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Physical Review Letters

Shot-to-Shot Displacement Noise in State-Expansion Protocols with Inverted Potentials

Giuseppe Paolo Seta, Louisiane Devaud, Lorenzo Dania, Lukáš Novotný, Martin Frimmer

Published Mar 2, 2026• 3 citations
Publisher

Abstract

Optically levitated nanoparticles are promising candidates for the generation of macroscopic quantum states of mechanical motion. Protocols to generate such states expose the particle to a succession of different potentials. Limited reproducibility of the alignment of these potentials across experimental realizations introduces additional noise. Here, we experimentally investigate and model how such shot-to-shot noise limits the coherence length of a levitated nanoparticle during a state-expansion protocol using a dark, inverted electrical potential. We identify electric stray fields and mechanical instabilities as major sources of shot-to-shot fluctuations. We discuss the resulting experimental requirements for state-expansion protocols exploiting inverted potentials.

DOI
10.1103/y1q9-pnlc

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Optically levitated nanoparticles are promising candidates for the generation of macroscopic quantum states of mechanical motion. Protocols to generate such states expose the particle to a succession of different potentials. Limited reproducibility of the alignment of these potentials across experimental realizations introduces additional noise. Here, we experimentally investigate and model how such shot-to-shot noise limits the coherence length of a levitated nanoparticle during a state-expansion protocol using a dark, inverted electrical potential. We identify electric stray fields and mechanical instabilities as major sources of shot-to-shot fluctuations. We discuss the resulting experimental requirements for state-expansion protocols exploiting inverted potentials.
Optically levitated nanoparticles are promising candidates for the generation of macroscopic quantum states of mechanical motion. Protocols to generate such states expose the particle to a succession of different potentials. Limited reproducibility of the alignment of these potentials across experimental realizations introduces additional noise. Here, we experimentally investigate and model how such shot-to-shot noise limits the coherence length of a levitated nanoparticle during a state-expansion protocol using a dark, inverted electrical potential. We identify electric stray fields and mechanical instabilities as major sources of shot-to-shot fluctuations. We discuss the resulting experimental requirements for state-expansion protocols exploiting inverted potentials.
Optically levitated nanoparticles are promising candidates for the generation of macroscopic quantum states of mechanical motion. Protocols to generate such states expose the particle to a succession of different potentials. Limited reproducibility of the alignment of these potentials across experimental realizations introduces additional noise. Here, we experimentally investigate and model how such shot-to-shot noise limits the coherence length of a levitated nanoparticle during a state-expansion protocol using a dark, inverted electrical potential. We identify electric stray fields and mechanical instabilities as major sources of shot-to-shot fluctuations. We discuss the resulting experimental requirements for state expansion protocols exploiting inverted potentials.
Powerful approaches to squeeze the motional state of a harmonic oscillator rely on the stepwise modulation of its resonance frequency. Such protocols can be limited by forces that vary slowly between experimental runs but are constant during a single experimental shot. Such shot-to-shot noise gives rise to a spread in experimental outcomes that masks the uncertainty intrinsic to quantum theory. Taking inspiration from spin-echo protocols, we propose a decoupling technique that, under ideal conditions, perfectly cancels shot-to-shot force noise in squeezing experiments based on parametric modulation. We implement the protocol using an optically levitated nanoparticle, where shot-to-shot force noise arises from slowly varying stray fields acting on the charge carried by the particle. Using our oscillator-echo protocol, we demonstrate shot-to-shot noise suppression to the measurement-backaction limit.
Realizing quantum superpositions of massive objects provides a pathway to explore the quantum-to-classical transition. Levitated nanoparticles appear as a promising platform for this purpose due to their large mass and unbound motion. This thesis follows the proposal that particle evolution in a double-well potential expands the particle’s motional state within an inverted harmonic region, while the quartic potential generates the non-Gaussian states needed to certify quantum delocalization. As this protocol has been recently developed, we perform experiments in the classical regime as an important milestone to identify the technical challenges and the decoherence sources. While the nanoparticle’s motional state grows linearly under free evolution, inverted harmonic potentials offer exponentially accelerated state expansion. In this thesis, we experimentally demonstrate the expansion of the center-of-mass state of a 125 nm silica nanoparticle from an initial position uncertainty of 45.6 pm to 43.4 nm within 260 μs. This expansion represents a 952-fold increase, reaching a state size comparable to the particle’s radius, and is achieved by employing an electrostatic inverted potential to disable decoherence from photon recoil. The incoherent dynamics allow us to estimate the remaining decoherence sources in the dark. To accomplish dark dynamics, we developed two segmented linear Paul trap devices providing 2D confinement while generating DC potentials in the third axis of motion: a planar micro-fabricated chip and a PCB based wheel trap. Simulations of tunable double-well potentials of tens to hundreds of micrometers based on the device layouts are performed alongside a study of the resulting classical non-Gaussian states. This work marks a key advancement in the effort to generate macroscopic quantum superpositions at unprecedented mass and length scales.
Nonclassical states of nano- and micro-mechanical motion enable measurements beyond the standard quantum limit and constitute a key resource for quantum sensing and metrology. The most strongly squeezed mechanical states to date have been generated with electromechanical platforms under cryogenic refrigeration and using reservoir engineering. To push mechanical systems deeper into the quantum-squeezed regime requires protocols that increase the rate at which squeezing is generated to more strongly overcome the decoherence rate at which state purity is lost. Here, we squeeze the 800 kHz libration mode of a silica nanoparticle optically levitated in vacuum at room temperature. We expose our mechanical oscillator to an optically generated inverted potential, where the squeezing operation proceeds at an exponentially accelerated rate. We reach a squeezed quadrature variance 11 dB below the vacuum fluctuations within 250 ns. Our protocol establishes a new paradigm for generating quantum squeezing of mechanical motion and offers a platform for quantum-enhanced sensing with massive oscillators.
Levitated nanoparticles in vacuum are prime candidates for generating macroscopic quantum superposition states of massive objects. Most protocols for preparing these states necessitate coherent expansion beyond the scale of the zero-point motion to produce sufficiently delocalized and pure phase-space distributions. Here, we spatially expand and subsequently recontract the thermal state of a levitated nanoparticle by modifying the stiffness of the trap holding the particle. We achieve state-expansion factors of 25 in standard deviation for a particle initially feedback-cooled to a center-of-mass thermal state of \SI{155}{\milli\kelvin}. Our method relies on a hybrid scheme combining an optical trap, for cooling and measuring the particle's motion, with a Paul trap for expanding its state. Consequently, state expansion occurs devoid of measurement backaction from photon recoil, making this approach suitable for coherent wavefunction expansion in future experiments.