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Physica D Nonlinear Phenomena

Quantum vs. classical spin: A comparative study of dipolar spin dynamics and the onset of chaos

Victor K. Henner, ALEXANDER A. NEPOMNYASHCHY, Tatyana Belozerova

Published Apr 19, 2026• 0 citations
Publisher
DOI
10.1016/j.physd.2026.135251

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We investigate the spin dynamics of a dipole-coupled system by comparing a direct solution of the Schrodinger equation for quantum spins with simulations of classical spins. Although classical spins have long been used in microscopic spin dynamics simulations, we demonstrate that their results differ significantly from those of quantum spins. Using Free Induction Decay as a benchmark, we find that while the overall patterns are qualitatively similar, significant discrepancies emerge at both short and long timescales. We trace these differences to fundamental distinctions in the two descriptions.
We investigate the onset of chaos in a periodically kicked Dicke model (KDM), using the out-of-time-order correlator (OTOC) as a diagnostic tool, in both the oscillator and the spin subspaces. In the large spin limit, the classical Hamiltonian map is constructed, which allows us to investigate the corresponding phase space dynamics and to compute the Lyapunov exponent. We show that the growth rate of the OTOC for the canonically conjugate coordinates of the oscillator is able to capture the Lyapunov exponent in the chaotic regime. The onset of chaos is further investigated using the saturation value of the OTOC, that can serve as an alternate indicator of chaos in a generic interacting quantum system. This is also supported by a system independent effective random matrix model. We further identify the quantum scars in KDM and detect their dynamical signature by using the OTOC dynamics. The relevance of the present study in the context of ongoing cold atom experiments is also discussed.
An extension of the concept of Kolmogorov entropy to quantum mechanical systems is given. Using the Kolmogorov entropy as a common basis for discussion, the onset of chaotic motion in classical mechanical and quantum mechanical systems is compared. It is found that if the spectrum of the system is discrete, the Kolmogorov entropy is zero, and therefore that a bounded quantum mechanical system cannot have chaotic motion like that observed for a corresponding classical mechanical system. This analysis leads to the prediction that if the distributions of states are similar for two bounded systems which in the classical limit have, respectively, quasiperiodic and chaotic motion, wave packets for the two systems decay at similar rates as found by Brumer and Shapiro. The relationship between the defined Kolmogorov entropy, previous interpretations of ’’KAMlike’’ onset of chaos in quantum mechanical systems, and the role played by preparation and observation of a system in influencing the intramolecular dynamics, are discussed.