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Quantum interference with undetected photons for sensing and imaging

Michelini, Chiara

Published Apr 20, 2026• 0 citations
OpenAlex

Abstract

Quantum interference with undetected photons has gained significant attention in the past ten years due to its potential to decouple the probing and the detection of an active sensing system. The technique is based on correlated photon pairs: one photon interacts with the analyte, and the signature of the interaction is stored in its correlated counterpart. The probing photon remains undetected, while the other photon is measured. When the photons are highly non-degenerate, the spectral separation of the probing and detected photons offers significant advantages in terms of ease of operation and enhanced sensitivity, enabling more precise measurements and analysis with respect to other sensing techniques. This possibility enables a wide range of applications, particularly in fields such as imaging, spectroscopy, and optical coherence tomography, among others. This thesis describes experiments for imaging and sensing based on undetected photons, both in a free-space optical setup and in an integrated photonic circuit. The free-space configuration was used to perform undetected three-dimensional imaging reconstruction of diffusive targets. This validation of imaging with undetected photons paves the way to further development to in vivo biomedical imaging, covert imaging, and remote sensing. On the other hand, the integrated configuration overcomes the limitation of alignment tolerance and scalability of a free-space optical setup, enabling the development of integrated sensors based on undetected photons.

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Quantum interference with undetected photons has gained significant attention in the past ten years due to its potential to decouple the probing and the detection of an active sensing system. The technique is based on correlated photon pairs: one photon interacts with the analyte, and the signature of the interaction is stored in its correlated counterpart. The probing photon remains undetected, while the other photon is measured. When the photons are highly non-degenerate, the spectral separation of the probing and detected photons offers significant advantages in terms of ease of operation and enhanced sensitivity, enabling more precise measurements and analysis with respect to other sensing techniques. This possibility enables a wide range of applications, particularly in fields such as imaging, spectroscopy, and optical coherence tomography, among others. This thesis describes experiments for imaging and sensing based on undetected photons, both in a free-space optical setup and in an integrated photonic circuit. The free-space configuration was used to perform undetected three-dimensional imaging reconstruction of diffusive targets. This validation of imaging with undetected photons paves the way to further development to in vivo biomedical imaging, covert imaging, and remote sensing. On the other hand, the integrated configuration overcomes the limitation of alignment tolerance and scalability of a free-space optical setup, enabling the development of integrated sensors based on undetected photons.
Interference measurements with undetected photons employ entangled photon pairs in order to overcome classical limitations in measurement sensitivity. With the undetected photon technique, one photon (signal) interacts with an object, and the signature of the interaction is stored in its entangled counterpart (idler): the interacting photon remains undetected, while the detection is performed on the photon that did not interact with the object. While the signal photon can be chosen in any spectral region suitable for the interaction, the idler photon is generated in a spectral region where detectors are efficient, scalable, and cheap. To date, the configurations proposed are in bulk setups. In this work, we propose a novel configuration on an integrated device, with the advantages of the reduced dimension, the lower cost and the robustness to alignment. In our experiment, we pumped a silicon-on-silica integrated circuit with a classical beam at a wavelength of 1.568 μm. Via intermodal spontaneous four-wave mixing, we generated highly non-degenerate time-energy entangled signal and idler photons at 1.99 μm and 1.29 μm, respectively. As we have integrated two identical sources of entangled photons in series, the photon pairs generated in the two sources are indistinguishable, and controlling the phase of the pump beam and the phase of the signal photons after the first nonlinear source, we observed interference patterns with 24% maximum visibility in the idler photon counts. We successfully measured the dephasing induced on the signal photons by measuring only the idler ones.
Novel imaging techniques utilizing nondegenerate, correlated photon pairs sparked intense interest during the last couple of years among scientists of the quantum optics community and beyond. It is a key property of such “ghost imaging” or “quantum interference” methods that they use those photons of the correlated pairs for imaging that never interacted with the sample, allowing detection in a spectral range different from that of the illumination of the object. Extensive applications of these techniques in spectroscopy and microscopy are envisioned, however, their limited spatial resolution to date has not yet supported real-life microscopic investigations of tiny biological objects. Here we report a modification of the method based on quantum interference by using a seeding laser and confocal scanning, that allows the improvement of the resolution of imaging with undetected photons by more than an order of magnitude, and we also present examples of application in the microscopy of biological samples.
Quantum imaging with undetected photons (QIUP) is an active imaging method in which the detected and the probing photons are distinct and can be selected from different spectral regions. This technique holds potential for a wide range of applications affected by the trade-off between illumination wavelength and detection efficiency. The state-of-the-art experimental configurations assess the spectral absorption and phase information of a target solely in a transmissive configuration, which presents a limitation for applications where the target cannot be aligned with optical elements positioned behind it. In this work, we present an experimental configuration for QIUP of a scattering target, aiming to fill the gap in the applicability of the QIUP technique and enabling QIUP to detect remote targets.
In this work a quantum imaging setup based on undetected squeezed photons is employed for metrological applications such as sensitive phase measurement and quantum imaging. Unlike traditional quantum imaging with undetected photons, as introduced by A. Zeilinger et al., the proposed setup incorporates a homodyne detection system and enhances the brightness of the quantum light using optical parametric oscillators (OPOs). The inclusion of OPOs may challenge the validity of the low-gain approximation, necessitating the development of a new theoretical framework that extends beyond this approximation. The results demonstrate a higher signal-to-noise ratio, which serves as a key metric for both image quality and phase-measurement accuracy. Furthermore, an imaging protocol is introduced to effectively suppress background noise. Notably, this protocol enables the extraction of image information encoded in quantum fluctuations (noise), paving the way for non-disruptive imaging. This is particularly significant in the field of bio-imaging, since the object (a sensitive living cell) is interrogated by longer-wavelength idler light while detection is applied at optical frequency in which the sensors are less noisy and has more quantum efficiency.
Quantum imaging with undetected photons (QIUP) has recently emerged as a new powerful imaging tool. Exploiting the spatial entanglement of photon pairs, it allows decoupling of the sensing and detection wavelengths, facilitating imaging in otherwise challenging spectral regions by leveraging mature silicon-based detection technology. All existing implementations of QIUP have so far utilised the momentum correlations within the biphoton states produced by spontaneous parametric downconversion. Here, for the first time, we implement and examine theoretically and numerically the complementary scenario - utilising the tight position correlations formed within photon pairs at birth. This image plane arrangement facilitates high resolution imaging with comparative experimental ease, and we experimentally show resolutions below 10 μm at a sensing wavelength of 3.7 μm. Moreover, we present a quantitative numerical model predicting the imaging capabilities of QIUP for a wide range of parameters. Finally, by imaging mouse heart tissue at the mid-IR to reveal morphological features on the cellular level, we further demonstrate the viability of this technique for the life sciences. These results offer new perspectives on the capabilities of QIUP for label-free widefield mid-IR microscopy, enabling real-world biomedical as well as industrial imaging applications.
Metrology with undetected photons is an emerging technique that leverages quantum effects and photon correlations (entanglement) to retrieve valuable information in a target spectral range (e.g., mid-infrared, mid-IR) using measurements in an easily accessible domain (e.g., visible, near-IR). The underlying quantum process of spontaneous parametric down-conversion (SPDC) is utilized to generate non-degenerate correlated signal and idler photons to serve as detection and probing photons, respectively. Sensing with undetected photons enables important advantages, such as ultra-low probe powers, room-temperature operation, and shot-noise-limited detection. In this contribution, we apply a quantum nonlinear interferometer based on an SPDC source to perform applied mid-IR spectroscopy, mid-IR microscopy, and mid-IR optical coherence tomography (OCT) as among the most promising techniques for quantum-based routine non-destructive testing. Moreover, we characterize the system, benchmark it against classical systems, and provide a prospective outlook for this new technology.