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Conductivity of Ultracold Fermions in an Optical Lattice

Rhys Matt Andrew Anderson

Published Jun 1, 2021• 0 citations
OpenAlex

Abstract

In this thesis, we observe and characterize the current response of neutral fermions to a periodic applied force, thereby obtaining their conductivity. The experiment takes place in a 3D optical lattice subject to weak harmonic confinement, where a quantum gas microscope enables high-resolution fluorescence imaging of atoms pinned to lattice sites. Using micron-scale periodic displacements of an underlying harmonic potential to provide the oscillating uniform force, we measure the global current response of the atoms up to frequencies sufficient to characterize intraband transport, but well below the bandgap. We observe that the current response scales linearly with the forcing, providing experimental verification that data is taken in the linear response regime. The resulting conductivity spectra are analyzed and fit using five different models, from which a broadening parameter and the spectral weight of the response may be obtained. Broadening of the current response spectrum provides a measure of the rate of dissipation, and increases with lattice depth, interaction strength, and density. This dissipation occurs purely due to fermion-fermion collisions, given the absence of phonons or impurities in our potentials. It is observed to require a finite lattice depth in order to break Galilean invariance, as well as to enable Umklapp scattering events, which play a significant role in the dynamics. Measured dissipation rates collapse onto the predictions of a kinetic theory under the wide range of conditions studied. The spectral weight of the conductivity spectrum predicts the impulse response of the global current. It satisfies a sum rule in the limit of small lattice depth, but diminishes as the depth increases, reflecting an increase in the band-averaged effective mass. Measured under varying temperatures, densities, interaction strengths, and lattice depths, the spectral weight is shown to collapse onto the predictions of a thermodynamic description of the system. Furthermore, it is shown to be unaffected by varying the strength of interactions between the fermions, illustrating a fundamental prediction for conductivity spectra. As our measurements approach a high-temperature regime, the inverse of the spectral weight is shown to approach T-linear behaviour.

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In this thesis, we observe and characterize the current response of neutral fermions to a periodic applied force, thereby obtaining their conductivity. The experiment takes place in a 3D optical lattice subject to weak harmonic confinement, where a quantum gas microscope enables high-resolution fluorescence imaging of atoms pinned to lattice sites. Using micron-scale periodic displacements of an underlying harmonic potential to provide the oscillating uniform force, we measure the global current response of the atoms up to frequencies sufficient to characterize intraband transport, but well below the bandgap. We observe that the current response scales linearly with the forcing, providing experimental verification that data is taken in the linear response regime. The resulting conductivity spectra are analyzed and fit using five different models, from which a broadening parameter and the spectral weight of the response may be obtained. Broadening of the current response spectrum provides a measure of the rate of dissipation, and increases with lattice depth, interaction strength, and density. This dissipation occurs purely due to fermion-fermion collisions, given the absence of phonons or impurities in our potentials. It is observed to require a finite lattice depth in order to break Galilean invariance, as well as to enable Umklapp scattering events, which play a significant role in the dynamics. Measured dissipation rates collapse onto the predictions of a kinetic theory under the wide range of conditions studied. The spectral weight of the conductivity spectrum predicts the impulse response of the global current. It satisfies a sum rule in the limit of small lattice depth, but diminishes as the depth increases, reflecting an increase in the band-averaged effective mass. Measured under varying temperatures, densities, interaction strengths, and lattice depths, the spectral weight is shown to collapse onto the predictions of a thermodynamic description of the system. Furthermore, it is shown to be unaffected by varying the strength of interactions between the fermions, illustrating a fundamental prediction for conductivity spectra. As our measurements approach a high-temperature regime, the inverse of the spectral weight is shown to approach T-linear behaviour.
We measure the conductivity of neutral fermions in a cubic optical lattice. Using in situ fluorescence microscopy, we observe the alternating current resultant from a single-frequency uniform force applied by displacement of a weak harmonic trapping potential. In the linear response regime, a neutral-particle analog of Ohm's law gives the conductivity as the ratio of total current to force. For various lattice depths, temperatures, interaction strengths, and fillings, we measure both real and imaginary conductivity, up to a frequency sufficient to capture the transport dynamics within the lowest band. The spectral width of the real conductivity reveals the current dissipation rate in the lattice, and the integrated spectral weight is related to thermodynamic properties of the system through a sum rule. The global conductivity decreases with increased band-averaged effective mass, which at high temperatures approaches a T-linear regime. Relaxation of current is observed to require a finite lattice depth, which breaks Galilean invariance and enables damping through collisions between fermions.
We measure the conductivity of neutral fermions in a cubic lattice. A uniform force is applied at a single frequency by periodic displacement of the trapping potential, and the current response is observed though the global displacement of atoms. In the linear response regime, the steady-state ratio between current and force gives the ac conductivity. The tensor properties of the conductivity reveal temporal and spatial symmetries of the sample. Similarly to optical conductivity commonly measured in materials with reflectivity, exact sum rules relate dynamical measurements to thermodynamic properties. We explore the effect of lattice depth, temperature, interaction strength, and atom number on conductivity. Using a relaxation-time approximation, we extract the transport time of current. Our work enables a direct comparison between cold-atom experiments and conductivity studies of materials.
In the present thesis, we discuss the dynamical response to a static forcing of collisionally interacting, neutral fermionic atoms loaded into a one-dimensional optical lattice. It is well known that for a single particle, as well as for many non-interacting particles, there are two fundamental results: the Bloch oscillations of the total momentum and the absence of a net current, which are accompanied by the localization of the particles in configuration space. In our work, we recall (and, in the presence of an additional parabolic confinement, generalize) the single particle results and, then, solve the associated transport problem for two many-particle systems with non-vanishing atom-atom interactions. In the first case, we analyze the behavior of a two-component (i.e., non-pola-rized) fermionic gas under static forcing. We show that, while the atom-atom interactions do not induce a net current of fermions in this system, a variety of new phenomena emerge. These range from the amplitude modulation of Bloch oscillations with a new frequency, which is proportional to the interaction constant, over doubling of the Bloch frequency, to a rescaling of the characteristic time scales at strong interactions. In the second case, we discuss the requirements to witness directed atomic transport, and propose a microscopic model to describe the normal transport behavior of a dilute gas of polarized (hence non-interacting) fermions, where the net current emerges due to the collision-induced coupling with the finite bath, which is made of bosonic atoms loaded in to the same optical lattice. The outcome is a current-voltage'' characteristics which displays both Ohmic and negative differential conductivity, and a maximum current right at the transition between both regimes. This transition point is completely determined by the microscopic model parameters, and weakly depends on the bath temperature, while the current amplitude asymptotically vanishes with increasing temperature.
We investigate the interaction-induced resistivity of ultracold fermions in a three-dimensional optical lattice. In situ observations of transport dynamics enable the determination of real and imaginary resistivity. In the strongly interacting metallic regime, we observe a striking saturation of the current-dissipation rate toward a value that is independent of the interaction strength. This phenomenon is quantitatively captured by a dissipation model that uses a renormalized two-body scattering matrix. We further measure the temperature dependence of resistivity in the strongly interacting limit and discuss the predicted asymptotic high-temperature behavior. Our results provide a clear microscopic understanding of bounded resistivity of low-density metals, thus providing a useful benchmark for studies of strongly correlated atomic and electronic systems.
We study a harmonically confined atomic gas which is subjected to an additional external potential such as an optical lattice. Using a linear response formulation, we determine the response of the gas to a small, time-dependent displacement of the harmonic trap and derive a simple exact relation showing that the centre-of-mass position of the atomic cloud is directly related to the global optical conductivity of the system. We demonstrate the usefulness of this approach by calculating the optical conductivity of bosonic atoms in an optical lattice. In the Mott insulating phase, there is clear evidence of an optical Mott gap, providing a proof-of-principle demonstration that the global optical conductivity gives high-quality information about the excitations of strongly correlated quantum gases.
This dissertation presents my research covering the field of ultracold atoms loaded in optical lattices. The static and dynamical properties of atoms in combined periodic and parabolic potentials are studied, with a focus on the strongly interacting regimes. Because parabolic magnetic and optical potentials are routinely used to confine atoms, the results of this research are directly relevant to ongoing experimental endeavours in atomic physics. After a review of the basic theory of atoms in homogeneous periodic potentials, the equilibrium and non-equilibrium properties of non-interacting and interacting atoms in periodic plus parabolic potentials are studied. The problem of the localization of the many-body wavefunction for systems with arbitrary peak onsite density is presented in Chapters 3 and 4. The physics pertaining to the experimental realization of Mott insulator states with one or more atoms per sites in inhomogeneous lattices is elucidated by introducing an intuitive model for strongly interacting bosons in one dimension. This model is then utilized to study the decay of the dipole oscillations of atomic ensembles subject to a small displacement of the parabolic potential. Good agreement is found with results of recent experiments. Chapters 5 and 6 are dedicated to the characterization of the Mott insulator state with unit filling, which plays a central role in proposed schemes for neutral atom quantum computation. The usefulness of Bragg spectroscopy to probe the excitation spectrum of the Mott state in homogeneous lattices is analyzed in Chapter 5, where the limits of validity of linear response theory in this strongly correlated regime are delimited. In Chapter 6 the effects of finite temperature on the confined Mott insulator state are studied, and a scheme is devised for possibly estimating the system's temperature, at energies of the order of the inter-particle interaction energy. Finally, in Chapter 7, a proposal is introduced to utilize the Mott state as a robust register for neutral atom quantum computation. Unwanted residual quantum coherences inherent to the Mott insulator ground state are eliminated by a judicious choice of the trapping potentials and a selective measurement on a molecular photo-associative transition.