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Laser probing measurements and calculations of lifetimes of the 2D3/2 and 2D5/2 metastable states in Ba II

J. Gurell, Émile Biémont, K. Blagoev, V. Fivet, Peter Lundin, S. Mannervik, L.‐O. Norlin, P. Quinet, D. Rostohar, Peder Royen, Peter Schef

Published May 7, 2007• 0 citations
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Proceedings of SPIE, the International Society for Optical Engineering/Proceedings of SPIE•Jun 21, 2004•1 citation
The development of an all-solid-state systems of lasers is described for the cooling and probing of strontium ions in a radio-frequency (rf) trap. The Sr+ ions created within the rf trap are laser cooled by repeated cycling on the 422 nm 2S1/2 - 2P1/2 resonance transition. The 422 nm light was generated from a single mode 70 mW 844 nm diode laser, whose output was frequency doubled to 422 nm in a KNbO3 crystal inside a resonant enhancement cavity. Decays from the Sr+ upper resonance level into the 2D3/2 metastable state remove ions from the cooling cycle. This loss was prevented by driving the 1092 nm 2D3/2 - 2P1/2 transition using a Nd3+-doped fiber laser, diode-pumped at 826 nm. The 2S1/2 - 2D5/2 optical 'clock' transition at 674 nm has a natural linewidth of 0.4 Hz and may be probed with an AlGaInP laser diode. The laser diodes at 844 nm and 674 nm are both collimated using a piezo-mounted GRIN rod which also provides longitudinal mode selection. The spectral output is optically narrowed using resonant optical feedback.
We report advances towards the development of frequency standards based on narrow two-photon transitions in the silver atom at 576 and 661 nm from the ground 4d105s2S1/2 state to the 2D3/2,5/2 levels of the configuration 4d95s2. We describe detection schemes for metastable atoms, localisation of the position of the metastable 2D5/2 level and diode-pumped Nd:YLF lasers around 1.3 μm destined to replace dye lasers for both cooling and spectroscopy of the clock transition. Our result for the position of the 2D5/2 level is more than a factor of two improvement over previous vales.