EN The laser-cooling of ions to temperatures below 1 millikelvin is a standard technique in quantum computing development, but achieving similar cooling for electrons remains difficult. Discovering an effective method could lead to new qubit architecture possibilities. This thesis presents a potential appro- ach for cooling electrons based on Coulomb interactions with laser-cooled ions, providing the necessary theoretical foundation, surveying the latest li- terature, and detailing an experimental implementation currently underway. It also explores how the ultracold ion and electron system could serve as a quantum detector for radio-frequency waves and microwaves. The core ex- perimental work focuses on developing a technique for fabricating miniature optical cavities from optical fibres, with preliminary results and future di- rections for producing highly integrated optical devices provided. 1
"The work presented in this thesis is concerned with the manipulation of laser- cooled rubidium atoms and the detection of small numbers of cold atoms using very sensitive light detectors. Laser-cooled atoms are atoms that have been slowed to very low velocities, corresponding to temperatures of the order of 100 //K, and they can be trapped in magnetic and/or optical traps. The advantage of using cold atoms for experiments in atomic and quantum physics stems from the fact that these atoms are effectively confined within a region of space and this provides longer interaction and observation times compared to atoms at room temperature. Hence, it is possible to explore and observe a number of effects that would otherwise be extremely challenging. The achievement of laser cooling and trapping of neutral atoms was a major breakthrough in the mid 80’s and has resulted in significant advances being made in modern spectroscopy, the realisation of Bose-Einstein condensation, atomic clocks, and quantum information technologies amongst others. In particular, the work focuses on two theoretical proposals for developing microtraps for cold rubidium atoms involving (i) ultrathin optical fibres and (ii) wavelength sized apertures in thin films. In addition, a number of experimental techniques are explored with emphasis on the detection of small numbers of atoms near ultrathin optical fibres using both avalanche photodiodes and single photon detectors. A study on the interactions between atoms and photons is crucial for a full understanding of quantum mechanical processes at the few atom scale and detection schemes sensitive to very low levels of fluorescence from the laser-cooled atoms are vital for attaining this goal. Finally, an experimental study on the design and fabrication of arrays of silica microdisks, that could be used for facilitating interactions between cold atoms and photons, is presented."
This Dissertation details the development of state-of-the-art hybrid atom-ion trapping architecture and technique towards increasing the quantum control of matter and the detection of chemical processes at cold temperatures. Experimental work discussed herein is performed primarily using the second-generation of the MOTion trap, a hybrid atom-ion trap consisting of a co-located magneto-optical trap (MOT) and a linear quadrupole trap (LQT), with which
40Ca and a variety of atomic and molecular ions (Yb
+, Ba
+, BaCl
+, and others) can be co-trapped and cooled. Such a device enables the immersion of laser-cooled, ionic Coulomb crystals in diffuse gases of laser-cooled, highly-polarizable neutral atoms, allowing for studies in sympathetic cooling, cold atom-ion chemistry, and nonequilbrium collisional dynamics.In the first of these studies, I discuss our method of sympathetic cooling in which we use a laser-cooled gas of Ca atoms to sympathetically cool BaCl
+ ions confined in the LQT. Because of the large polarizability of Ca, this method is found to be extremely efficient at cooling the notoriously difficult vibrational degree of freedom. This technique opens the door to research with general, ultracold, highly-localized molecular ions in the quantum ground-state which are not able to be produced using the more traditional methods of Doppler-cooling or photoassociation.In the study of cold chemistry in the hybrid trap, I characterize a fundamental reaction, known as charge exchange, at the single-particle level in which an electron is transferred from a neutral atom to an atomic ion during an inelastic collision. This low-temperature process is thought to be foundational to the chemistry leading to the formation of stars, planets and interstellar clouds in our universe. Herein I discuss how improved experimental architecture has enabled the determination of reaction rate constants for individual electronic states of the reactants.Our theoretical study of the collisional processes in hybrid atom-ion traps has led to the discovery of surprising nonequilibrium physics which exists in the hybrid trap environment. Herein I outline the collisional dynamics between neutral atoms and atomic ions in the presence of a time-dependent confining potential and describe how these dynamics manifest themselves in the emergence of nonequilbrium phenomena as indicated by bifurcations in steady-state energies of trapped ions. I show how the these dynamics can potentially limit the efficiency and overall viability of using neutral buffer gases to sympathetically cool the translational motion of trapped ions to ultracold temperatures.In addition to these experimental studies, the development of architecture is discussed with focus given to the implementation of a novel time-of-flight mass spectrometer (TOF-MS) for use with hybrid atom-ion traps as well as standard LQTs. This simple, modular device couples radially with the LQT and enables the straightforward mass analysis of trapped species without complications derived from typical experimental difficulties, engineering constraints, and financial concerns. With this robust device we precisely characterize chemical processes which can take place in these hybrid atom-ion traps. Additionally, I describe how this new architecture is used to perform the action spectroscopy of several previously unstudied molecular ions in order to further establish the field of cold molecular ion research and the widespread use of hybrid atom-ion traps.
A single trapped ion, laser cooled into its quantum ground state of motion, may be used as a very-low-temperature detector of radio-frequency signals applied to the trap end caps. If the signal source is a resonant oscillator of sufficiently high Q, the source may also be placed in its quantum ground state by coupling to the ion. Parametric couplings may be used to cool and detect source modes other than the mode directly coupled to the ion. A theoretical analysis of these cooling and detection processes is presented, and as an example, their application to single trapped electron and proton spectroscopy is examined. Squeezing and low noise detection of one quadrature component of the source oscillation are also discussed. The techniques discussed here may lead to radio-frequency measurements of improved accuracy and sensitivity. Cooling and detection of vibrations of macroscopic oscillators also appear possible.
Ion traps are widely used to contain and study charged particles. In recent years, there has been an effort to utilize trapped particles as quantum detectors or as components of quantum computers. Before trapping a particle inside an ion trap, it needs to be ionised and cooled, which is commonly achieved using fine-tuned semiconductor lasers. The main objective of this thesis is to develop PID regulator capable of stabilising a 423nm photoionising laser, which is a part of the ion trapping experiment in the Ultracold plasma laboratory. The thesis includes a basic insight into the theory of linear regulators, as well as a detailed implementation procedure with thorough description of employed hardware components.
"In this thesis, laser cooling and trapping techniques are implemented to forrn a cold atom cloud of 85Rb atoms in a magneto-optical trap (Mon configuration. The system produces an atom cloud of~ 1.5 mm in diameter, containing ~ 108 atoms and an average temperature in the sub-Doppler range. Tapered optical fibres (TOFs) are also detailed here, including their guiding properties and the process used for their fabrication. Many possible applications for TOFs have been proposed and one such application is investigated, i.e. the use of TOFs as highly sensitive atom probes. The research results contained within this thesis describe two techniques whereby TOFs can be used as probes. By overlapping the TOF and a cold atom cloud spontaneously emitted photons from the trapped atoms are coupled into the guided mode of the TOF. This then allows characteristics of the cold atom cloud, such as the cloud profile, loading time, lifetime and temperature to be determined. The second technique uses light guided by, but external to, the fibre, i.e. within the evanescent field, to probe the surrounding environment, which may be a cold atom cloud or a background vapour. The work presented also describes a theoretical basis for quantum state preparation using multi-level-atom optics, allowing for the creation of spatial superposition states in which one has perfect control over the population distribution and also the phase relation."
The progress toward laser cooling an ultracold plasma is presented in this thesis. Ultracold neutral plasmas are created by photo-ionizing laser cooled Strontium atoms. Initially this system is very strongly coupled, however the ions rapidly heat up leaving the plasma on the borderline of the strongly coupled regime. To counteract the effects of this heating an attempt to laser cool the ions in the system is undertaken. However, from these experiments we discovered that velocity changing collisions occurring in the system prevented laser cooling. In order to determine the collisions rate, a collision model was developed to simulate the spectra of the plasma from optical pumping experiments. These experiments and simulations in fact demonstrate that collisions are occurring at a fast enough rate to prevent ion cooling on the time scale of our experiment.