ps) which is not comparable to the time resolution (1ns) of the measuring system. The existence of the accidental correlation would severely prevent us from observing the bunching effect of the true two-photon correlation. Therefore to suppress the much larger accidental correlation and to extract the small true two-photon correlation, a novel intensity interferometer has been developed for soft X-ray synchrotron radiation. This intensity interferometer consists of an optical vacuum chamber and an electric correlator. All the essential optical elements which includes a wire scanner, a precise diffraction slit, a grating monochromator with a coherence time modulator, a beam divider and two fast-response photon detectors (microchannel plates) are mounted in this high vacuum chamber. The electric correlator completes the multiplication of the two broad band electric currents coming from the photoelectric detectors. The basic idea to suppress the much larger accidental correlation is to modulate the coherence time by modulating the entrance slit width of the monochromator by a piezoclectric translator. The two sets of light intensity are simultaneously modulated too. When the frequency of modulation is f, the third harmonics 3f is detected with a loch-in amplifier because the 3f components include only the true two-photon correlation. Practically it is difficult to modulate with frequency f without any higher order harmonics distortion which might add some false 3f components. To overcome this difficulty we have used a sharp bandpass filter of l00～350 MHz in each branch of the correlator, which is lower than the RF frequency 500 MHz and much higher than 1.6 MHz, the revolution frequency of the stored beam of the 2.5 GeV storage ring. This new apparatus has been operated successfully in the measurement of the horizontal two-photon correlation for the first harmonic of undulator radiation with photon energy of 70 eV at the Photon Factory, KEK. By narrowing the precise slit width which correspondingly changes the spatial coherence of the incident SR, a bunching effect of the normalized excess two-photon correlation has been clearly observed. This explicit bunching effect implies that synchrotron radiation is chaotic radiation. Further investigation shows that although second-order coherence is completely determined by the first-order coherence for the case of chaotic light, the measured information from the light source is essentially different. The two-photon correlation of synchrotron radiation does not depend on the response time of the detectors but gives the information of instantaneous emittance of the stored beam with the time scale of coherence time τC. By fitting the experimental data, the horizontal instantaneous emittance of the stored beam is estimated to be 40nmrad. This intensity interferometer can be utilized to characterize the coherence properties of incomplete FELs, such as SASE, because if they are fully coherent light sources the normalized excess two-photon correlation would have a flat response, but not showing a photon-bunching effect.
High-order photon correlations of light fields are important for characterizing the quantum nature. Since Hanbury Brown and Twiss conducted the pioneering experiments in the 1950s, the HBT effect has inspired extensive research on high-order photon correlation in quantum optics, quantum information, and quantum imaging. The Single-photon counting module is one of the most widely used single-photon detectors. Due to its high detection efficiency and low dark counts in the visible and near-infrared region, it is reasonably chosen for basic research on quantum mechanics. Many researches have demonstrated that the maximum value of second-order photon correlation g(2)(τ) at zero delay (τ = 0) can be used to distinguish different light fields. Therefore, the HBT scheme containing two single photon detectors have been widely used in many advanced studies, such as space interference, ghost imaging, single photon detection with high efficiency, etc. However, higher-order photon correlations g(n) (n > 2) can reveal more measurable characteristics of light fields, such as information about the non-Gaussian scattering process, the skewness and kurtosis of photon number distribution, etc. When the extended HBT scheme is used to measure higher-order photon correlations, the experimental conditions including quantum efficiency and background noise greatly affect the photon correlation measurement. The influences of the counting rate and resolution time of the detection system on the measurements are also very important and cannot be ignored. Therefore, the comprehensive considering of various influence factors is necessary for accurately measuring the high-order photon correlations and also a challenge. In this paper, we present a method based on double Hanbury Brown-Twiss scheme for the accurate measuring of high-order photon correlations g(n) (n > 2). The system consists of four single photon counting modules and is used to detect and analyze the joint distribution probability of temporal photon correlation. Considering the effects of the background noise and overall efficiency, theoretically, we analyze the correlations of the third- and fourth-order photon with the incident light intensity, squeezing parameter and photon number respectively for thermal state, coherent state, squeezed vacuum state, and Fock state. Meanwhile, experimentally we study the influences of resolution time and counting rate on correlations of the coherent state and thermal state with third- and fourth-order photon. On condition that the resolution time is 210 ns and the counting rate is 80 kc/s, the correlations of third and fourth-order photon with the thermal state at zero time delay are accurately measured, and the relative statistical deviations of the measured vales from the theoretical values are 0.3% and 0.8%, respectively. In addition, the third- and fourth-order photon correlations of the thermal state at different delay times are also observed. It is demonstrated that the high-order photon correlations of light fields are measured accurately by comprehensively analyzing various influencing factors. This technique provides a promising and useful tool to investigate quantum correlated imaging and quantum coherence of light fields.