The precise control of quantum systems enables the development of a wide range of promising quantum technologies. These technologies allow for beating the limits of their classical pendants and outperform them in various tasks. This thesis employs and expands a variety of methods and concepts of optimal control theory in order to address different problems in quantum technologies and work towards their realization. Schrödinger cat states present a particularly versatile set of states, that have a broad range of applications for all types of quantum technologies. We employ optimal control theory to investigate how cat states can be prepared in different physical systems. This allows us to investigate the role of higher order nonlinearities in anharmonic resonators. Further, this enables the identification of strategies for cat state preparation in the presence of higher order anharmonicities and an analysis if they can be exploited as resource. Additionally, we develop a set of functionals, which allow for optimizing towards arbitrary cat states. This facilitates the preparation of cat states even in systems, where the reachable set of states is not immediately apparent. Quantum computing is a particularly prominent quantum technology and promises a completely new paradigm for computing. Crosstalk, the undesired interaction between different parts of a quantum processor, poses a major challenge across various architectures. Therefore, we utilize concepts from optimal control to introduce the perfect entangler spectrum as a tool to detect operational crosstalk, caused by spectator qubits. This allows us to identify parameter regimes of superconducting qubits, which exhibit crosstalk and determine the underlying mechanisms. In addition, we utilize optimal control and parameter optimizations to explore mitigation strategies for the different crosstalk mechanisms. Our work paves the way for systematically eliminating crosstalk, when scaling up quantum computing architectures.
The precise control of quantum systems enables the development of a wide range of promising quantum technologies. These technologies allow for beating the limits of their classical pendants and outperform them in various tasks. This thesis employs and expands a variety of methods and concepts of optimal control theory in order to address different problems in quantum technologies and work towards their realization. Schrödinger cat states present a particularly versatile set of states, that have a broad range of applications for all types of quantum technologies. We employ optimal control theory to investigate how cat states can be prepared in different physical systems. This allows us to investigate the role of higher order nonlinearities in anharmonic resonators. Further, this enables the identification of strategies for cat state preparation in the presence of higher order anharmonicities and an analysis if they can be exploited as resource. Additionally, we develop a set of functionals, which allow for optimizing towards arbitrary cat states. This facilitates the preparation of cat states even in systems, where the reachable set of states is not immediately apparent. Quantum computing is a particularly prominent quantum technology and promises a completely new paradigm for computing. Crosstalk, the undesired interaction between different parts of a quantum processor, poses a major challenge across various architectures. Therefore, we utilize concepts from optimal control to introduce the perfect entangler spectrum as a tool to detect operational crosstalk, caused by spectator qubits. This allows us to identify parameter regimes of superconducting qubits, which exhibit crosstalk and determine the underlying mechanisms. In addition, we utilize optimal control and parameter optimizations to explore mitigation strategies for the different crosstalk mechanisms. Our work paves the way for systematically eliminating crosstalk, when scaling up quantum computing architectures.
The recently emerged field of quantum technology is aiming to employ quantum coherence and entanglement for realization of next generation sensors, standards, imaging systems, secure communication and computers.Although applications of quantum technologies cover a broad spectrum and their development stage varies from early demonstrations to commercially available devices, many challenges have been identified.The first includes tailoring materials for quantum technologies, which is playing an essential role in technological applications of quantum science.Solid state systems allowing long coherence time are essential for quantum computation and quantum sensing.Ultrapure materials with tailored isotopic content are important for reaching long coherence time of spin qubits (Awschalom et al., 2013).The ability to place single dopants with high precision and form spin qubits at desired location is essential for both quantum computing and quantum sensing applications (McCallum et al., 2012;Smith et al., 2019).The performance of different types of qubits is usually benchmarked in terms of controllability and coherence time.Usually solid-state systems allow fast control, but exhibit fast decoherence owing to complex environment.It is therefore important to search for new types of qubits combining isolation from environment and access via fast coherent control and readout.Novel approaches combining different quantum systems into build hybrid quantum devices for optimal performance is a promising avenue.Examples of such hybrid approaches are spin systems coupled to superconducting qubits (Kubo et al., 2011) and hybrid nuclear-electronic qubits (Morley et al., 2013).Optimal protocols for quantum technologies requires extension of coherence time of qubits beyond the coherence time of the isolated quantum system.The efficient protection toolkit includes dynamical decoupling (Yang et al., 2011) and quantum error correction (Terhal, 2015) based techniques.Although general principles of qubits protection were developed and tested experimentally in different model environments, it is essential to adapt them to realistic environmental noise.In the field of quantum sensing, it is also essential to combine protections against noise with non-reduced sensing performance.Experimental imperfections can be addressed using optimal control tools (Glaser et al., 2015).The development of efficient quantum algorithms is another growing field belonging to quantum software area.On one hand, it is essential to find problems where a quantum computer can outperform classical computers.On the other hand, it is essential to develop an application scenario for a limited number of qubits (Montanaro, 2016).In addition, in order to develop new algorithms, future work must include discoveries of application scenarios of already known algorithms.Application of quantum Fourier transform for sensing is a promising example of such new applications (Vorobyov et al., 2021).Signal processing is another field of quantum software that is becoming essential in applications.Advanced signal analysis protocols, like quantum compressed sensing, can be employed to quantify entanglement in large quantum devices via efficient quantum tomography (Riofrío et al., 2017).
For several decades it has been appreciated that quantum computers hold incredible promise to perform calculations intractable to classical computation. However, this promise has be slow to realize. Dozens of quantum systems are currently being investigated for use in quantum information processing - none of which have yet demonstrated algorithms involving more than a handful of qubits and it remains unclear which, if any, of these systems will ultimately compose a scalable, robust quantum information processing architecture. In this thesis we employ analytical, optimal and algebraic control techniques to evaluate various quantum systems for their potential use in quantum information processing. In doing so, we have additionally identified several novel characterization procedures capable of probing both the coherent and incoherent dynamics of quantum systems. The first part of this thesis discusses work motivated by attempts to utilize donor qubits in silicon as quantum bits. We first propose a measurement of the state of a single donor electron spin using two-dimensional electron gas of a field-effect transistor and electrically detected magnetic resonance. We analyze the potential sensitivity of this measurement and show that it is a quantum nondemolition measurement of an electron-encoded state. We then present the first of two novel qubit characterization procedures. We consider the problem of rapidly characterizing a large number of similarly prepared qubits using techniques from optimal experiment design. All qubits are assumed to evolve according to the same physical processes, though the Hamiltonian parameters may vary from device to device - an inevitability in solid state qubits. We use the Cram\\'er-Rao bound on the variance of a point estimator to construct the optimal series of experiments to estimate these free parameters, and present a complete analysis of the optimal experimental configuration. Though applied to dipole- and exchange-coupled qubits, this technique is widely applicable to other systems. The second part of the thesis discusses the role that control can play in measuring and mitigating noise in qubit systems. Our first result describes a method for quickly simulating the effects of arbitrary markovian noise on qubit systems through the use of a numerically optimized, multi-state Markovian fluctuator. This ability to rapidly simulate the noisy qubit evolution allows us to compute control sequences capable of maximally decoupling the qubit from the noise source. We then introduce the second characterization procedure of the these, showing that a single measurable and controllable qubit may act as a spectrometer of dephasing noise. We show that the formalism of dynamical decoupling can be used to estimate the short-time correlation function of the noise source, while long time correlations may be estimated by a very simple series of free evolution experiments. This technique is applicable to the wide range of physical implementations which suffer from dephasing noise.The final part of this thesis demonstrates that trapped neutral atoms may be utilized for the robust simulation of complex systems exhibiting a topological phase. We present a method to simulate the toric code Hamiltonian stroboscopically, and demonstrate that our technique preserves the ground state degeneracy . Furthermore, we introduce a dissipative mechanism allowing for thermalization of the system to a finite temperature or direct cooling to the ground state manifold.
It is control that turns scientific knowledge into useful technology: in physics and engineering it provides a systematic way for driving a dynamical system from a given initial state into a desired target state with minimized expenditure of energy and resources. As one of the cornerstones for enabling quantum technologies, optimal quantum control keeps evolving and expanding into areas as diverse as quantum-enhanced sensing, manipulation of single spins, photons, or atoms, optical spectroscopy, photochemistry, magnetic resonance (spectroscopy as well as medical imaging), quantum information processing and quantum simulation. In this communication, state-of-the-art quantum control techniques are reviewed and put into perspective by a consortium of experts in optimal control theory and applications to spectroscopy, imaging, as well as quantum dynamics of closed and open systems. We address key challenges and sketch a roadmap for future developments.
This thesis addresses the of developing a counter-part of the well established classical theory of control. We dwell on the fundamental fact that states are generally not perfectly distinguishable, and measurements typically introduce noise in the system being measured. Because of these, it is generally not clear whether the central concept of the classical control theory --- that of observing the system and then applying feedback --- is always useful in the setting. We center our investigations around the of transforming the state of a system into a given target state, when the system can be prepared in different ways, and the target state depends on the choice of preparation. We call this the quantum tracking problem and show how it can be formulated as an optimization that can be approached both numerically and analytically. This provides a simple route to the characterization of the trade-off between information gain and disturbance, and is seen to have several applications in information. In order to characterize the optimality of our tracking procedures, some figure-of-merit has to be specified. Naturally, distance measures for states are the ideal candidates for this purpose. We investigated several possibilities, and found that there is usually a compromise between physically motivated and mathematically tractable measures. We also introduce an alternative to the Uhlmann-Jozsa fidelity for mixed states, which besides reproducing a number of properties of the standard fidelity, is especially attractive because it is simpler to compute. We employ some ideas of convex analysis to construct optimal control schemes analytically. In particular, we obtain analytic forms of optimal controllers for stabilizing and tracking any pair of states of a single-qubit. In the case of stabilization, we find that feedback control is always useful, but because of the trade-off between information gain and disturbance, somewhat different from the type of feedback performed in classical systems. In the case of tracking, we find that feedback is not always useful, meaning that depending on the choice of states one wants to achieve, it may be better not to introduce any noise by the application of measurements. We also demonstrate that our optimal controllers are immediately applicable in several information applications such as state-dependent cloning, purification, stabilization, and discrimination. In all of these cases, we were able to recover and extend previously known optimal strategies and performances. Finally we show how optimal single-step control schemes can be concatenated to provide multi-step strategies that usually over-perform optimal control protocols based on a single interaction between the controller and the system.
This paper explores the integration of nonlinear control theory with quantum system modeling, presenting a novel approach to designing and optimizing control strategies for quantum systems. The core claim centers on leveraging the optimization techniques within nonlinear control theory to address the inherent complexities of quantum system dynamics. The mechanism involves formulating quantum systems' nonlinear dynamics into equivalent control problems, subsequently employing nonlinear control theory's optimization methods for solution. This combined approach promises enhanced precision and efficiency in quantum system control. The work demonstrates a theoretical framework for tackling this challenge, paving the way for future research and practical applications in areas such as quantum computing and quantum sensing. The key mathematical concepts utilized are presented, including Hamiltonian formalism, Liouville-Perron equation, and nonlinear control theory formulations. The final results offer a pathway to more effective manipulation of quantum states.
Precisely characterizing and controlling the dynamics of realistic open quantum systems has emerged in recent years as a key challenge across contemporary quantum sciences and technologies, with implications ranging from physics, chemistry and applied mathematics to quantum information processing (QIP) and quantum engineering. Quantum control theory aims to provide both a general dynamical-system framework and a constructive toolbox to meet this challenge. The purpose of this special issue of Journal of Physics B: Atomic, Molecular and Optical Physics is to present a state-of-the-art account of recent advances and current trends in the field, as reflected in two international meetings that were held on the subject over the last summer and which motivated in part the compilation of this volume—the Topical Group: Frontiers in Open Quantum Systems and Quantum Control Theory , held at the Institute for Theoretical Atomic, Molecular and Optical Physics (ITAMP) in Cambridge, Massachusetts (USA), from 1–14 August 2010, and the Safed Workshop on Quantum Decoherence and Thermodynamics Control , held in Safed (Israel), from 22–27 August 2010. Initial developments in quantum control theory date back to (at least) the early 1980s, and have been largely inspired by the well-established mathematical framework for classical dynamical systems. As the above-mentioned meetings made clear, and as the burgeoning body of literature on the subject testifies, quantum control has grown since then well beyond its original boundaries, and has by now evolved into a highly cross-disciplinary field which, while still fast-moving, is also entering a new phase of maturity, sophistication, and integration. Two trends deserve special attention: on the one hand, a growing emphasis on control tasks and methodologies that are specifically motivated by QIP, in addition and in parallel to applications in more traditional areas where quantum coherence is nevertheless vital (such as, for instance, quantum control of chemical reactions or high-resolution magnetic resonance spectroscopy); on the other hand, an unprecedented demand for close coupling between theory and experiment , with theoretical developments becoming more and more attuned to and driven by experimental advances as different quantum technologies continue to evolve at an impressive pace in the laboratory. Altogether, these two trends account for several of the recurrent themes in this volume, as well as in the current quantum control literature as a whole: namely, the quest for control strategies that can attain the highest degree of precision and robustness possible, while striving for efficiency and, ultimately, optimality in achieving the intended control task under realistic operational constraints. From a theory standpoint, this makes it imperative to take into account increasingly more realistic control settings; to assess the quantitative impact of limited control resources and/or system knowledge; and to provide a rigorous and general foundation for existing experimental approaches in order to further enhance applicability and performance. From an experimental standpoint, renewed emphasis is in turn placed on validating theoretical predictions and benchmarking performance, so that the limiting constraints can be singled out for additional theoretical analysis and guidance. This ongoing cross-talk is clearly reflected in this collection, which brings together theoreticians and experimentalists, with a significant fraction of the papers reporting on combined quantum control theory–experiment efforts. While a precise categorization would neither be possible nor desirable, contributions to this volume have been loosely grouped into five broad sections. This grouping has been made in the hope that connections between different problems and/or technical approaches will become more transparent, facilitating the transfer of concepts and methods. The special issue opens with a section devoted to open-loop control methods, with special emphasis on dynamical decoupling (DD), which is becoming an increasingly important tool for decoherence control at the physical 'quantum firmware' level. In addition to including original research results, the first two articles, by Brion et al and Biercuk et al , also serve to pedagogically review some background in their respective subjects. In particular, Brion et al revisit one of the conceptually simplest approaches to open-loop manipulation of both closed and open quantum systems, nonholonomic control , motivated by its broad applicability to QIP settings. A special instance of open-loop control based on sequences of (nearly) instantaneous `bang-bang' pulses is addressed by Biercuk et al , who reformulate the simplest DD scenario, suppression of phase decoherence in a single qubit, as a filter-design problem. Peng et al report on the implementation of 'concatenated' DD for arbitrary single-qubit decoherence in the context of nuclear magnetic resonance QIP. A dedicated analysis of the performance of different DD schemes in the presence of realistic pulse errors is given by Wang and Dobrovitski. DD is also one of the strategies used by Lucamarini et al to reduce polarization decoherence in a photon qubit. These authors additionally report on the use of active feedback to counter transmission noise, effectively setting the stage for the second section, which is centered on closed-loop control. Unlike in open-loop control, measurement is an essential ingredient in closed-loop schemes aimed at both reliably identifying features of the target quantum system and further modifying its dynamics. The importance of directly measuring the spectrum of the underlying system-environment coupling is stressed by Almog et al , who show how this knowledge is crucial, in particular, for predicting the performance of DD sequences in experiments and for optimizing performance. Riofrio et al address a weak-measurement protocol for implementing quantum state tomography , which is a necessary 'primitive' for inferring the target quantum state and thereby diagnosing the control performance. Next, the impact of realistic control and system imperfections in continuous-time Markovian feedback strategies for rapid state preparation is analyzed by Combes and Wiseman. A prominent role is played in the special issue by optimal control (OC) approaches, reflecting their central importance for quantum control and QIP. The OC contributions have been divided into two separate sections, depending on whether the target dynamics is modeled as Hamiltonian (section 3) or dissipative (section 4), respectively. The contribution by Beltrani et al deals with `control landscapes', which provide a foundation for analyzing the performance of numerical OC algorithms and their robustness against control errors. Specifically, this paper characterizes geometric properties of the control landscape, relevant to the optimal control of state-to-state transitions. Application of OC theory to the problem of population transfer and coherence enhancement in Λ-systems is studied by Kumar et al , whereas Goerz et al report on the OC-design of a high-fidelity controlled phase-gate in atomic qubits. The robustness of an OC solution is specifically addressed by Negretti et al , along with an approach for identifying easily implementable while still 'close-to-optimal' control pulses. Powerful relaxation-optimized OC schemes (based on so-called opengrape algorithms) for generating unitary target gates in the presence of known dissipation parameters are discussed by Schulte-Herbrüggen et al . Next, Lapert et al report on the problem of time-optimal control of spin-1/2 systems undergoing Bloch relaxation dynamics, highlighting the crucial role played by singular extremals in the control synthesis. Alternative approaches for optimized control of qubits exposed to various decoherence processes are developed by Esher et al and Xue et al , based on a perturbative 'bath-optimized' formalism and on numerical optimization via a genetic algorithm, respectively. Testifying to the richness of the field, the volume concludes with four contributions that address a diverse range of problems. The exploitation of properties of adiabatic quantum evolutions is common to the first two papers. In particular, Legthtas et al offer a rigorous explanation for the robustness of a control protocol, chirped pulsing , that is widely employed in 'adiabatic rapid passage' experiments, while Han et al present a theoretical framework for adiabatic Raman photo-association schemes relevant to ultracold atomic systems. In the context of cavity quantum electrodynamics, Montenegro and Orszag describe how to engineer a system of two atoms coupled to distant lossy cavities so that stable atomic entanglement is generated. Finally, still very little is known about the physical mechanisms that are responsible for and control the experimentally observed 'coherent' features of transport phenomena in biological systems. The last contribution by Alicki and Giraldi analyzes energy transport in dynamical systems that can be modeled as 'quantum networks', and points to this fascinating emerging frontier. It is our hope that the above papers may help readers to gain an overview of some of the main trends in current quantum control efforts, both theoretical and experimental. In closing, we take the opportunity to thank the organizations which sponsored the above-mentioned ITAMP Topical Group (the United States National Science Foundation and Harvard University) and the Safed Workshop (the Israeli Science Foundation, the Safed Scientific Workshop program, CECAM and ACAM). Last but not least our sincere gratitude goes to all of the contributors to the volume and the reviewers as well as the J. Phys. B staff, for their respective efforts in preparing the papers and ensuring the overall quality of this special issue.