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Optical and Quantum Sensing and Precision Metrology II

Quantum-amplified global-phase spectroscopy: a new spectroscopy protocol

Simone Colombo

Published Mar 5, 2026• 0 citations
Publisher

Abstract

I will present our development of global-phase spectroscopy, a Rabi-like metrological protocol inspired by geometric control techniques originally introduced for holonomic quantum gates and based on detuning-dependent Aharonov–Anandan phase. Applied to an optical clock transition, we deployed this method to realize quantum-amplified, time-reversal spectroscopy, yielding 2.4(7) dB metrological gain and 4.0(8) dB laser-noise suppression beyond the standard quantum limit. I will focus on the key metrological advantages of global-phase spectroscopy: i) an intrinsically favorable scaling of sensitivity to local-oscillator high-frequency noise (compared to for Rabi and for Ramsey), and, unlike standard Rabi spectroscopy, ii) featuring quantum enhancement when operated with entangled collective states, such as spin-squeezed inputs. I will close by connecting these results to the broader QIS-NP landscape, highlighting opportunities for applying this protocol to (other) nuclear-spin qubits, nuclear clocks, and other emerging quantum-enhanced sensing and quantum-information platforms.

DOI
10.1117/12.3089850

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I will present our development of global-phase spectroscopy, a Rabi-like metrological protocol inspired by geometric control techniques originally introduced for holonomic quantum gates and based on detuning-dependent Aharonov–Anandan phase. Applied to an optical clock transition, we deployed this method to realize quantum-amplified, time-reversal spectroscopy, yielding 2.4(7) dB metrological gain and 4.0(8) dB laser-noise suppression beyond the standard quantum limit. I will focus on the key metrological advantages of global-phase spectroscopy: i) an intrinsically favorable scaling of sensitivity to local-oscillator high-frequency noise (compared to for Rabi and for Ramsey), and, unlike standard Rabi spectroscopy, ii) featuring quantum enhancement when operated with entangled collective states, such as spin-squeezed inputs. I will close by connecting these results to the broader QIS-NP landscape, highlighting opportunities for applying this protocol to (other) nuclear-spin qubits, nuclear clocks, and other emerging quantum-enhanced sensing and quantum-information platforms.
High-bandwidth, high-stability clocks offer unique chances to study fundamental physics beyond simple metrology. Today, the most stable clocks are optical lattice clocks and they can reach a fractional stability of 3.1 × 10^−18 at 1 s averaging time. Their applications are ranging from the redefinition of the SI time unit, the Second, to the possible detection of gravitational waves in space. The stability of optical lattice clocks is primarily limited by quantum projection noise and Dick noise. In this thesis, I present our effort in creating a platform for studying quantum enhanced metrology and its application towards optical lattice clocks. We demonstrated the laser cooling in an optical cavity with Raman-sideband cooling and achieved average vibration number of n = 0.2. We utilized cavity feedback squeezing to demonstrate unitary spin squeezing on magnetic sub-levels of 171Yb, achieving 6.5 dB quantum projection noise reduction over the standard quantum limit (SQL). With coherent optical state transfer by ultra stable laser pulses, we successfully transferred the spin squeezed state from magnetic sub-levels to the optical transition, and demonstrated quantum enhanced metrology in the optical lattice clock for the first time. We achieved 4.4 dB of metrological gain over the SQL, which corresponds to a reduction of the averaging time by a factor of 2.8 in clock operation. Furthermore, we studied quantum enhanced metrology with time-reversal-based protocols. We performed a signal amplification through time-reversed interaction protocol between the ground state magnetic sublevels of 171Yb, achieving the largest sensitivity improvement beyond SQL in any interferometers to date at 11.8dB. Besides that, we experimentally studied the connection between quantum information scrambling, by measuring out-of-time-order correlators (OTOCs), and quantum metrology, by measuring metrological gain. We found these values to agree with each other, and concluded that the time-reversal quantum metrology can saturate the attainable gain from the quantum information scrambling.
Ramsey interferometry is a widely used tool for precisely measuring transition frequencies between two energy levels of a quantum system, with applications in time keeping, precision spectroscopy, quantum optics, and quantum information. Often, the coherence time of the quantum system surpasses the one of the oscillator probing the system, thereby limiting the interrogation time and associated spectral resolution. Correlation spectroscopy overcomes this limitation by probing two quantum systems with the same noisy oscillator for a measurement of their transition frequency difference; this technique has enabled very precise comparisons of atomic clocks. Here, we extend correlation spectroscopy to the case of multiple quantum systems undergoing strong correlated dephasing. We model Ramsey correlation spectroscopy with N particles as a multiparameter phase estimation problem and demonstrate that multiparticle correlations can assist in reducing the measurement uncertainties even in the absence of entanglement. We derive precision limits and optimal sensing techniques for this problem and compare the performance of probe states and measurement with and without entanglement. Using one- and two-dimensional ion Coulomb crystals with up to 91 qubits, we experimentally demonstrate the advantage of measuring multiparticle correlations for reducing phase uncertainties and apply correlation spectroscopy to measure ion-ion distances, transition frequency shifts, laser-ion detunings, and path-length fluctuations. Our method can be straightforwardly implemented in experimental setups with globally coherent qubit control and qubit-resolved single-shot readout and is, thus, applicable to other physical systems such as neutral atoms in tweezer arrays. Published by the American Physical Society 2024
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Quantum entanglement offers powerful opportunities for enhancing measurement sensitivity beyond classical limits, with optical atomic clocks serving as a leading platform for such advances. This chapter introduces the principles of entanglement-enhanced quantum metrology and explores their applications to timekeeping. We review the theoretical framework of quantum phase estimation, comparing frequentist and Bayesian approaches, and discuss paradigmatic entangled states such as spin-squeezed and GHZ states. Particular emphasis is placed on the challenges posed by decoherence, which constrain the practical advantages that can be realized in large-scale devices. The discussion then turns to frequency estimation in atomic clocks, highlighting how experimental constraints shape the translation of abstract quantum limits into real performance gains. Finally, we outline emerging directions of contemporary quantum metrology. Together, these developments underscore the increasingly close interplay between quantum information processing and precision metrology.
Advances in engineering quantum systems are expected to lead to a new generation of quantum technology with fundamentally new capabilities and no classical analogue. Specifically, in the near future, quantum entanglement may become useful for enhancing state-of-the-art atomic clocks and sensors. I have performed experiments using laser-cooled rubidium atoms trapped in a high finesse optical cavity to explore quantum and collective enhancements to precision measurements.\nIn this thesis, I will present a recent experiment to create record amounts of entanglement-enhancement, or spin squeezing, in a proof-of-principle atomic sensor using entanglement-generating collective measurements. We have demonstrated up to a factor of 60 in directly observed spin squeezing beyond the standard quantum limit for an unentangled quantum sensor and have demonstrated squeezing with real-time feedback to create deterministic entangled states. Second, I will present a new method that has generated over a factor of 10 in homogeneous entanglement that could be resolvable in free-space quantum sensors such as matter-wave interferometers and discuss a new method to reduce errors in manipulating collective spin states using reversible dephasing. These experiments and methods are directly applicable to some of the world's best optical lattice clocks such as those housed here at JILA and NIST.\nIn addition, I have studied and demonstrated a proof-of-principle superradiant laser that relies on collectively enhanced laser emission. These lasers have the potential to realize state-of-the-art frequency purity useful for optical atomic clocks and long baseline interferometry. I will discuss an experiment that demonstrates injection locking of a superradiant laser for the first time as well as explores the collective synchronization behaviors in the system. This study of synchronization informs research on current and future narrow linewidth superradiant lasers and may also provide a platform for future studies of quantum phase transitions in open quantum systems.