The spin dynamics of two alkali-metal atoms in an optical tweezer is driven by spin-changing collisions that couple the spin state of the atoms to their relative motion. This paper experimentally studies the resulting spin states when the relative motion is in a thermal state with kBT much larger than the energies of the spin states that take part in the dynamics. We find that an initially unentangled spin state can evolve into an entangled state. This is contrary to the common case when coupling a quantum system to hot degrees of freedom leads to loss of entanglement and not its generation. Moreover, we show that the generated entanglement is technologically useful as it, in principle, can enhance the sensitivity of measurements beyond the standard quantum limit. This may provide a promising avenue for robust entanglement generation for future technologies.
The spin dynamics of two alkali-metal atoms in an optical tweezer is driven by spin-changing collisions that couple the spin state of the atoms to their relative motion. This paper experimentally studies the resulting spin states when the relative motion is in a thermal state with kBT much larger than the energies of the spin states that take part in the dynamics. We find that an initially unentangled spin state can evolve into an entangled state. This is contrary to the common case when coupling a quantum system to hot degrees of freedom leads to loss of entanglement and not its generation. Moreover, we show that the generated entanglement is technologically useful as it, in principle, can enhance the sensitivity of measurements beyond the standard quantum limit. This may provide a promising avenue for robust entanglement generation for future technologies.
The spin-dynamics of two alkali atoms in an optical tweezer is driven by spin-changing collisions that couple the spin-state of the atoms to their relative motion. This paper experimentally studies the resulting spin-states when the relative motion is in a thermal state with k B T much larger than the energies of the spin-states that take part in the dynamics. We find that an initially unentangled spin-state can evolve into an entangled state. This is contrary to the common case when coupling a quantum system to hot degrees of freedom leads to loss of entanglement and not its generation. Moreover, we show that the generated entanglement is technologically useful as it, in principle, can enhance the sensitivity of measurements beyond the standard quantum limit. This may provide a promising avenue for robust entanglement generation for future technologies.
A significant challenge in atomic physics is the precise preparation, manipulation, and measurement of the quantum-mechanical states of physical systems. One intriguing aspect of multi-particle quantum states is entanglement. Entanglement is of high interest for conducting non-classical computations, particularly in the application of quantum information, and the enhancement of measurements through entanglement. Spin-entangled states in many-body systems have been engineered and verified via spin-changing collisions. Using optical tweezers to isolate individual atomic pairs provides a unique avenue for investigating spin-changing collisions and the entangled states at the particle level. Up until now, the entanglement for an atomic pair has been achieved with groundstate-cooled atoms. The ability to generate entanglement at a higher temperature would be a step forward to robust practical applications in real world scenarios.
Abstract The complex collisional properties of atoms fundamentally limit investigations into a range of processes in many-atom ensembles. In contrast, the bottom-up assembly of few- and many-body systems from individual atoms offers a controlled approach to isolating and studying such collisional processes. Here, we use optical tweezers to individually assemble pairs of trapped 85Rb atoms, and study the spin dynamics of the two-body system in a thermal state. The spin-2 atoms show strong pair correlation between magnetic sublevels on timescales exceeding one second, with measured relative number fluctuations 11.9 ± 0.3 dB below quantum shot noise, limited only by detection efficiency. Spin populations display relaxation dynamics consistent with simulations and theoretical predictions for 85Rb spin interactions, and contrary to the coherent spin waves witnessed in finite-temperature many-body experiments and zero-temperature two-body experiments. Our experimental approach offers a versatile platform for studying two-body quantum dynamics and may provide a route to thermally robust entanglement generation.
The predictions of quantum mechanics often differ from our everyday experiences. In the classical case, the state of a system can be predicted precisely, assuming the exact knowledge of all parameters. This is not possible in quantum mechanics. For example, the spin of one particle can be simultaneously in two different states, until a measurement defines the actual state. If multiple particles are in such superposition states, their spins can be coupled with each other such that the measurement of one particle changes the physical state of the other particles. This coupling effect is a fundamental part of quantum mechanics and is called entanglement. It is a central requirement for applications in the fields of quantum communication, quantum cryptography and quantum computing. One possibility to create entanglement are spin-changing collisions in a spinor Bose-Einstein condensate. These collisions are described by a nonlinear process, which creates non-classical correlations between all atoms of the Bose-Einstein condensate. Within this thesis, 87Rb spinor Bose-Einstein condensates are used to demonstrate Einstein-Podolsky-Rosen entanglement by the generation and analysis of a two-mode entangled state in spin space [A1]. These states are applied in an interferometric measurement with a resolution of 2.05+0.34 -0.37 dB beyond the standard quantum limit [A2]. Depending on the dynamics, the process can also be analogous to the dynamical Casimir effect [A3]. The entanglement between the particles in these publications is strongly connected with their indistinguishability. It is thus possible to make the particles distinguishable again and recover the entanglement between the now separated particles? This question is approached by cutting an entangled state of indistinguishable particles into two spatially separated atomic modes - creating a two-mode entangled state in real space. As shown in Ref. [A4], the entanglement between the two separated clouds of a Bose-Einstein condensate can be measured directly. In the future, the created state can be employed for a test of quantum nonlocality.
Abstract Quantum technologies use entanglement to outperform classical technologies, and often employ strong cooling and isolation to protect entangled entities from decoherence by random interactions. Here we show that the opposite strategy—promoting random interactions—can help generate and preserve entanglement. We use optical quantum non-demolition measurement to produce entanglement in a hot alkali vapor, in a regime dominated by random spin-exchange collisions. We use Bayesian statistics and spin-squeezing inequalities to show that at least 1.52(4) × 1013 of the 5.32(12) × 1013 participating atoms enter into singlet-type entangled states, which persist for tens of spin-thermalization times and span thousands of times the nearest-neighbor distance. The results show that high temperatures and strong random interactions need not destroy many-body quantum coherence, that collective measurement can produce very complex entangled states, and that the hot, strongly-interacting media now in use for extreme atomic sensing are well suited for sensing beyond the standard quantum limit.
Polar molecules are a promising platform for quantum-enhanced sensing and precision tests of fundamental physics, owing to their strong long-range dipolar interactions, broad sensitivity to electromagnetic fields, and sensitivity to potential physics beyond the Standard Model. However, the creation of metrologically useful entangled states in molecular systems has remained elusive. Here, we report the first observation of a class of metrologically useful entangled states - spin-squeezed states - in polar CaF molecules trapped in an optical tweezer array. The spin degree of freedom is encoded in rotational levels which are directly coupled by dipolar exchange interactions. By harnessing appropriate dynamical decoupling schemes we observe up to 3.0(3)dB of metrological gain, (2.2(3)dB without measurement correction) from direct exchange interactions. Using Floquet engineering, we further realize richer Hamiltonians that preserve spin squeezing while enabling the development of longer-range quantum correlations. Using site- and spin-resolved measurements we demonstrate that these entangled states enhance sensitivity to both homogeneous and spatially varying fields, and reveal strong non-classical correlations, including bipartite entanglement and Einstein-Podolsky-Rosen steering. Finally, we transfer the spin-squeezed states into long-lived and non-interacting hyperfine states, where the metrological enhancement persists for up to 100ms. Our results establish molecular optical tweezer arrays as a scalable platform for generating, controlling, characterizing, and storing entangled states of molecules, opening new opportunities for quantum-enhanced sensing and precision tests of fundamental physics.